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In crystals, energy band extrema in momentum space can be identified by their valley index. The internal quantum degree of freedom associated with valley pseudospin indices can act as a useful information carrier analogous to electronic…

Electrical control over the energy exchange between exciton states mediated by cavity-polaritons at room temperature is demonstrated. Spatially separated field effect transistors based on monolayers of WS$_2$ and MoS$_2$ are placed in a…

介观与纳米尺度物理 · 物理学 2019-09-04 Henry A. Fernandez , Freddie Withers , Saverio Russo , William L. Barnes

Recent advancements in transition metal dichalcogenides (TMDs) have unveiled exceptional optical and electronic characteristics, opened up new opportunities, and provided a unique platform for exploring light-matter interactions under the…

Transition metal dichalcogenides (TMDs) constitute a versatile platform for atomically thin optoelectronics devices and spin-valley memory applications. In monolayers optical absorption is strong, but the transition energy is not tunable as…

Over the past few decades, thin film optoelectronic devices based on transition metal dichalcogenides (TMDs) have made significant progress. However, the sensitivity of the exciton states to environmental change presents challenges for…

光学 · 物理学 2024-03-13 Shuangping Han , Pengyu Zan , Yu Yan , Yaoxing Bian , Chengbing Qin , Liantuan Xiao

We developed a comprehensive theoretical framework focusing on many-body effects of exciton species in monolayer WS$_2$, including bright and dark excitons, and intra- and inter-valley biexcitons, to investigate valley dynamics in monolayer…

介观与纳米尺度物理 · 物理学 2020-04-17 Fanyao Qu , Helena Bragança , Railson Vasconcelos , Fujun Liu , S-J Xie , Hao Zeng

Monolayers of semiconducting transition metal dichalcogenides are two-dimensional direct-gap systems which host tightly-bound excitons with an internal degree of freedom corresponding to the valley of the constituting carriers. Strong…

Monolayer transition-metal dichalcogenides, such as WSe$_2$, are direct gap, multi-valley semiconductors. Long-range electron-hole exchange interactions mix the valleys, yielding dispersion relations for massive ($\propto Q^2$) as well as…

介观与纳米尺度物理 · 物理学 2025-08-20 A. Delhomme , T. Amit , P. Ji , C. Faugeras , S. Refaely-Abramson , J. J. Finley , A. V. Stier

The interaction of intralayer and interlayer excitons is studied in a two-dimensional semiconductor, homobilayer MoS$_2$. It is shown that the measured optical susceptibility reveals both the magnitude and the sign of the coupling…

We report a new dark exciton in monolayer MoS$_2$ using second harmonic generation spectroscopy. Hereby, the spectrally dependent second harmonic generation intensity splits into two branches, and an anticrossing is observed at $\sim$ 25…

介观与纳米尺度物理 · 物理学 2024-08-22 Chenjiang Qian , Viviana Villafañe , Pedro Soubelet , Peirui Ji , Andreas V. Stier , Jonathan J. Finley

Screening due to surrounding dielectric medium reshapes the electron-hole interaction potential and plays a pivotal role in deciding the binding energies of strongly bound exciton complexes in quantum confined monolayers of transition metal…

介观与纳米尺度物理 · 物理学 2017-08-16 Garima Gupta , Sangeeth Kallatt , Kausik Majumdar

We use nonlinear pump-probe spectroscopy to study optical excitations in a charge-tunable MoSe$_2$\WS$_2$ moir\'e heterostructure. An intense red-detuned laser pulse creates a photonic dressing of the material by introducing a large virtual…

强关联电子 · 物理学 2025-06-02 B. Evrard , H. S. Adlong , A. A. Ghita , T. Uto , L. Ciorciaro , K. Watanabe , T. Taniguchi , M. Kroner , A. İmamoğlu

Mobile electrons in the semiconductor monolayer-MoS$_2$ form a ferromagnetic state at low temperature. The Fermi sea consists of two circles, one at the $K$-point, the other at the $\tilde{K}$-point, both with the same spin. Here, we…

Controlling resonant Raman scattering in two-dimensional semiconductors typically requires tuning the excitation energy to match excitonic transitions. Here we show that mechanical deformation can achieve the same effect without changing…

材料科学 · 物理学 2026-03-27 Álvaro Rodríguez , Carmen Munuera , Andres Castellanos-Gomez

We study experimentally and theoretically the exciton-phonon interaction in MoSe2 monolayers encapsulated in hexagonal BN, which has an important impact on both optical absorption and emission processes. The exciton transition linewidth…

A direct band gap, remarkable light-matter coupling as well as strong spin-orbit and Coulomb interaction establish two-dimensional (2D) crystals of transition metal dichalcogenides (TMDs) as an emerging material class for fundamental…

The interaction potential of a two-dimensional system of excitons with spatially separated electron-hole layers is considered in the strong magnetic field limit. The excitons are assumed to have free dynamics in the $x$-$y$ plane, while…

介观与纳米尺度物理 · 物理学 2009-10-31 M. A. Olivares-Robles , S. E. Ulloa

Exciton mobility in two-dimensional semiconductors is a key ingredient in materials-based design of optoelectronic functionalities. Monolayer transition metal dichalcogenides (TMDs) set a good test case, with tightly bound excitons and…

材料科学 · 物理学 2026-02-17 Amir Kleiner , Sivan Refaely-Abramson

Two-dimensional excitons formed in quantum materials such as monolayer transition-metal dichalcogenides and their strong light-matter interaction have attracted unrivalled attention by the research community due to their extraordinarily…

介观与纳米尺度物理 · 物理学 2018-12-31 Lorenz Maximilian Schneider , Shanece Esdaille , Daniel Rhodes , Katayun Barmak , James Hone , Arash Rahimi-Iman

Many-body exciton interactions shape the optoelectronic response of atomically-thin transition metal dichalcogenides, yet optical control of these interactions remains largely unexplored. To date, modulation of exciton-exciton interactions…