相关论文: Long-range Rydberg molecule Rb$_2$: Two-electron \…

Ultra-long-range Rydberg molecules (ULRMs) have attracted significant interest due to their unique electronic properties and potential applications in quantum technologies. We theoretically investigate the formation and characteristics of…

Rydberg atoms with principal quantum number n >> 1 have exaggerated atomic properties including dipole-dipole interactions that scale as n^4 and radiative lifetimes that scale as n^3. It was proposed a decade ago to take advantage of these…

Ultracold YbAg molecules have been recently proposed as promising candidates for electron electric dipole moment searches [Verma, Jayich, and Vutha, Phys. Rev. Lett. 125, 153201 (2020)]. Here, we calculate potential energy curves, permanent…

We present a study of the variation of total energies and excitationenergies along a range-separated adiabatic connection. This connectionlinks the non-interacting Kohn-Sham electronic system to the physicalinteracting system by…

Estimating energy gaps, i.e. the energy difference between two different states, in quantum systems is crucial for understanding their properties. Conventionally, spectral gap estimation relies on independently computing the ground-state…

Electron-impact cross sections for the dissociation process of vibrationally excited He2+ molecular ion, as a function of the incident electron energy are calculated for the dissociative transition X2\Sigma+u \to A2\Sigma+g by using the…

In this paper, we report on numerical calculations of the spontaneous emission rates and Lamb shifts of a $^{87}\text{Rb}$ atom in a Rydberg-excited state $\left(n\leq30\right)$ located close to a silica optical nanofiber. We investigate…

The passage of cold cesium 49S$_{1/2}$ Rydberg atoms through an electric-field-induced multi-level avoided crossing with nearby hydrogen-like Rydberg levels is employed to prepare a cold, dipolar Rydberg atom gas. When the electric field is…

Structural properties of a finite number ($N = 2 - 20$) of point charges (classical electrons) confined laterally in a two-dimensional two-minima potential are calculated as a function of the distance ($d$) between the minima. The particles…

Rydberg atoms have large transition electric dipole moments and high sensitivity to electric fields. We describe a new method for microwave field sensing in a vapor cell consisting of separate excitation, quantum evolution between two…

Ultracold trapped atomic ions excited into highly energetic Rydberg states constitute a promising platform for scalable quantum information processing. Elementary building blocks for such tasks are high-fidelity and sufficiently fast…

Atoms in highly excited (Rydberg) states have a number of unique properties which make them attractive for applications in quantum information. These are large dipole moments, lifetimes and polarizabilities, as well as strong long-range…

We study a novel regime of the Rydberg excitation blockade using highly Stark-shifted, yet long-living, states of Rb atoms subject to electric fields above the classical ionization limit. Such states allow tuning the dipole-dipole…

We review ultralong-range Rydberg molecules (ULRM), which are bound states between a Rydberg atom and one or more ground-state atoms with bond lengths on the order of thousands of Bohr radii. The binding originates from multiple…

Rydberg atoms, with their giant electronic orbitals, exhibit dipole-dipole interaction reaching the GHz range at a distance of a micron, making them a prominent contender for realizing quantum operations well within their coherence time.…

We revisit the implementation of a two-qubit entangling gate, the M{\o}lmer-S{\o}rensen gate, using the adiabatic Rydberg dressing paradigm for neutral atoms as studied in [Phys. Rev. A 101, 030301 (R) (2020)]. We study the implementation…

Motivated by recent progress in the experimental manipulation of cold atoms in optical lattices, we study three different protocols for non-adiabatic quantum state preparation and state transport in chains of Rydberg atoms. The protocols we…

Density functional calculations of Rydberg excited states up to high energy are carried out for several molecules using an approach where the orbitals are variationally optimized by converging on saddle points on the electronic energy…

An operator that generates an approximate symmetry of long-range Rydberg molecules (LRRMs) formed by two alkali atoms, one in a Rydberg state and the other in the ground state, is identified. This is first done by evaluating the natural…

We theoretically explore photoassociation by Adiabatic Passage of two colliding cold ^{85}Rb atoms in an atomic trap to form an ultracold Rb_2 molecule. We consider the incoherent thermal nature of the scattering process in a trap and show…