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We propose a physical principle for implementation of controllable interactions of identical electromagnetic bosons (excitons or polaritons) in two-dimensional (2D) semiconductors. The key ingredients are tightly bound biexcitons and…

量子气体 · 物理学 2024-05-22 Sergueï V. Andreev

Exciton-phonon interactions govern the energy level spectrum and thus the optical response in semiconductors. In this respect, lead-halide perovskite nanocrystals represent a unique system, for which the interaction with optical phonons is…

We investigate the photon statistics of the light emitted by single self-assembled hybrid gold-CdSe/CdS/CdZnS colloidal nanocrystal supraparticles through the detailed analysis of the intensity autocorrelation function $g^{(2)}(\tau)$. We…

介观与纳米尺度物理 · 物理学 2023-02-16 V. Blondot , D. Gérard , G. Quibeuf , C. Arnold , A. Delteil , A. Bogicevic , T. Pons , N. Lequeux , S. Buil , J-P. Hermier

Two dimensional (2D) semiconductors present unique opportunities to intertwine optical and magnetic functionalities and to tune these performances through defects and dopants. Here, we integrate exciton pumping into a quantum sensing…

We investigate the dynamics of single- and multi-photon emission from detuned strongly coupled systems based on the quantum-dot-photonic-crystal resonator platform. Transmitting light through such systems can generate a range of…

Moir\'e potential acts as periodic quantum confinement for optically generated exciton, generating spatially ordered zero-dimensional quantum system. However, broad emission spectrum arising from inhomogeneity among moir\'e potential…

The dependence of the excitonic two-photon absorption on the quantum correlations (entanglement) of exciting biphotons by a semiconductor quantum well is studied. We show that entangled photon absorption can display very unusual features…

介观与纳米尺度物理 · 物理学 2015-05-30 L. J. Salazar , D. A. Guzmán , F. J. Rodríguez , L. Quiroga

Although both epitaxial quantum dots (QDs) and colloidal nanocrystals (NCs) are quantum-confined semiconductor nanostructures, so far they have demonstrated dramatically-different exciton fine structure splittings (FSSs) at the cryogenic…

介观与纳米尺度物理 · 物理学 2017-07-19 Chunyang Yin , Liyang Chen , Yan Lv , Fengrui Hu , Chun Sun , William W. Yu , Chunfeng Zhang , Xiaoyong Wang , Yu Zhang , Min Xiao

Due to the spatial confinement, two-dimensional metal chalcogenides display an extraordinary optical re-sponse and carrier transport ability. Solution-based synthesis techniques such as colloidal hot injection and ion exchange provide a…

材料科学 · 物理学 2021-10-25 Ziyi Hu , Ryan O'Neill , Rostyslav Lesyuk , Christian Klinke

In monolayer transition metal dichalcogenides, quantum emitters are associated with localized strain that can be deterministically applied to create designer nano-arrays of single photon sources. Despite an overwhelming empirical…

Excitons, Coulomb bound electron-hole pairs, dominate the optical response of two-dimensional semiconductors across near-infrared and visible frequencies due to their large binding energy and prominent oscillator strength. Previous…

介观与纳米尺度物理 · 物理学 2026-01-07 Anna Roche , Michael R. Koehler , David G. Mandrus , Takashi Taniguchi , Kenji Watanabe , John R. Schaibley , Brian J. LeRoy

Excitons are vital in the photophysics of materials, especially in low-dimensional systems. The conceptual and quantitative understanding of excitonic effects in nonlinear optical (NLO) processes is more challenging compared to linear ones.…

材料科学 · 物理学 2026-02-26 Jiawei Ruan , Y. -H. Chan , Steven G. Louie

We provide a self-contained review of master equation approaches to modelling phonon effects in optically driven self-assembled quantum dots. Coupling of the (quasi) two-level excitonic system to phonons leads to dissipation and dephasing,…

介观与纳米尺度物理 · 物理学 2016-06-14 Ahsan Nazir , Dara P. S. McCutcheon

We theoretically study the quantum-coherence-enhanced subradiance in a chiral-coupled atomic chain with nonreciprocal decay channels. The collective radiation in this one-dimensional (1D) nanophotonics system results from the resonant…

量子物理 · 物理学 2020-09-14 H. H. Jen

First-order perturbation theory and many-body Green function analysis are used to quantify the influence of size, surface reconstruction and surface treatment on exciton transport between small silicon quantum dots. Competing radiative…

介观与纳米尺度物理 · 物理学 2011-11-01 Zhibin Lin , Huashan Li , Alberto Franceschetti , Mark T. Lusk

Excitons, Coulomb-bound electron-hole pairs, are the fundamental excitations governing the optoelectronic properties of semiconductors. While optical signatures of excitons have been studied extensively, experimental access to the excitonic…

For high-speed optoelectronic applications relying on fast relaxation or energy transfer mechanisms, understanding of carrier relaxation and recombination dynamics is critical. Here, we compare the differences in photoexcited carrier…

介观与纳米尺度物理 · 物理学 2020-10-28 Verena A. Hintermayr , Lakshminarayana Polavarapu , Alexander S. Urban , Jochen Feldmann

We have theoretically investigated a generation of entangled photons from biexcitons in a semiconductor film with thickness in nano-to-bulk crossover regime. In contrast to the cases of quantum dots and bulk materials, we can highly control…

其他凝聚态物理 · 物理学 2010-09-20 Motoaki Bamba , Hajime Ishihara

Distinguished by their long lifetimes, strong dipolar interactions, and periodic confinement, moir\'e excitons provide a fertile territory for realizing interaction-driven excitonic phases beyond conventional semiconductor systems. Formed…

We study the optical emission from single semiconductor quantum dots coupled to the optical modes of photonic crystal nanocavities. For dots that are both spectrally and spatially coupled, auto-correlation measurements reveal efficient…

介观与纳米尺度物理 · 物理学 2009-11-13 M. Kaniber , A. Laucht , A. Neumann , J. M. Villas-Boas , M. Bichler , M. -C. Amann , J. J. Finley