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We present a scalable method for direct patterning of graphite and transition metal dichalcogenide (TMD) films on polycarbonate (PC) and other transparent substrates using fiber laser ablation. This process facilitates the fabrication of…

应用物理 · 物理学 2025-06-05 Yigit Sozen , Yu Kyoung Ryu , Javier Martinez , Andres Castellanos-Gomez

We report the observation and interpretation of new Raman peaks in few-layer tungsten diselenide (WSe2), induced by the reduction of symmetry going from 3D to 2D. In general, Raman frequencies in 2D materials follow quite closely the…

材料科学 · 物理学 2014-01-06 Xin Luo , Yanyuan Zhao , Jun Zhang , Minglin Toh , Christian Kloc , Qihua Xiong , Su Ying Quek

We show that bulk rhenium diselenide, ReSe2 is characterized by record high value of the refractive index exceeding 5 in near-infrared frequency range. We use back focal plane reflection spectroscopy to extract the components of the ReSe2…

介观与纳米尺度物理 · 物理学 2023-01-18 Alexey Mikhin , Anton Shubnic , Tatyana Ivanova , Ivan Shelykh , Anton Samusev , Ivan Iorsh

One-dimensional (1D) metal-dielectric (MD) periodic structures take advantage of large refractive index contrast between metal and dielectrics to invoke extremely high nonlinear ultrafast responses of metal. These structures are also…

On-chip integration of two-dimensional (2D) materials offers great potential for the realization of novel optoelectronic devices in different photonic platforms. In particular, indium selenide (InSe) is a very promising 2D material due to…

Due to the absence of interlayer coupling and inversion symmetry, transition metal dichalcogenide (MX$_2$) semiconductor monolayers exhibit novel properties that are distinctly different from their bulk crystals such as direct optical band…

介观与纳米尺度物理 · 物理学 2015-06-16 Chung-Yu Wang , Guang-Yu Guo

We have developed a nonlinear differential effective dipole approximation (NDEDA), in an attempt to investigate the effective linear and third-order nonlinear susceptibility of composite media in which graded spherical inclusions with weak…

材料科学 · 物理学 2007-05-23 L. Gao , J. P. Huang , K. W. Yu

Electromagnetically induced transparency in an optically thick, cold medium creates a unique system where pulse-propagation velocities may be orders of magnitude less than $c$ and optical nonlinearities become exceedingly large. As a…

量子物理 · 物理学 2009-11-10 Danielle A. Braje , Vlatko Balic , G. Y. Yin , S. E. Harris

The invention of laser immediately enabled us to detect nonlinearities of photon interaction in matter, as manifested for example by Franken et al.'s detection of second harmonic generation and the excitation of the Brillouin forward…

量子物理 · 物理学 2010-06-24 Kensuke Homma , Dieter Habs , Toshiki Tajima

Palladium diselenide (PdSe2) is a recently isolated layered material that has attracted a lot of interest for the pentagonal structure, the air stability and the electrical properties largely tunable by the number of layers. In this work,…

应用物理 · 物理学 2020-08-25 A. Di Bartolomeo , F. Urban , A. Pelella , A. Grillo , M. Passacantando , X. Liu , F. Giubileo

2D materials offer a large variety of optical properties, from transparency to plasmonic excitation. They can be structured and combined to form heterostructures that expand the realm of possibility to manipulate light interactions at the…

光学 · 物理学 2023-09-27 Bruno Majérus , Emerick Guillaume , Pascal Kockaert , Luc Henrard

The determination of the nonlinear optical coefficient \( n_2 \) of pure water is of great interest for applications such as imaging biological systems, performing femtosecond laser surgery, and underwater ablation. Traditionally, probing…

光学 · 物理学 2025-02-06 Ilyes Betka

We report first-principles calculations of the frequency dependent linear and second-order optical properties of the two probable extended-solid phases of CO$_2$--V, i.e. $I\bar42d$ and $P2_12_12_1$. Compared to the parent $Cmca$ phase the…

材料科学 · 物理学 2009-11-10 S. Sharma , J. K. Dewhurst , C. Ambrosch-Draxl

We investigate the nonlinear optical response of a commercial extended-wavelength In$_{0.81}$Ga$_{0.19}$As photodetector. Degenerate two-photon absorption in the mid-infrared range is observed at room temperature using a quantum cascade…

In this paper two-photon absorption coefficient $\beta$ and nonlinear refractive index ${n}_{2}$ have been measured at 1064 nm for a new two-dimensional (CH3(CH2)2NH3)2(CH3NH3)2Pb3Br10 hybrid perovskite. The nonlinear optical properties…

Following a recently manifested guide of how to team up infrared transparency and high electrical conductivity within semimetal materials [C. Cui $et$ $al.$ Prog. Mater. Sci. 2023, 136, 101112], we evaluate an applicability of the calcium…

We report on the successful synthesis of highly conductive PdCoO2 ultrathin films on Al2O3 (0001) by pulsed laser deposition. The thin films grow along the c-axis of the layered delafossite structure of PdCoO2, corresponding to the…

强关联电子 · 物理学 2018-04-24 T. Harada , K. Fujiwara , A. Tsukazaki

Monolayer transition metal dichalcogenides (e.g., MoS2) exhibit exceptionally large optical nonlinearities for high-order nonlinear light generation (NLG), yet their inherent atomic thickness fundamentally limits light-matter interactions…

In this article, we employed nanosecond Z-scan technique to demonstrate the nonlinear optical response in Ge30Se55Bi15 thin films after thermal and photo annealing. The intensity dependent open aperture Z-scan traces reveal that for all the…

光学 · 物理学 2020-02-26 Adyasha Aparimita , Pritam Khan , J. R. Aswin , K. V Adarsh , R. Naik

The development of nanomaterials with a large nonlinear susceptibility is essential for nonlinear nanophotonics. We show that transition-metal-dichalcogenide (TMD) nanotriangles have a large effective second-order susceptibility…

光学 · 物理学 2021-04-07 F. Karimi , S. Soleimanikahnoj , I. Knezevic