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Understanding the molecular-level structure and dynamics of ice surfaces is crucial for deciphering several chemical, physical, and atmospheric processes. Vibrational sum-frequency generation (SFG) spectroscopy is the most prominent tool…

Freezing in the vicinity of water-vapor interfaces is of considerable interest to a wide range of disciplines, most notably the atmospheric sciences. In this work, we use molecular dynamics and two advanced sampling techniques, forward flux…

统计力学 · 物理学 2014-11-04 Amir Haji-Akbari , Ryan S. DeFever , Sapna Sarupria , Pablo G. Debenedetti

In this paper we study the process termed thermal regelation at single particle level. We experimentally extract the physical parameters that determine the interactions between ice and the silica particle for the regelation process. As the…

软凝聚态物质 · 物理学 2020-07-13 Siyu Chen , Julia M. H. Schollick , Roel P. A. Dullens , Dirk G. A. L. Aarts

We present a new microscopic model of granular medium to study the role of dynamical correlations and the onset of spatial order induced by the inelasticity of the interactions. In spite of its simplicity, it features several different…

统计力学 · 物理学 2009-11-07 A. Baldassarri , U. Marini Bettolo Marconi , A. Puglisi

Context. Millimetric observations have measured high degrees of molecular deuteration in several species seen around low-mass protostars. The Herschel Space Telescope, launched in 2009, is now providing new measures of the deuterium…

The properties of the interface between solid and melt are key to solidification and melting, as the interfacial free energy introduces a kinetic barrier to phase transitions. This makes solidification happen below the melting temperature,…

统计力学 · 物理学 2015-12-02 Bingqing Cheng , Gareth A. Tribello , Michele Ceriotti

Molecular simulations employing empiric force fields have provided valuable knowledge about the ice growth process in the last decade. The development of novel computational techniques allows us to study this process, which requires long…

软凝聚态物质 · 物理学 2023-06-07 Pablo Montero de Hijes , Salvatore Romano , Alexander Gorfer , Christoph Dellago

We derive a coarse-grained description of the dynamics of a nanoparticle immersed in an isothermal simple fluid by performing a systematic coarse graining of the underlying microscopic dynamics. As coarse-grained or relevant variables we…

介观与纳米尺度物理 · 物理学 2016-01-20 Pep Español , Aleksandar Donev

We investigate the properties of membranes under tension by Monte-Carlo simulations of a generic coarse-grained model for lipid bilayers. We give a comprising overview of the behavior of several membrane characteristics, such as the area…

生物物理 · 物理学 2010-03-17 Jörg Neder , Beate West , Peter Nielaba , Friederike Schmid

Grains of ice are formed spontaneously when water vapor is injected into a weakly-ionized laboratory plasma in which the background gas has been cooled to cryogenic temperatures comparable to those of deep space. These ice grains are…

等离子体物理 · 物理学 2024-04-26 André Nicolov , Murthy S. Gudipati , Paul M. Bellan

We characterize both analytically and numerically short-range forces between spatially diffuse interfaces in multi-phase-field models of polycrystalline materials. During late-stage solidification, crystal-melt interfaces may attract or…

材料科学 · 物理学 2015-05-14 N. Wang , R. Spatschek , A. Karma

Some basic questions about the hydrodynamical approach to relativistic heavy ion collisions are discussed aiming to clarify how far we can go with such an approach to extract useful information on the properties and dynamics of the QCD…

高能物理 - 唯象学 · 物理学 2015-06-11 Ph. Mota , T. Kodama , J. Takahashi , R. Derradi de Souza

Soft particles display highly versatile properties with respect to hard colloids, even more so at fluid-fluid interfaces. In particular, microgels, consisting of a cross-linked polymer network, are able to deform and flatten upon adsorption…

Convective flows coupled with solidification or melting in water bodies play a major role in shaping geophysical landscapes. Particularly in relation to the global climate warming scenario, it is essential to be able to accurately quantify…

流体动力学 · 物理学 2021-03-11 Ziqi Wang , Enrico Calzavarini , Chao Sun , Federico Toschi

When materials freeze, they often undergo damage due to ice growth. Although this damage is commonly ascribed to the volumetric expansion of water upon freezing, it is usually driven by suction of water towards growing ice crystals. The…

软凝聚态物质 · 物理学 2022-08-24 Dominic Gerber , Lawrence A. Wilen , Florian Poydenot , Eric R. Dufresne , Robert W. Style

Although the pattern formation on polymer gels has been considered as a result of the mechanical instability due to the volume phase transition, we found a macroscopic surface pattern formation not caused by the mechanical instability. It…

斑图形成与孤子 · 物理学 2007-05-23 Hiroaki Katsuragi

The issue of ice accumulation at low-temperature circumstances causes multiple problems and serious damages in many civil infrastructures which substantially influence human daily life. However, despite the significant consideration in…

化学物理 · 物理学 2020-11-24 Amir Afshar , Dong Meng

The low kinetic friction between ice and numerous counterbodies is commonly attributed to an interfacial water layer, which is believed to originate from pre-existing surface water or from melt water induced by high contact pressures or…

软凝聚态物质 · 物理学 2025-09-03 Achraf Atila , Sergey V. Sukhomlinov , Martin H. Müser

Water-ice systems undergoing melting develop complex spatio-temporal interface dynamics and a non-trivial temperature field. In this contribution, we present computational aspects of a recently conducted validation study that aims at…

流体动力学 · 物理学 2018-01-12 K. Schüller , B. Berkels , J. Kowalski

I use the method of classical density-functional theory in the weighted-density approximation of Tarazona to investigate the phase diagram and the interface structure of a two-dimensional lattice-gas model with three phases -- vapour,…

统计力学 · 物理学 2009-11-10 S. Prestipino