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Several theoretical predictions have claimed that the neutral exciton of TMDCs splits into a transversal and longitudinal exciton branch, with the longitudinal one, which is the upper branch, exhibiting an extraordinary strong dispersion in…

介观与纳米尺度物理 · 物理学 2020-05-29 Lorenz Maximilian Schneider , Shanece Esdaille , Daniel Rhodes , Katayun Barmak , James Hone , Arash Rahimi-Iman

Increasing the speed limits of conventional electronics requires innovative approaches to manipulate other quantum properties of electrons besides their charge. An alternative approach utilizes the valley degree of freedom in…

介观与纳米尺度物理 · 物理学 2023-03-29 A. O. Slobodeniuk , P. Koutenský , M. Bartoš , F. Trojánek , P. Malý , T. Novotný , M. Kozák

Lifting the valley degeneracy of monolayer transition metal dichalcogenides (TMD) would allow versatile control of the valley degree of freedom. We report a giant valley exciton splitting of 18 meV/T for monolayer WS2, using the proximity…

介观与纳米尺度物理 · 物理学 2019-10-09 Tenzin Norden , Chuan Zhao , Peiyao Zhang , Renat Sabirianov , Athos Petrou , Hao Zeng

Excitons in thin layers of semiconducting transition metal dichalcogenides are highly subject to the strongly modified Coulomb electron-hole interaction in these materials. Therefore, they do not follow the model system of a two-dimensional…

We study theoretically the Coulomb interaction between excitons in transition metal dichalcogenide (TMD) monolayers. We calculate direct and exchange interaction for both ground and excited states of excitons. The screening of the Coulomb…

介观与纳米尺度物理 · 物理学 2017-09-13 V. Shahnazaryan , I. Iorsh , I. A. Shelykh , O. Kyriienko

We develop a model of the coherent exciton spin-valley dynamics in two-dimensional transition metal dichalcogenides under elastic strain. The strain splits the exciton radiative doublet in linearly polarized states. Consequently, it induces…

介观与纳米尺度物理 · 物理学 2023-01-04 M. M. Glazov

The optical properties of monolayer and bilayer transition metal dichalcogenide semiconductors are governed by excitons in different spin and valley configurations, providing versatile aspects for van der Waals heterostructures and devices.…

介观与纳米尺度物理 · 物理学 2020-10-28 J. Förste , N. V. Tepliakov , S. Yu. Kruchinin , J. Lindlau , V. Funk , M. Förg , K. Watanabe , T. Taniguchi , A. S. Baimuratov , A. Högele

Monolayers (MLs) of MoS2 and WSe2 are 2D semiconductors with strong, direct optical transitions that are governed by tightly Coulomb bound eletron-hole pairs (excitons). The optoelectronic properties of these transition metal…

材料科学 · 物理学 2015-03-06 G. Wang , X. Marie , I. Gerber , T. Amand , D. Lagarde , L. Bouet , M. Vidal , A. Balocchi , B. Urbaszek

By implementing four-wave mixing (FWM) micro-spectroscopy we measure coherence and population dynamics of the exciton transitions in monolayers of MoSe$_2$. We reveal their dephasing times T$_2$ and radiative lifetime T$_1$ in a…

Reflectance and magneto-reflectance experiments together with theoretical modelling based on the $\mathbf{k\cdot p}$ approach have been employed to study the evolution of direct bandgap excitons in MoS$_2$ layers with a thickness ranging…

介观与纳米尺度物理 · 物理学 2019-03-01 A. O. Slobodeniuk , Ł. Bala , M. Koperski , M. R. Molas , P. Kossacki , K. Nogajewski , M. Bartos , K. Watanabe , T. Taniguchi , C. Faugeras , M. Potemski

Interlayer excitons are observed coexisting with intralayer excitons in bi-layer, few-layer, and bulk MoSe2 single crystals by confocal reflection contrast spectroscopy. Quantitative analysis using the Dirac-Bloch-Equations provides…

材料科学 · 物理学 2018-06-13 Jason Horng , Tineke Stroucken , Long Zhang , Eunice Y. Paik , Hui Deng , Stephan W. Koch

Strong interactions between surface plasmons in ultra-compact nanocavities and excitons in two dimensional materials have attracted wide interests for its prospective realization of polariton devices at room temperature. Here, we propose a…

The suppression of Zeeman energy splitting due to spin-dependent interactions within a Bose-Einstein condensate (the spin Meissner effect) was predicted to occur up to a certain value of magnetic field strength. We report a clear…

Motional narrowing implies narrowing induced by motion, for example, in nuclear resonance, the thermally induced random motion of the nuclei in an inhomogeneous environment leads to counter-intuitive narrowing of the resonance line.…

介观与纳米尺度物理 · 物理学 2024-05-10 Garima Gupta , Kenji Watanabe , Takashi Taniguchi , Kausik Majumdar

Realizing nonlinear optical response in the low photon density limit in solid-state systems has been a long-standing challenge. Semiconductor microcavities in the strong coupling regime hosting exciton-polaritons have emerged as attractive…

We propose a pair spin-orbit interaction (PSOI) mechanism by establishing a mesoscopic many-particle Rashba Hamiltonian. In lowest order, this Hamiltonian self-consistently describes exciton spin relaxation in monolayer transition metal…

介观与纳米尺度物理 · 物理学 2026-02-18 Henry Mittenzwey , Andreas Knorr

We investigate the optical excitation spectra and the photoluminescence depolarization dynamics in bilayer WS$_2$. A different understanding of the optical excitation spectra in the recent photoluminescence experimentby Zhu {\em et al.}…

介观与纳米尺度物理 · 物理学 2014-07-25 T. Yu , M. W. Wu

We study the effect of Coulomb interactions on the low energy band structure of single-layer transition metal dichalcogenide semiconductors using an effective low energy model. We show how a large conduction band spin splitting and a spin…

介观与纳米尺度物理 · 物理学 2014-12-25 Yago Ferreiros , Alberto Cortijo

We develop a model, which incorporates both intra- and intervalley scatterings to master equation, to explore exciton valley coherence in monolayer WS$_2$ subjected to magnetic field. For linearly polarized (LP) excitation accompanied with…

介观与纳米尺度物理 · 物理学 2023-08-09 Kang Lan , Shijie Xie , Jiyong Fu , Fanyao Qu

Atomically thin crystals of transition metal dichalcogenides are ideally suited to study the interplay of light-matter coupling, polarization and magnetic field effects. In this work, we investiagte the formation of exciton-polaritons in a…