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We present a density-functional theory study of the effects of oxygen vacancies on the structural and electronic properties of vanadium dioxide (VO$_2$). Our motivation is the reported suppression of the metal-insulator transition by oxygen…

材料科学 · 物理学 2025-11-11 Oskar Leibnitz , Peter Mlkvik , Nicola A. Spaldin , Claude Ederer

The magneto-optical properties of titanium dioxide systems are related to the presence of impurity states in the band gap due to oxygen vacancies. To understand about the interplay between localized electrons and structural distortions at…

材料科学 · 物理学 2023-05-10 C. Echeverria-Arrondo , H. Raebiger , J. Perez-Conde , C. Gomez-Polo , A. Ayuela

We investigate the behavior of oxygen vacancies in three different metal-oxide semiconductors (rutile and anatase TiO2, monoclinic WO3, and tetragonal ZrO2) using a recently proposed hybrid density-functional method in which the fraction of…

The formation energies and electronic structure of europium doped zinc oxide has been determined using DFT and many-body $GW$ methods. In the absence of intrisic defects we find that the europium-$f$ states are located in the ZnO band gap…

材料科学 · 物理学 2016-03-23 M. Lorke , T. Frauenheim , A. L. da Rosa

In a common paradigm, the electronic structure of condensed matter is divided into weakly and strongly correlated compounds. While conventional band theory usually works well for the former class, many-body effects are essential for the…

材料科学 · 物理学 2016-03-17 Frank Lechermann , Harald O. Jeschke , Aaram J. Kim , Steffen Backes , Roser Valenti

The large error of the DFT+U method on full-filled shell metal oxides is due to the residue of self-energy from the localized d orbitals of cations and p orbitals of the anions. U parameters are self-consistently found to achieve the…

材料科学 · 物理学 2016-03-23 Bolong Huang

Photocatalysis, a promising solution for environmental challenges, relies on the generation and utilization of photogenerated charge carriers within photocatalysts. However, recombination of these carriers often limits efficiency.…

材料科学 · 物理学 2024-03-18 Mona Asadinamin , Aleksandar Živkovic , Nora H. De Leeuw , Steven P. Lewis

The structural and electronic properties of cubic GaN are studied within the local density approximation by the full-potential linear muffin-tin orbitals method. The Ga $3d$ electrons are treated as band states, and no shape approximation…

凝聚态物理 · 物理学 2009-10-22 Vincenzo Fiorentini , Michael Methfessel , Matthias Scheffler

We perform full-potential screened-hybrid density-functional theory (DFT) calculations to compare the thermodynamic stability of neutral and charged states of the surface oxygen vacancy at the rutile TiO$_2$(110) surface. Solid-state…

材料科学 · 物理学 2015-08-19 Daniel Berger , Harald Oberhofer , Karsten Reuter

Hubbard-corrected density functional theory, denoted by DFT+U method, was developed to enable correct prediction of insulating properties for strongly-correlated electron systems. UO$_2$ is an example having O-$2p$, U-$6d$, and U-$5f$…

强关联电子 · 物理学 2023-02-28 Mahmoud Payami

CdTe and its alloy CdTeSe are widely used in optoelectronic devices, such as radiation detectors and solar cells, due to their superior electrical properties. However, the formation of defects and defect complexes in these materials can…

材料科学 · 物理学 2024-08-29 Xiaofeng Xiang , Yijun Tong , Aaron Gehrke , Scott Dunham

In this study, oxygen vacancies and adatoms have been considered on the surface of both hexagonal and triangular ZnO nanowires. Their effect on the electronic structure and optical spectra of the nanowires have been investigated using the…

强关联电子 · 物理学 2018-03-01 Veysel Çelik , Ersen Mete

Defects in halide perovskites play an essential role in determining the efficiency and stability of the resulting optoelectronic devices. Here, we present a systematic study of intrinsic point defects in six primary metal halide…

材料科学 · 物理学 2022-01-03 Haibo Xue , Geert Brocks , Shuxia Tao

In some topological insulators, such as graphene and WTe$_2$, band inversion originates from chemical bonding and space group symmetry, in contrast to materials such as Bi$_2$Se$_3$, where the band inversion derives from relativistic…

材料科学 · 物理学 2020-07-15 Lukas Muechler , Wei Hu , Chao Yang , Lin Lin , Roberto Car

Oxygen vacancies are ubiquitous in TiO$_2$ and play key roles in catalysis and magnetism applications.Despite being extensively investigated, the electronic structure of oxygen vacancies in TiO$_2$ remains controversial both experimentally…

材料科学 · 物理学 2021-02-03 Ji Chen , Nikolay A. Bogdanov , Denis Usvyat , Wei Fang , Angelos Michaelides , Ali Alavi

Room temperature ferromagnetism is observed in undoped TiO2 films deposited on Si substrates using pulsed laser deposition (PLD). The ferromagnetic properties of the samples depend on the oxygen partial pressure during the PLD synthesis.…

材料科学 · 物理学 2009-11-13 Abdul K Rumaiz , Bakhtyar Ali , Abdullah Ceylan , M. Boggs , T. Beebe , S. Ismat Shah

Vivianite (Fe$_3$(PO$_4$)$_2$8H$_2$O) is a naturally occurring layered material with significant environmental and technological relevance. This work presents a comprehensive theoretical investigation of its two-dimensional (2D)…

The structural and electronic properties of the wurtzite phase of the InAs and GaAs compounds are, for the first time, studied within the framework of Density Functional Theory (DFT). We used the full-potential linearized augmented plane…

材料科学 · 物理学 2007-05-23 Zeila Zanolli , Ulf von Barth

An investigation of U2Ti, a potentially safe and heavy metal-based storage material for radioactive tritium for fusion reactor, has been performed using pseudopotential density functional theory. The analysis of the elastic constants and…

材料科学 · 物理学 2012-06-27 M. Z. Hasan , M. M. Hossain , M. S. Islam , F. Parvin , A. K. M. A. Islam

We have carried out ab initio electronic structure calculations on graphane (hydrogenated graphene) with single and double vacancy defects. Our analysis of the density of states reveal that such vacancies induce the mid gap states and…

材料科学 · 物理学 2010-02-11 Bhalchandra S. Pujari , D. G. Kanhere