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相关论文: Optical Absorption by Indirect Excitons in a Trans…

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The effect of a magnetic field on the optical absorption in semiconductors has been measured experimentally and modeled theoretically for various systems in previous decades. We present a new first-principles approach to systematically…

介观与纳米尺度物理 · 物理学 2020-06-03 Thorsten Deilmann , Peter Krüger , Michael Rohlfing

Semiconducting MXenes are an intriguing two-dimensional (2D) material class with promising electronic and optoelectronic properties. Here, we focused on recently prepared Hf-based MXenes, namely Hf$_3$C$_2$O$_2$ and Hf$_2$CO$_2$. Using the…

材料科学 · 物理学 2024-04-03 Nilesh Kumar , Miroslav Kolos , Sitangshu Bhattacharya , František Karlický

The optical response of semiconducting monolayer transition-metal dichalcogenides (TMDCs) is dominated by strongly bound excitons that are stable even at room temperature. However, substrate-related effects such as screening and disorder in…

When transition-metal dichalcogenide monolayers lack inversion symmetry, their low-energy single particle spectrum can described by tilted massive Dirac Hamiltonians. The so-called Janus materials fall into that category. Inversion symmetry…

介观与纳米尺度物理 · 物理学 2022-09-15 M. F. C. Martins Quintela , A. T. Costa , N. M. R. Peres

The excitonic states of transition metal dichacolgenide (TMD) monolayers are heavily influenced by their external dielectric environment based on the substrate used. In this work, various wide bandgap dielectric materials, namely hexagonal…

Excitonic effects play a particularly important role in the optoelectronic behavior of two-dimensional semiconductors. To facilitate the interpretation of experimental photoabsorption and photoluminescence spectra we provide (i)…

介观与纳米尺度物理 · 物理学 2017-08-23 E. Mostaani , M. Szyniszewski , C. H. Price , R. Maezono , M. Danovich , R. J. Hunt , N. D. Drummond , V. I. Fal'ko

Transition metal dichalcogenides (TMDs) are emerging as promising two-dimensional (2d) semiconductors for optoelectronic and flexible devices. However, a microscopic explanation of their photophysics -- of pivotal importance for the…

We investigate excitons in stacked transition metal dichalcogenide (TMDC) layers under perpendicularly applied electric field, herein MoSe$_2$/WSe$_2$ van der Waals heterostructures. Band structures are obtained with density functional…

介观与纳米尺度物理 · 物理学 2018-09-19 A. Chaves , J. G. Azadani , V. Ongun Özçelik , R. Grassi , T. Low

We study theoretically the Coulomb interaction between excitons in transition metal dichalcogenide (TMD) monolayers. We calculate direct and exchange interaction for both ground and excited states of excitons. The screening of the Coulomb…

介观与纳米尺度物理 · 物理学 2017-09-13 V. Shahnazaryan , I. Iorsh , I. A. Shelykh , O. Kyriienko

A quantitative analysis of the excitonic luminescence efficiency in hexagonal boron nitride (hBN) is carried out by cathodoluminescence in the ultraviolet range and compared with zinc oxide and diamond single crystals. A high quantum yield…

Monolayer transition metal dichalcogenides feature Coulomb-bound electron-hole pairs (excitons) with exceptionally large binding energy and coupled spin and valley degrees of freedom. These unique attributes have been leveraged for…

Exciton spectra of monolayer transition metal dichalcogenides (TMDs) in various dielectric environments are studied. The screened hydrogen model (SHM) [Phys. Rev. Lett. 116, 056401 (2016)] is examined by comparing its exciton spectra with…

介观与纳米尺度物理 · 物理学 2019-02-20 Jian-zhong Zhang , Jin-zhong Ma

Excitonic semiconductors such as transition metal dichalcogenides (TMDCs) are attractive for next-generation photovoltaics (PVs) with low cost, light weight, and low material consumption. In WS2 and other TMDCs, the simultaneous large…

光学 · 物理学 2024-10-22 Adam D. Alfieri , Tobia Ruth , Cheryl Lim , Jason Lynch , Deep Jariwala

The energy landscape of optical excitations in mono- and few-layer transition metal dichalcogenides (TMDs) is dominated by optically bright and dark excitons. These excitons can be fully localized within a single TMD layer, or the electron-…

Recent results on the optical properties of mono- and few-layers of semiconducting transition metal dichalcogenides are reviewed. Experimental observations are presented and discussed in the frame of existing models, highlighting the limits…

介观与纳米尺度物理 · 物理学 2017-09-19 M. Koperski , M. R. Molas , A. Arora , K. Nogajewski , A. O. Slobodeniuk , C. Faugeras , M. Potemski

We present a microscopic theory of neutral excitons and charged excitons (trions) in monolayers of transition metal dichalcogenides, including molybdenum disulfide. Our theory is based on an effective mass model of excitons and trions,…

材料科学 · 物理学 2015-08-12 Timothy C. Berkelbach , Mark S. Hybertsen , David R. Reichman

We studied the exciton properties in double layers of transition metal dichalcogenides (TMDs) with a dielectric spacer between the layers. We developed a method based on an expansion of Chebyshev polynomials to solve the Wannier equation…

介观与纳米尺度物理 · 物理学 2023-08-09 Luiz G. M. Tenório , Teldo A. S. Pereira , K. Mohseni , T. Frederico , M. R. Hadizadeh , Diego R. da Costa , André J. Chaves

Twisted bilayer two-dimensional transition-metal dichalgocenides (TMDCs) exhibit a range of novel phenomena such as the formation of moir\'e excitons and strongly correlated phases. The coupling between the layers is crucial for the…

材料科学 · 物理学 2024-09-27 Eileen Schneider , Kenji Watanabe , Takashi Taniguchi , Janina Maultzsch

Excitons in optoelectronic devices have been generated through optical excitation, external carrier injection, or employing pre-existing charges. Here, we reveal a new way to electrically generate excitons in transition metal…

介观与纳米尺度物理 · 物理学 2022-10-03 Sotirios Papadopoulos , Lujun Wang , Takashi Taniguchi , Kenji Watanabe , Lukas Novotny

Exciton spectroscopy serves as a sensitive probe of electronic states in two-dimensional semiconductors. A prominent feature in optical spectra is the trion peak arising from the binding of a charge carrier to an exciton. The splitting…

介观与纳米尺度物理 · 物理学 2025-07-23 Arthur Christianen , Atac Imamoglu