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Unique superconductivity at surfaces/interfaces, as exemplified by LaAlO3/SrTiO3 interfaces, and the high transition temperature in ultrathin FeSe films, have triggered intense debates on how superconductivity is affected in atomic and…

Rutile Sn$_{1-x}$Ge$_x$O$_{2}$ alloys are promising materials for high-power electronic applications due to their dopability and tunable ultra-wide band gaps. We use first-principles density functional theory and statistical mechanics to…

Thermal transport by phonons in films with thicknesses of less than 10 nm is investigated in a soft system (Lennard-Jones argon) and a stiff system (Tersoff silicon) using two-dimensional lattice dynamics calculations and the Boltzmann…

介观与纳米尺度物理 · 物理学 2020-01-22 Bo Fu , Kevin D. Parrish , Hyun-Young Kim , Guihua Tang , Alan J. H. McGaughey

We report on the successful synthesis of highly conductive PdCoO2 ultrathin films on Al2O3 (0001) by pulsed laser deposition. The thin films grow along the c-axis of the layered delafossite structure of PdCoO2, corresponding to the…

强关联电子 · 物理学 2018-04-24 T. Harada , K. Fujiwara , A. Tsukazaki

Motivated by the recently observed unconventional Hall effect in ultra-thin films of ferromagnetic SrRuO$_3$ (SRO) we investigate the effect of strain-induced oxygen octahedral distortion in the electronic structure and anomalous Hall…

材料科学 · 物理学 2021-03-31 Kartik Samanta , Marjana Ležaić , Stefan Blügel , Yuriy Mokrousov

The lattice dynamics of TiO$_2$ in the rutile crystal structure was studied by a combination of thermal diffuse scattering, inelastic x-ray scattering and density functional perturbation theory. We experimentally confirm the existence of an…

材料科学 · 物理学 2016-01-13 Björn Wehinger , Alexeï Bosak , Paweł T. Jochym

The ultrathin film limit has been shown to be a rich playground for unusual low dimensional physics. Taking the example of SrRuO$_3$ which is ferromagnetic and metallic at the bulk limit, one finds that it becomes antiferromagnetic and…

材料科学 · 物理学 2014-09-10 Kapil Gupta , Basudeb Mandal , Priya Mahadevan

Binary rutile oxides of 5d metals such as IrO2, stand out as a paradox due to limited experimental studies despite the rich predicted quantum phenomena. Here, we investigate the electrical transport properties of IrO2 by engineering…

材料科学 · 物理学 2024-05-21 Sreejith Nair , Zhifei Yang , Kevin Storr , Bharat Jalan

Mott metal-insulator transitions possess electronic, magnetic, and structural degrees of freedom promising next generation energy-efficient electronics. We report a previously unknown, hierarchically ordered state during a Mott transition…

The large spin-orbit coupling in iridium oxides plays a significant role in driving novel physical behaviors, including emergent phenomena in the films and heterostructures of perovskite and Ruddlesden-Popper iridates. In this work, we…

PtSe2 is attracting considerable attention as a high mobility two-dimensional material with envisionned applications in microelectronics, photodetection and spintronics. The growth of high quality PtSe2 on insulating substrates with…

Lattice structure can dictate electronic and magnetic properties of a material. Especially, reconstruction at a surface or heterointerface can create properties that are fundamentally different from those of the corresponding bulk material.…

We report on the systematic characterization of Ba(Fe$_{0.92}$Co$_{0.08}$)$_2$As$_2$ epitaxial thin films on CaF$_2$ substrate in view of their possible use for superconducting electronic applications. By using different and complementary…

超导电性 · 物理学 2016-09-02 D. Daghero , P. Pecchio , F. Laviano , R. S. Gonnelli , F. Kurth , V. Grinenko , K. Iida

Three different film systems have been systematically investigated to understand the effects of strain and substrate constraint on the phase transitions of perovskite films. In SrTiO$_3$ films, the phase transition temperature T$_C$ was…

其他凝聚态物理 · 物理学 2007-05-23 Feizhou He , B. O. Wells , Z. -G. Ban , S. P. Alpay , S. Grenier , S. M. Shapiro , Weidong Si , A. Clark , X. X. Xi

The availability of low-index rutile TiO2 single crystal substrates with atomically flat surfaces is essential for enabling epitaxial growth of rutile transition metal oxide films. The high surface energy of the rutile (001) surface often…

High-critical-temperature (Tc) superconductivity at 48 K is reported for hydrogen-doped SmFeAsO epitaxial films on MgO single-crystal substrates. The key processes are pulsed laser deposition to grow undoped SmFeAsO epitaxial films and…

Photocatalytic materials are pivotal for the implementation of disruptive clean energy applications such as conversion of H$_{2}$O and CO$_{2}$ into fuels and chemicals driven by solar energy. However, efficient and cost-effective materials…

材料科学 · 物理学 2019-09-04 Zhao Liu , Joel Shenoy , Cesar Menéndez , Judy N. Hart , Charles C. Sorrell , Claudio Cazorla

Altermagnets, which exhibit the advantages of both antiferromagnets and ferromagnets, have attracted significant attention recently. Among them, ruthenium dioxide (RuO2), a prototypical altermagnet candidate, is under intensive debate on…

We explore the electrical transport and magneto-conductance in quasi two-dimensional strongly correlated ultrathin films of LaNiO$_{3}$ (LNO) to investigate the effect of hetero-epitaxial strain on electron-electron and electron-lattice…

强关联电子 · 物理学 2015-05-28 E. J. Moon , B. A. Gray , M. Kareev , J. Liu , S. G. Altendorf , F. Strigari , L. H. Tjeng , J. W. Freeland , J. Chakhalian

Weakly disordered superconducting films can be driven into an anomalous low temperature resistive state upon applying a magnetic field. Recent experiments on weakly disordered amorphous InO$_x$ have established that both the Hall…

超导电性 · 物理学 2018-07-04 Luca V. Delacrétaz , Sean A. Hartnoll