相关论文: A multi-pathway model for Photosynthetic reaction …
We describe a method for simulating exciton dynamics in protein-pigment complexes, including effects from charge transfer as well as fluorescence. The method combines the hierarchical equations of motion, which are used to describe quantum…
We theoretically investigate a photosystem II-based reaction center modeled as a nonequilibrium quantum junction. We specifically focus on the electron-electron interactions that enable cotunneling events to be captured through quantum…
We analyze a theoretical model for energy and electron transfer in an artificial photosynthetic system. The photosystem consists of a molecular triad (i.e., with a donor, a photosensitive unit, and an acceptor) coupled to four accessory…
We study a model of a light-induced proton pump in artificial reaction centers. The model contains a molecular triad with four electron states (i.e., one donor state, two photosensitive group states, and one acceptor state) as well as a…
Understanding the behavior of charged complex fluids is crucial for a plethora of important industrial, technological, and medical applications. Using coarse-grained molecular dynamics simulations, here we investigate the properties of a…
Quantum information theorems state that it is possible to exploit collective quantum resources to greatly enhance the charging power of quantum batteries (QBs) made of many identical elementary units. We here present and solve a model of a…
One of the promising approaches to revealing the photosynthetic efficiency of close to one unit is to investigate the quantum regime of excitation energy transfer (EET). The majority of studies, however, have concluded that different…
Quantum batteries (QBs), harnessing quantum systems to transfer and store energy, have garnered substantial attention recently, enabling potentials in enhanced charging capacity, increased charging power, and device miniaturization.…
Non-equilibrium transport properties and energy conversion performance of a molecular photo-voltaic cell are analyzed using the Lindblad master equation within the open quantum systems approach. The method allows us to calculate the…
We explore a protocol that efficiently charges multiple open quantum batteries in parallel using a single charger. This protocol shows super-extensive charging through collective coupling of the charger and the battery to the same thermal…
A quantum heat engine (QHE) based on the interaction driving of a many-particle working medium is introduced. The cycle alternates isochoric heating and cooling strokes with both interaction-driven processes that are simultaneously…
The majority of photoelectrochemical (PEC) water splitting cells cannot drive the overall water splitting reactions without the assistance of an external power source. To provide added power, the cells are usually connected to photovoltaic…
The quantum well solar cell (QWSC) has been proposed as a route to higher efficiency than that attainable by homojunction devices. Previous studies have established that carriers escape the quantum wells with high efficiency in forward bias…
With intensive studies of quantum thermodynamics, quantum batteries (QBs) have been proposed to store and transfer energy via quantum effects. Despite many theoretical models, decoherence remains a severe challenge and practical platforms…
Separating heat from charge in a material is an extremely challenging task since they are transported by the very same carriers, i.e. electrons or holes. In this Letter we show that such separation can reach 100% efficiency in a hybrid…
Recently, significant progress in the development of III-V/Si dual-junction solar cells has been achieved. This not only boosts the efficiency of Si-based photovoltaic solar cells, but also offers the possibility of highly efficient green…
Enhanced interaction between two two-level emitters (e.g., atoms) by nonreciprocal photonic media can be of benefit to broad areas, from quantum information science to biological detection. Here we provide a detailed analysis on why…
Recombination of photogenerated charge carriers in polymer bulk heterojunction (BHJ) solar cells reduces the short circuit current (Jsc) and the fill factor (FF). Identifying the mechanism of recombination is, therefore, fundamentally…
In organic photovoltaic systems, a photogenerated molecular exciton in the donor domain dissociates into a hole and an electron at the donor/acceptor heterojunction, and subsequently separate into free charge carriers that can be extracted…
In green plants, chlorophyll-a and chlorophyll-b are the predominant pigments bound to light-harvesting proteins. While the individual characteristics of these chlorophylls are well understood, the advantages of their coexistence remain…