English

Optical nonlinearity in Ar and N$_2$ near the ionization threshold

Optics 2015-05-28 v3 Atomic Physics Plasma Physics

Abstract

We directly measure the nonlinear optical response in argon and nitrogen in a thin gas target to laser intensities near the ionization threshold. No instantaneous negative nonlinear refractive index is observed, nor is saturation, in contrast with a previous measurement [Loriot et al., Opt. Express v. 17, 13429 (2009)] and calculations [Br\'ee et al., Phys. Rev. Lett. v. 106, 183902 (2011)]. In addition, we are able to cleanly separate the instantaneous and rotational components of the nonlinear response in nitrogen. In both Ar and N2_2, we observe the peak instantaneous index response scale linearly with the laser intensity until the point of ionization, whereupon it turns abruptly negative and ~constant, consistent with plasma generation.

Keywords

Cite

@article{arxiv.1105.6334,
  title  = {Optical nonlinearity in Ar and N$_2$ near the ionization threshold},
  author = {J. K. Wahlstrand and Y. -H. Cheng and Y. -H. Chen and H. M. Milchberg},
  journal= {arXiv preprint arXiv:1105.6334},
  year   = {2015}
}

Comments

Slightly extended version including data with 800 nm probe. 5 pages, 4 figures

R2 v1 2026-06-21T18:15:29.933Z