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We use above-bandgap optical excitation, via a 1047 nm laser, to hyperpolarize the $^{31}$P spins in low-doped (N$_D =6\times10^{15}$ cm$^{-3}$) natural abundance silicon at 4.2 K and 6.7 T, and inductively detect the resulting NMR signal.…

介观与纳米尺度物理 · 物理学 2018-11-21 P. Gumann , H. Haas , S. Sheldon , L. Zhu , M. L. W. Thewalt , D. G. Cory , C. Ramanathan

We demonstrate a method which can hyperpolarize both the electron and nuclear spins of 31P donors in Si at low field, where both would be essentially unpolarized in equilibrium. It is based on the selective ionization of donors in a…

Coherence times of electron spins bound to phosphorus donors have been measured, using a standard Hahn echo technique, to be up to 20 ms in isotopically pure silicon with [P]$ = 10^{14}$ cm$^{-3}$ and at temperatures $\leq 4 $K. Although…

介观与纳米尺度物理 · 物理学 2020-12-29 Philipp Ross , Brendon C. Rose , Cheuk C. Lo , Mike L. W. Thewalt , Alexei M. Tyryshkin , Stephen A. Lyon , John J. L. Morton

We characterize the phase memory time of phosphorus donor electron spins in lightly-doped natural silicon at high magnetic field (8.58 T) in the dark and under low-power optical excitation. The spin echo decays are dominated by spectral…

量子物理 · 物理学 2021-07-15 Lihuang Zhu , Johan van Tol , Chandrasekhar Ramanathan

Phosphorus-doped silicon single crystals with 0.19 % <= f <= 99.2 %, where f is the concentration of 29^Si isotopes, are measured at 8 K using a pulsed electron spin resonance technique, thereby the effect of environmental 29^Si nuclear…

材料科学 · 物理学 2010-11-16 Eisuke Abe , Akira Fujimoto , Junichi Isoya , Satoshi Yamasaki , Kohei M. Itoh

A study of donor electron spins and spin--dependent electronic transitions involving phosphorous ($^{31}$P) atoms in proximity of the (111) oriented crystalline silicon (c-Si) to silicon dioxide (SiO$_{2}$) interface is presented for…

材料科学 · 物理学 2015-05-13 S. -Y. Paik , S. -Y. Lee , W. J. Baker , D. R. McCamey. C. Boehme

Pulsed electrically-detected magnetic resonance of phosphorous (31P) in bulk crystalline silicon at very high magnetic fields (B > 8.5 T) and low temperatures (T = 2.8 K) is presented. We find that the spin-dependent capture and reemission…

量子物理 · 物理学 2009-09-25 G. W. Morley , D. R. McCamey , H. A. Seipel , L. -C. Brunel , J. van Tol , C. Boehme

We use the nuclear spin coherence of $^{31}$P donors in $^{28}$Si to determine flip-flop rates of donor electron spins. Isotopically purified $^{28}$Si crystals minimize the number of $^{29}$Si flip-flops, and measurements at 1.7 K suppress…

We demonstrate the coherent control and electrical readout of the nuclear spins of ionized phosphorus donors in natural silicon. By combining pulsed illumination with coherent electron spin manipulation, we selectively ionize the donor…

材料科学 · 物理学 2012-01-17 Lukas Dreher , Felix Hoehne , Martin Stutzmann , Martin S. Brandt

We demonstrate an efficient control of $^{29}$Si nuclear spin orientation for specific lattice sites near $^{31}$P donors in silicon crystals at temperatures below 1 K and in high magnetic field of 4.6 T. Excitation of the forbidden…

We report a pulsed EPR study of the phase relaxation of electron spins bound to phosphorus donors in isotopically purified 29^Si and natural abundance Si single crystals measured at 8 K.

材料科学 · 物理学 2007-05-23 Eisuke Abe , Kohei M. Itoh , Junichi Isoya , Satoshi Yamasaki

Donor spins in silicon are some of the most promising qubits for upcoming solid-state quantum technologies. The nuclear spins of phosphorus donors in enriched silicon have among the longest coherence times of any solid-state system as well…

We experimentally demonstrate a method for obtaining nuclear spin hyperpolarization, that is, polarization significantly in excess of that expected for a thermal equilibrium. By exploiting a modified Overhauser process, we obtain more than…

材料科学 · 物理学 2009-02-26 D. R. McCamey , J. van Tol , G. W. Morley , C. Boehme

Pulsed electron paramagnetic resonance measurements of donor electron spins in natural phosphorus-doped silicon (Si:P) and isotopically-purified 28Si:P show a strongly temperature-dependent longitudinal relaxation time, T1, due to an Orbach…

材料科学 · 物理学 2009-11-10 A. M. Tyryshkin , S. A. Lyon , A. V. Astashkin , A. M. Raitsimring

Spins in the `semiconductor vacuum' of silicon-28 ($^{28}$Si) are suitable qubit candidates due to their long coherence times. An isotopically purified substrate of $^{28}$Si is required to limit the decoherence pathway caused by magnetic…

Single crystal silicon is an excellent system in which to explore dynamic nuclear polarization (DNP), as it exhibits a continuum of properties from metallic to insulating as a function of doping concentration and temperature. At low doping…

材料科学 · 物理学 2011-09-09 Anatoly E. Dementyev , David G. Cory , Chandrasekhar Ramanathan

The electron and nuclear spins of the shallow donor 31P are promising qubit candidates invoked in many proposed Si-based quantum computing schemes. We have recently shown that the near-elimination of inhomogeneous broadening in highly…

We demonstrate that the dynamic nuclear polarization (DNP) of phosphorus donors in silicon can be very effective in a magnetic field of 4.6 T and at temperatures below 1 K. The DNP occurs due to the Overhauser effect following a cross…

Spins of single donor atoms are attractive candidates for large scale quantum information processing in silicon, since quantum computation can be realized through the manipulation of electron and/or nuclear spins. We here report on…

材料科学 · 物理学 2007-05-23 A. Ferretti , M. Fanciulli , A. Ponti , A. Schweiger

Spectral diffusion arising from $^{29}$Si nuclear spin flip-flops, known to be a primary source of electron spin decoherence in silicon, is also predicted to limit the coherence times of neutral donor nuclear spins in silicon. Here, the…

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