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We review our recent development of a first-principles lattice dynamics method that can treat anharmonic effects nonperturbatively. The method is based on the self-consistent phonon theory and temperature-dependent phonon frequencies can be…

材料科学 · 物理学 2018-01-29 Terumasa Tadano , Shinji Tsuneyuki

We present an analytic scheme to connect the fragility and viscoelasticity of metallic glasses to the effective ion-ion interaction in the metal. This is achieved by an approximation of the short-range repulsive part of the interaction,…

软凝聚态物质 · 物理学 2015-10-29 Johannes Krausser , Konrad Samwer , Alessio Zaccone

In two and three dimensions, this study is focused on the numerical analysis of an eigenproblem associated with a fluid-structure model for sloshing and elasto-acoustic vibration. We use a displacement-Herrmann pressure formulation for the…

数值分析 · 数学 2025-11-05 Arbaz Khan , Felipe Lepe , David Mora , Ricardo Ruíz-Baier , Jesus Vellojin

We introduce a lattice dynamics package which calculates elastic, thermodynamic and thermal transport properties of crystalline materials from data on their force and potential energy as a function of atomic positions. The data can come…

We use electronic structure calculations based upon density functional theory to search for ideal plasmonic materials among the alkali noble intermetallics. Importantly, we use density functional perturbation theory to calculate the…

光学 · 物理学 2021-08-24 Martin G. Blaber , Matthew D. Arnold , Michael J. Ford

The thermoelectric properties of the three pyrite-type IIB-VIA2 dichalcogenides (ZnS2, CdS2 and CdSe2) are systematically investigated and compared with those of the prototype ZnSe2 in order to optimize their thermoelectric properties.…

应用物理 · 物理学 2022-03-08 Tiantian Jia , Jesús Carrete , Georg K. H. Madsen , Yongsheng Zhang , Suhuai Wei

The structural, electronic, optical and vibrational properties of LiN$_3$ under high pressure have been studied using plane wave pseudopotentials within the generalized gradient approximation for the exchange and correlation functional. The…

材料科学 · 物理学 2013-11-07 K. Ramesh Babu , Ch. Bheema Lingam , Surya P. Tewari , G. Vaitheeswaran

The structures and electronic states in all polymorphs of poly(vinylidene fluoride) (PVDF) were calculated in various levels using the CRYSTAL software. The calculated lattice constants with PBE0/cc-pVTZ agreed well with experimental…

材料科学 · 物理学 2014-05-27 Akira Itoh

Quantum Monte Carlo (QMC) forces have been studied extensively in recent decades because of their importance with spectroscopic observables and geometry optimization. Here we benchmark the accuracy and statistical cost of QMC forces. The…

计算物理 · 物理学 2021-06-16 Juha Tiihonen , Raymond C. Clay , Jaron T. Krogel

A set of 55 clarinet reeds is observed by holography, collecting 2 series of measurements made under 2 different moisture contents, from which the resonance frequencies of the 15 first modes are deduced. A statistical analysis of the…

Precipitation of fine particles into the base material of a metal is a potent strengthening mechanism. This is numerically analyzed within a continuum framework based on a higher order strain gradient plasticity theory and by use of an…

材料科学 · 物理学 2021-06-17 Mohammadali Asgharzadeh , Jonas Faleskog

The quasiharmonic approximation is the most common method for modeling the specific heat of solids; however, it fails to capture the effects of intrinsic anharmonicity. In this study, we introduce the "elastic softening approximation," an…

We present a simple, first principles scheme for calculating mechanical properties of nonequilibrium bulk systems assuming an ideal ballistic distribution function for the electronic states described by the external voltage bias. This…

介观与纳米尺度物理 · 物理学 2022-11-15 Nick Papior , Susanne Leitherer , Mads Brandbyge

Due to their outstanding mechanical properties, diamond and diamond-like materials find significant technological applications ranging from well-established industrial fields (cutting tools, coatings, etc.) to more advanced mechanical…

We determine the frequency dependence of four independent CdWO$_4$ Cartesian dielectric function tensor elements by generalized spectroscopic ellipsometry within mid-infrared and far-infrared spectral regions. Single crystal surfaces cut…

材料科学 · 物理学 2017-04-26 A. Mock , R. Korlacki , S. Knight , M. Schubert

Machine Learning (ML) techniques are revolutionizing the way to perform efficient materials modeling. Nevertheless, not all the ML approaches allow for the understanding of microscopic mechanisms at play in different phenomena. To address…

We demonstrate that the melting points and other thermodynamic quantities of the alkali metals can be calculated based on static crystalline properties. To do this we derive analytic interatomic potentials for the alkali metals fitted…

材料科学 · 物理学 2016-06-02 Alan Nichol , Graeme J. Ackland

Limiting chain extensibility is a characteristic that plays a vital role in the stretching of highly elastic materials. The Gent model has been widely used to capture this behaviour, as it performs very well in fitting stress-stretch data…

混沌动力学 · 物理学 2024-07-12 Amin Alibakhshi , Weiqiu Chen , Michel Destrade

We assess the predictive power of alchemical perturbations for estimating fundamental properties in ionic crystals. Using density functional theory we have calculated formation energies, lattice constants, and bulk moduli for all sixteen…

化学物理 · 物理学 2016-05-27 Alisa Solovyeva , O. Anatole von Lilienfeld

Out of self-consistent semi-classical calculations performed within the so-called Extended Thomas-Fermi approach for 212 nuclei at all even angular momentum values I ranging between 0 and 80 \hbar and using the Skyrme SkM* effective force,…

核理论 · 物理学 2009-10-31 J. Piperova , D. Samsoen , P. Quentin , K. Bencheikh , J. Bartel , J. Meyer