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We develop a theoretical description of the critical zipping dynamics of a self-folding polymer. We use tension propagation theory and the formalism of the generalized Langevin equation applied to a polymer that contains two complementary…

软凝聚态物质 · 物理学 2017-05-12 Takahiro Sakaue , Jean-Charles Walter , Enrico Carlon , Carlo Vanderzande

We develop off-lattice simulations of semiflexible polymer chains subjected to applied mechanical forces using Markov Chain Monte Carlo. Our approach models the polymer as a chain of fixed-length bonds, with configurations updated through…

软凝聚态物质 · 物理学 2024-11-26 Lijie Ding , Chi-Huan Tung , Bobby G. Sumpter , Wei-Ren Chen , Changwoo Do

We use Newtonian and overdamped Langevin dynamics to study long flexible polymers dragged by an external force at a constant velocity $v$. The work $W$ by that force depends on the initial state of the polymer and the details of the…

统计力学 · 物理学 2017-08-30 Raz Halifa Levi , Yacov Kantor

We study the translocation of polymers across varying-section channels. Using systematic approximations, we derive a simplified model that reduces the problem of polymer translocation through varying-section channels to that of a point-like…

软凝聚态物质 · 物理学 2017-07-13 Valentino Bianco , Paolo Malgaretti

How much time does it take for a fluctuating system, such as a polymer chain, to reach a target configuration that is rarely visited -- typically because of a high energy cost ? This question generally amounts to the determination of the…

统计力学 · 物理学 2020-03-18 Nicolas Levernier , Olivier Bénichou , Raphaël Voituriez , Thomas Guérin

The emergent fluctuating hydrodynamics of a viscoelastic fluid modeled by the multiparticle collision dynamics (MPC) approach is studied. The fluid is composed of flexible, Gaussian phantom polymers, which interact by local…

软凝聚态物质 · 物理学 2020-01-29 David Toneian , Gerhard Kahl , Gerhard Gompper , Roland G. Winkler

We revisit the celebrated Wilemski-Fixman (WF) treatment for the looping time of a free-draining polymer. The WF theory introduces a sink term into the Fokker-Planck equation for the $3(N+1)$-dimensional Ornstein-Uhlenbeck process of the…

软凝聚态物质 · 物理学 2019-10-29 Felix X. -F. Ye , Panos Stinis , Hong Qian

We investigate the effect of hydrodynamic interactions on the non-equilibrium drift dynamics of an ideal flexible polymer pulled by a constant force applied at one end of the polymer using the perturbation theory and the renormalization…

统计力学 · 物理学 2009-11-13 Semjon Stepanow , Norio Kikuchi

A polymer model given in terms of beads, interacting through Hookean springs and hydrodynamic forces, is studied. Brownian dynamics description of this bead-spring polymer model is extended to multiple resolutions. Using this multiscale…

化学物理 · 物理学 2018-06-13 Edward Rolls , Radek Erban

We report results of molecular-dynamics simulations of a model polymer melt consisting of short non-entangled chains in the supercooled state above the critical temperature of mode-coupling theory (MCT). To analyse the dynamics of the…

软凝聚态物质 · 物理学 2007-05-23 M. Aichele , J. Baschnagel

Inspired by recent experiments on chromosomal dynamics, we introduce an exactly solvable model for the interaction between a flexible polymer and a set of motor-like enzymes. The enzymes can bind and unbind to specific sites of the polymer…

软凝聚态物质 · 物理学 2019-04-03 Stefanie Put , Takahiro Sakaue , Carlo Vanderzande

We solve the Chapman-Kolmogorov equation and study the exact splitting probabilities of the general stochastic process which describes polymer translocation through membrane pores within the broad class of Markov chains. Transition…

统计力学 · 物理学 2015-05-19 Felipe Mondaini , L. Moriconi

Some recent results on the rotational dynamics of polymers are reviewed and extended. We focus here on the relaxation of a polymer, either flexible or semiflexible, initially wrapped around a rigid rod. We also study the steady polymer…

统计力学 · 物理学 2015-06-22 Jean-Charles Walter , Michiel Laleman , Marco Baiesi , Enrico Carlon

The longitudinal response of single semiflexible polymers to sudden changes in externally applied forces is known to be controlled by the propagation and relaxation of backbone tension. Under many experimental circumstances, realized, e.g.,…

软凝聚态物质 · 物理学 2011-02-25 Florian Thüroff , Benedikt Obermayer , Erwin Frey

The conformational and dynamical properties of active polymers in solution are determined by the nature of the activity, and the behavior of polymers with self-propelled, active Brownian particle-type monomers differs qualitatively from…

软凝聚态物质 · 物理学 2020-05-27 Aitor Martin-Gomez , Thomas Eisenstecken , Gerhard Gompper , Roland G. Winkler

Understanding confined flows of complex fluids requires simultaneous access to the mechanical behaviour of the liquid and the boundary condition at the interfaces. Here, we use evanescent wave microscopy to investigate near-surface flows of…

软凝聚态物质 · 物理学 2020-12-01 Gabriel Guyard , Alexandre Vilquin , Nicolas Sanson , Frederic Restagno , Joshua D. Mcgraw

We construct a continuous-time, positively divisible non-Markovian process with memory of the initial state that satisfies the differential Chapman--Kolmogorov equation. In the stationary state, the correlation function exhibits exponential…

概率论 · 数学 2026-05-29 Bilal Canturk , Gokhan Baris Bagci , Onur Pusuluk

Non-Markovian effects are important in modeling the behavior of open quantum systems arising in solid-state physics, quantum optics as well as in study of biological and chemical systems. The non-Markovian environment is often approximated…

量子物理 · 物理学 2022-01-05 Rahul Trivedi , Daniel Malz , J. Ignacio Cirac

We study the reaction kinetics of end-functionalized polymer chains dispersed in an unreactive polymer melt. Starting from an infinite hierarchy of coupled equations for many-chain correlation functions, a closed equation is derived for the…

软凝聚态物质 · 物理学 2009-10-31 Ben O'Shaughnessy , Dimitrios Vavylonis

Recent theoretical works exploring the hydrodynamics of soft material in non-equilibrium situations are reviewed. We discuss the role of hydrodynamic interactions for three different systems: i) the deformation and orientation of…

软凝聚态物质 · 物理学 2012-03-08 Manoel Manghi , Xaver Schlagberger , Yong-Woon Kim , Roland R. Netz