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相关论文: Role of Defects in Photocatalytic Water Splitting:…

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TiO2 is a wide band-gap semiconductor that has been intensively investigated for photocatalysis and water-spiting. However, weak light absorption in the visible region of the spectrum poses stringent limitation to its practical application.…

材料科学 · 物理学 2023-02-07 Fernando P. Sabino , Anderson Janotti

Defects trap photocarriers and hinder solar water splitting. The nanoscale photocarrier transport, trapping, and recombination mechanisms are usually inferred from ensemble-averaged measurements and remain elusive. Because an individual…

First principles calculations through density functional theory (DFT)+$U$ method were performed to assess the effect of Li interstitial doping on the optoelectronic properties of NiO and of cubic, hexagonal, and monoclinic WO$_3$. The…

Photocatalytic water splitting has emerged as a sustainable pathway for hydrogen production, leveraging sunlight to drive chemical reactions. This review explores the integration of density functional theory (DFT) with machine learning (ML)…

计算物理 · 物理学 2025-12-30 Dennis Delali Kwesi Wayo , Leonardo Goliatt , Darvish Ganji

In this work, the electronic and optical properties of a Nitrogen (N) or a Boron (B) doped BeO monolayer are investigated in the framework of density functional theory. It is known that the band gap of a BeO monolayer is large leading to…

Photoreduction of CO$_2$ is an important alternative approach aimed to reduce the CO$_2$ atmospheric content which is responsible of the global warming. The development of an efficient photocatalyst can strongly improve the efficiency and…

材料科学 · 物理学 2025-04-29 Onofrio Tau , Giacomo Giorgi , Riccardo Rurali

The hole-doped NdNiO$_2$ layer deposited on the SrTiO$_{3}$ surface exhibits unconventional superconductivity. Here, we present a systematic study of the electronic and magnetic properties of the NdNiO$_2$ superconductor using the density…

材料科学 · 物理学 2025-12-24 Sajid Sekh , Andrzej Ptok , Wojciech Brzezicki , Przemysław Piekarz , Andrzej M. Oleś

This study presents a comprehensive numerical analysis of a quantum-dot-engineered heterostructure, PbS:$Yb^{3+},Er^{3+}$/CuBiO, optimized for water splitting applications. Using density functional theory (DFT) coupled with machine…

Photocatalytic water splitting is a promising renewable energy source as an alternative for limited fossil fuels. The effectiveness of the conversion from solar energy to hydrogen fuel relies primarily on the material. Previously,…

材料科学 · 物理学 2022-01-04 Celine Wu , Xuan Luo

Graphene like 2D materials have attracted tremendous attention in the field of photocatalytic water splitting. Indium Selenide (InSe) is one such potential material. Here, we report the effect of Tellurium on InSe monolayer for the…

材料科学 · 物理学 2016-10-04 M. R. Ashwin Kishore , P. Ravindran

Theoretical work has suggested that monolayer MoS2 doped with Mn should behave as a two-dimensional dilute magnetic semiconductor, which would open up possibilities for spintronic applications, device physics, and novel ground states. The…

A major goal of energy research is to use visible light to cleave water directly, without an applied voltage, into hydrogen and oxygen. Since the initial reports of the ultraviolet (UV) activity of TiO2 and SrTiO3 in the 1970s, researchers…

Due to the energy supply pressure caused by non-renewable fuels as well as the environment-related issues, the efficient conversion of solar-chemical energy via photo-induced water splitting is one of the promising strategies to address the…

化学物理 · 物理学 2021-03-23 Zhexu Xi

Samples of nitrogen-doped titanium dioxide (anatase, $0.2 \leq N \leq 1.0~wt\%$) prepared by the sol-gel method were investigated using X-band EPR spectroscopy, photoconductivity and photocatalysis measurements. $N\bullet$ and $NO\bullet$…

材料科学 · 物理学 2017-04-18 A. A. Minnekhanov , N. T. Le , E. A. Konstantinova , P. K. Kashkarov

Recent rapid progress in efficiencies for solar water splitting by photoelectrochemical devices has enhanced its prospects to enable storable renewable energy. Efficient solar fuel generators all use tandem photoelectrode structures, and…

A swift chemical route to synthesize Co-doped SnO$_2$ nanopowders is described. Pure and highly stable Sn$_{1-x}$Co$_x$O$_{2-\delta}$ (0 $\le$ x $\le$ 0.15) crystalline nanoparticles were synthesized, with mean grain sizes < 5 nm and the…

材料科学 · 物理学 2015-03-31 T. Entradas , J. Cabrita , S. Dalui , M. R. Nunes , O. C. Monteiro , A. J. Silvestre

The integration of sonocatalysis with photocatalysis offers a powerful strategy for advanced wastewater treatment by overcoming rapid charge carrier recombination in conventional photocatalytic systems. Although these processes are often…

Efficient artificial photosynthesis systems are currently realized as catalyst- and surfacefunctionalized photovoltaic tandem- and triple-junction devices, enabling photoelectrochemical (PEC) water oxidation while simultaneously recycling…

We investigate the room temperature electronic properties of MnTiO3 synthesised by different preparation conditions. For this purpose, we prepared MnTiO3 under two different cooling rates, one is naturally cooled while the other is quenched…

强关联电子 · 物理学 2017-10-25 R. K. Maurya , Priyamedha Sharma , Ashutosh Patel , R. Bindu

In recent years, photosensitive materials have been in huge demand because of their fascinating ability to convert absorbed photon energy to generate strain and henceforth tuning the physical properties. In this report we detect the…