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The electrical performance of two dimensional transitional metal dichalcogenides (TMDs) is strongly influenced by the amount of structural defects inside. In this work, we provide an optical spectroscopic characterization approach to…

We directly measure the nonlinear optical response in argon and nitrogen in a thin gas target to laser intensities near the ionization threshold. No instantaneous negative nonlinear refractive index is observed, nor is saturation, in…

光学 · 物理学 2015-05-28 J. K. Wahlstrand , Y. -H. Cheng , Y. -H. Chen , H. M. Milchberg

We have fabricated Ce/Pd bilayers grown on the SiO$_2$ substrate by magnetron sputtering under ultrahigh vacuum. Usage of palladium layer on top of the Ce film appears to prevent effectively the sample oxidation. The thickness of the cerium…

强关联电子 · 物理学 2018-06-13 P. Skokowski , A. Marczyńska , S. Pacanowski , T. Toliński , B. Szymański , Ł. Majchrzycki , L. Smardz

Optical parametric amplification (OPA) represents a powerful solution to achieve broadband amplification in wavelength ranges beyond the scope of conventional gain media, for generating high-power optical pulses, optical microcombs,…

We introduce a nanomechanical platform for fast and sensitive measurements of the spectrally-resolved optical dielectric function of 2D materials. At the heart of our approach is a suspended 2D material integrated into a nanomechanical…

Two-dimensional (2D) nanomaterials, especially the transition metal sulfide semiconductors, have drawn great interests due to their potential applications in viable photonic and optoelectronic devices, such as saturable absorbers (SAs) and…

光学 · 物理学 2023-07-19 Kan Wu , Xiaoyan Zhang , Jun Wang , Xing Li , Jianping Chen

Here, we report the full-fledged journey towards the material synthesis and characterization of few-layered/thin WSe$_2$ using sputtered W-films on SiO$_2$/Si substrates followed by electrical studies under dark and illumination conditions.…

We present nonlinear dielectric measurements of glass-forming glycerol and propylene carbonate applying electrical fields up to 671 kV/cm. The measurements extend to sufficiently high frequencies to allow for the investigation of the…

软凝聚态物质 · 物理学 2013-03-20 Th. Bauer , P. Lunkenheimer , S. Kastner , A. Loidl

A dielectric material's response to light is macroscopically described by electric displacement fields due to polarization and susceptibility, but the atomistic origin is light-cycle-driven motion of electron densities in the restoring…

Monolayers of transition-metal dichalcogenides such as WSe2 have become increasingly attractive due to their potential in electrical and optical applications. Because the properties of these 2D systems are known to be affected by their…

We have derived the local electric field inside graded metal-dielectric composite films with weak nonlinearity analytically, which further yields the effective linear dielectric constant and third-order nonlinear susceptibility of the…

材料科学 · 物理学 2007-05-23 J. P. Huang , L. Dong , K. W. Yu

The pronounced dependence of the nonlinear parameters of both dielectric and semiconductor materials on the wavelength, and the nonlinear interaction between the ultra-short laser pulse and the material requires precise control of the…

光学 · 物理学 2022-01-28 Roland Axel Richter , Vladimir Kalashnikov , Irina T. Sorokina

Lateral two-dimensional (2D) transitional metal dichalcogenide (TMD) heterostructures have recently attracted a wide attention as promising materials for optoelectronic nanodevices. Due to the nanoscale width of lateral heterojunctions, the…

光学 · 物理学 2018-07-18 Chenwei Tang , Zhe He , Weibing Chen , Shuai Jia , Jun Lou , Dmitri V. Voronine

Layered indium selenide (InSe), a new two-dimensional (2D) material with a hexagonal structure and semiconducting characteristic, is gaining increasing attention owing to its intriguing electronic properties. Here, by using first-principles…

材料科学 · 物理学 2017-12-19 Andrey A. Kistanov , Yongqing Cai , Kun Zhou , Sergey V. Dmitriev , Yong-Wei Zhang

We utilize the recently demonstrated orders of magnitude enhancement of extremely nondegenerate two-photon absorption in direct-gap semiconductor photodiodes to perform scanned imaging of 3D structures using IR femtosecond illumination…

The dynamics of thermal and non-thermal lattice deformation of nanometer thick polycrystalline aluminum film has been studied by means of femtosecond (fs) time-resolved electron diffraction. We utilized two different pump wavelengths: 800…

材料科学 · 物理学 2017-09-13 Runze Li , Pengfei Zhu , Jie Chen , Jianming Cao , Peter M. Rentzepis , Jie Zhang

Over the last few years, ReS2 has generated a myriad of unattended queries regarding its structure, the concomitant thickness dependent electronic properties and apparently contrasting experimental optical response. In this work, with…

Dielectric metasurfaces have shown prominent applications in nonlinear optics due to strong field enhancement and low dissipation losses at the nanoscale. Chalcogenide glasses are one of the promising materials for the observation of…

Herein we describe a novel spinning pump-probe photoacoustic technique developed to study nonlinear absorption in thin films. As a test case, an organic polycrystalline thin film of quinacridone, a well-known pigment, with a thickness in…

Nonlinear optical microscopy such as in the optical second-harmonic generation (SHG) modality has become a popular tool today for probing materials in the physical and biological sciences. While imaging and spectroscopy are widely used in…

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