Optical nonlinearity in Ar and N$_2$ near the ionization threshold
Abstract
We directly measure the nonlinear optical response in argon and nitrogen in a thin gas target to laser intensities near the ionization threshold. No instantaneous negative nonlinear refractive index is observed, nor is saturation, in contrast with a previous measurement [Loriot et al., Opt. Express v. 17, 13429 (2009)] and calculations [Br\'ee et al., Phys. Rev. Lett. v. 106, 183902 (2011)]. In addition, we are able to cleanly separate the instantaneous and rotational components of the nonlinear response in nitrogen. In both Ar and N, we observe the peak instantaneous index response scale linearly with the laser intensity until the point of ionization, whereupon it turns abruptly negative and ~constant, consistent with plasma generation.
Cite
@article{arxiv.1105.6334,
title = {Optical nonlinearity in Ar and N$_2$ near the ionization threshold},
author = {J. K. Wahlstrand and Y. -H. Cheng and Y. -H. Chen and H. M. Milchberg},
journal= {arXiv preprint arXiv:1105.6334},
year = {2015}
}
Comments
Slightly extended version including data with 800 nm probe. 5 pages, 4 figures