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In this paper we consider calculation of two-centre exchange integrals over Slater-type orbitals (STOs). We apply the Neumann expansion of the Coulomb interaction potential and consider calculation of all basic quantities which appear in…

量子物理 · 物理学 2016-11-04 Michał Lesiuk , Robert Moszynski

In this paper, which constitutes the first part of the series, we consider calculation of two-centre Coulomb and hybrid integrals over Slater-type orbitals (STOs). General formulae for these integrals are derived with no restrictions on the…

量子物理 · 物理学 2015-01-09 Michał Lesiuk , Robert Moszynski

In this paper methods for calculations of multi-center integrals of squared Coulomb potentials and Slater-type orbitals (STO) are derived. These integrals are necessary for accurate lower bounds to energy levels of molecular systems. All…

化学物理 · 物理学 2022-02-10 Sohei Ashida

The electron repulsion integrals over the Slater-type orbitals with non-integer principal quantum numbers are considered. These integrals are useful in both non-relativistic and relativistic calculations of many-electron systems. They…

量子物理 · 物理学 2023-01-05 A. Bağcı , Gustavo A. Aucar

We present a fast algorithm to calculate Coulomb/exchange integrals of prolate spheroidal electronic orbitals, which are the exact solutions of the single-electron, two-center Schr\"odinger equation for diatomic molecules. Our approach…

量子物理 · 物理学 2012-08-01 Christian B. Mendl

We present analytical formulas for the calculation of the two-center two-electron integrals in the basis of Slater geminals and products of Slater orbitals. Our derivation starts with establishing a inhomogeneous fourth-order ordinary…

量子物理 · 物理学 2012-12-07 Michał Lesiuk , Robert Moszynski

This paper advocates use of the atomic orbitals which have direct physical interpretation, i.e. Coulomb Sturmians and hydrogen-like orbitals. They are exponential type orbitals (ETOs). Their radial nodes are shown to be essential in…

量子物理 · 物理学 2010-10-27 Philip E. Hoggan

In this study, using the analytical and recurrence relations suggested by the authors in previous works, the new efficient and reliable program procedure for the overlap integrals over Slater type orbitals (STOs) is presented. The proposed…

化学物理 · 物理学 2015-05-13 I. I. Guseinov , B. A. Mamedov

The Slater orbitals are the natural basis functions in quantum molecular calculations. Three-center repulsion Coulomb-exchange integrals over Slater orbitals are evaluated analytically with arbitrary orbital exponents, first for linear…

数学物理 · 物理学 2012-09-18 Telhat Özdogan , Maria Belen Ruiz

The two-center two-electron Coulomb and hybrid integrals arising in relativistic and nonrelativistic ab-initio calculations of molecules are evaluated over the non-integer Slater-type orbitals via ellipsoidal coordinates. These integrals…

量子物理 · 物理学 2014-05-22 Ali Bağcı , Philip E. Hoggan

Using one-center expansion relations for the Slater type orbitals (STOs) of noninteger principal quantum numbers in terms of integer n STOs derived in this study with the help of - exponential type orbitals (-ETOs, the general formulas are…

化学物理 · 物理学 2007-06-13 I. I. Guseinov

In this study, the one-center expansion formulas in terms of complete orthonormal sets of -exponential type orbitals (-ETOs,) are established for the Slater type orbitals (STOs) and Coulomb-Yukawa like correlated interaction potentials…

化学物理 · 物理学 2013-02-12 I. I. Guseinov

Some typical overlap/potential energy integrals which occur in the use of extended Hylleraas-configuration interaction (E-Hy-CI) functions with Slater-type orbital (STO) basis for two-electron atomic structure calculations, have been…

原子物理 · 物理学 2019-01-23 B Padhy

We derive direct single-stage numerical evaluation of the electronic overlap integral between arbitrary atomic orbitals (including STOs). Integration is over cartesian co-ordinates, and replaces previous sums over 'special' functions. The…

化学物理 · 物理学 2016-04-21 Michael J Caola

Various properties of the general two-center two-electron integral over the explicitly correlated exponential function are analyzed for the potential use in high precision calculations for diatomic molecules. A compact one dimensional…

化学物理 · 物理学 2015-06-11 Krzysztof Pachucki

We present a general methodology to evaluate matrix elements of the effective core potentials (ECPs) within one-electron basis set of Slater-type orbitals (STOs). The scheme is based on translation of individual STO distributions in the…

化学物理 · 物理学 2017-05-17 Michal Lesiuk , Aleksandra M. Tucholska , Robert Moszynski

Ozdogan (Int. J. Quantum Chem., 92 (2003) 419) published formulas for evaluating the multielectron multicenter molecular integrals over Slater-type orbitals (STOs). It is demonstrated that the formulas presented in this work are not…

化学物理 · 物理学 2007-05-23 I. I. Guseinov

In this work, series expansions in terms of Bessel functions of the first kind are given for the sine and cosine integrals. These representations differ from many of the known Neumann-type series expansions for the sine and cosine…

经典分析与常微分方程 · 数学 2017-06-13 Chance Sanford

We discuss the efficient computation of the auxiliary integrals that arise when resolutions of two-electron operators (specifically, the Coulomb and long-range Ewald operators) are employed in quantum chemical calculations. We derive a…

化学物理 · 物理学 2013-01-10 Taweetham Limpanuparb , Joshua W. Hollett , Peter M. W. Gill

We present an efficient approach to evaluate two-center two-electron integrals with exponential functions and with an arbitrary polynomial in electron-nucleus and electron-electron distances. We show that the master integral with the single…

化学物理 · 物理学 2009-09-29 Krzysztof Pachucki
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