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We show how to simulate a model of many molecules with both strong coupling to many vibrational modes and collective coupling to a single photon mode. We do this by combining process tensor matrix product operator methods with a mean-field…

量子气体 · 物理学 2022-10-24 Piper Fowler-Wright , Brendon W. Lovett , Jonathan Keeling

Intramolecular energy transfer driven by near-field effects plays an important role in applications ranging from biophysics and chemistry to nano-optics and quantum communications. Advances in strong light-matter coupling in molecular…

介观与纳米尺度物理 · 物理学 2025-07-14 Kristin B. Arnardottir , Piper Fowler-Wright , Christos Tserkezis , Brendon W. Lovett , Jonathan Keeling

Phonon interactions are inevitable in cavity quantum electrodynamical systems based on solid-state emitters or fluorescent molecules, where vibrations of the lattice or chemical bonds couple to the electronic degrees of freedom. Due to the…

量子物理 · 物理学 2021-06-16 Matias Bundgaard-Nielsen , Jesper Mørk , Emil Vosmar Denning

We analytically tackle opto-vibronic interactions in molecular systems driven by either classical or quantum light fields. In particular, we examine a simple model of molecules with two relevant electronic levels, characterized by potential…

量子物理 · 物理学 2024-02-28 Q. Zhang , M. Asjad , M. Reitz , C. Sommer , B. Gurlek , C. Genes

Cascaded emission from the biexciton state of a quantum dot results in polarization entangled photon pairs. However, modelling this system becomes challenging when photon emission is cavity-mediated due to the large Hilbert space and…

量子物理 · 物理学 2026-03-24 Katy Snow , Mauro Paternostro

The observation that materials can change their properties when placed inside or near an optical resonator, has sparked a fervid interest in understanding the effects of strong light-matter coupling on molecular dynamics, and several…

化学物理 · 物理学 2024-03-20 Ilia Sokolovskii , Gerrit Groenhof

We present the experimental control of Non-Markovian dynamics of open quantum systems simulated with photonic entities. The polarization of light is used as the system, whereas the surrounding environment is represented by light's spatial…

The way a principle system and its environment interact characterizes the non-Markovianity of the dynamics. Herein, we investigate the non-Markovian dynamics of photon polarization in a birefringent crystal. We consider the so-called…

量子物理 · 物理学 2018-10-31 Kai-Hung Wang , Shih-Hsuan Chen , Yu-Cheng Lin , Che-Ming Li

Nanoscale devices - either biological or artificial - operate in a regime where the usual assumptions of a structureless, Markovian, bath do not hold. Being able to predict and study the dynamics of such systems is crucial and is usually…

量子物理 · 物理学 2021-11-17 Thibaut Lacroix , Angus Dunnett , Dominic Gribben , Brendon W. Lovett , Alex Chin

In the last decade, much theoretical research has focused on studying the strong coupling between organic molecules (or quantum emitters, in general) and light modes. The description and prediction of polaritonic phenomena emerging in this…

We report on time-resolved photoluminescence from semiconductor microcavities showing that an optically controllable mechanism exists to turn on and off memory effects in a polariton system. By increasing the laser pumping pulse intensity…

介观与纳米尺度物理 · 物理学 2009-11-13 F. J. Rodriguez , L. Quiroga , C. Tejedor , M. D. Martin , L. Vina , R. Andre

In the regime of strong coupling between molecular excitons and confined optical modes, the intra-molecular degrees of freedom are profoundly affected, leading to a reduced vibrational dressing of polaritons compared to bare electronically…

介观与纳米尺度物理 · 物理学 2018-10-17 Javier del Pino , Florian A. Y. N. Schröder , Alex W. Chin , Johannes Feist , Francisco J. Garcia-Vidal

We employ the exact factorization of a multi-component wavefunction to analyze the dynamics of interacting photons, electrons and nuclei. We consider physical situations emerging in the regime of strong coupling between light excitations…

化学物理 · 物理学 2026-04-24 Claudia Magi , Peter Schuerger , David Lauvergnat , Federica Agostini

The system-environment interaction is simulated by light propagating in coupled photonic waveguides. The profile of the electromagnetic field provides intuitive physical insight to study the Markovian and non-Markovian dynamics of open…

量子物理 · 物理学 2013-12-16 Chang-Ling Zou , Xiang-Dong Chen , Xiao Xiong , Fang-Wen Sun , Xu-Bo Zou , Zheng-Fu Han , Guang-Can Guo

Molecules constitute compact hybrid quantum optical systems that can interface photons, electronic degrees of freedom, localized mechanical vibrations and phonons. In particular, the strong vibronic interaction between electrons and nuclear…

Following our recent numerical study [arXiv:2601.16299 (2026)], we investigate vibrational excitation induced by transient optical driving in molecular ensembles strongly coupled to a cavity mode using the field-driven…

We study theoretically the quantum dynamics and spectroscopy of rovibrational polaritons formed in a model system composed of a single rovibrating diatomic molecule, which interacts with two degenerate, orthogonally polarized modes of an…

化学物理 · 物理学 2023-01-11 Eric W. Fischer , Peter Saalfrank

The simulation of quantum processes is a key goal for the grand programme aiming at grounding quantum technologies as the way to explore complex phenomena that are inaccessible through standard, classical calculators. Some interesting steps…

量子物理 · 物理学 2013-06-12 Andrea Chiuri , Chiara Greganti , Laura Mazzola , Mauro Paternostro , Paolo Mataloni

We present a microscopic theory for nonlinear optical spectroscopy of N molecules in an optical cavity. A quantum Langevin analytical expression is derived for the time- and frequency-resolved signals accounting for arbitrary numbers of…

量子物理 · 物理学 2023-03-29 Zhedong Zhang , Xiaoyu Nie , Dangyuan Lei , Shaul Mukame

When the interaction between a molecular system and confined light modes in an optical or plasmonic cavity is strong enough to overcome the dissipative process, hybrid light-matter states (polaritons) emerge as the fundamental excitations…

化学物理 · 物理学 2024-10-23 Xinyang Li , Sergei Tretiak , Yu Zhang
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