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A clear understanding of the mechanisms that control the electron dynamics in strong laser field is still a challenge that requires to be interpreted by advanced theory. Development of accurate theoretical and computational methods, able to…

We consider a quantum mechanical model for the high-order harmonic generation in bulk solids. The bandgap is assumed to be considerably larger than the exciting photon energy. Using dipole approximation, the dynamical equations for…

量子物理 · 物理学 2017-11-09 Viktor Szaszkó-Bogár , Katalin Varjú , Péter Földi

High harmonic generation(HHG) is one of the most commonly studied nonlinear optical phenomena, originating in the ultrafast dynamics of electrons in atomic gasses and semiconductors. It has attracted much attention because of its…

光学 · 物理学 2023-09-08 Akira Kofuji , Robert Peters

We studied the multi-plateau high-order harmonic generation (HHG) from solids numerically. It is found that the HHG spectrum in the second or higher plateau is redshifted in short laser pulses due to the nonadiabatic effect. The…

光学 · 物理学 2017-09-20 Guang-Rui Jia , Xue-Bin Bian

We investigate how short and long electron trajectory contributions to high harmonic emission and their interferences give access to intra-molecular dynamics. In the case of unaligned molecules, we show experimental evidences that the long…

We investigate the contributions from the $3\sigma_{g}$ and $1\pi_{u}$ and molecular orbitals in high-order harmonic generation in $N_{2}$, with particular emphasis on quantum-interference effects. We consider both the physical processes in…

原子物理 · 物理学 2009-09-08 C. Figueira de Morisson Faria , B. B. Augstein

We theoretically investigate correlated electron dynamics in high-harmonic generation (HHG), using all-electron \emph{ab initio} simulations for three-dimensional real alkali-metal atoms. The resulting harmonic spectra exhibit a plateau…

原子物理 · 物理学 2019-04-10 Yang Li , Takeshi Sato , Kenichi L. Ishikawa

High-harmonic generation (HHG) of a two-level-system driven by an intense monochromatic phase-locked laser is studied in terms of complex spectral analysis with the Floquet method. In contrast to the phenomenological approaches, this…

量子物理 · 物理学 2021-02-03 Hidemasa Yamane , Ken-ichi Noba , Tomio Petrosky , Satoshi Tanaka

The interaction of intense mid-infrared laser fields with atoms and molecules leads to a range of new opportunities, from the production of bright, coherent radiation in the soft x-ray range to imaging molecular structures and dynamics with…

The objective of this article is to investigate the profound nonlinear optical response exhibited by inversion symmetric fullerene molecules under the influence of different types of disorders described by the Anderson model. Our aim is to…

光学 · 物理学 2023-09-06 H. K. Avetissian , S. Sukiasyan , H. H. Matevosyan , G. F. Mkrtchian

High-order harmonic generation (HHG) with relativistically strong laser pulses is considered employing electron ionization-recollisions from multiply charged ions in counterpropagating, linearly polarized attosecond pulse trains. The…

原子物理 · 物理学 2015-05-19 Markus C. Kohler , Michael Klaiber , Karen Z. Hatsagortsyan , Christoph H. Keitel

High-harmonic generation (HHG) is one of the fundamental processes at the heart of attosecond physics. Traditionally viewed as an effective single-particle effect, recent advances have focused on contributions beyond this single-particle…

We present a theoretical study of high-order harmonic generation (HHG) driven by ultrashort optical pulses with different kind of chirps. The goal of the present work is perform a detailed study to clarify the relevant parameters in the…

原子物理 · 物理学 2016-12-21 E Neyra , F Videla , J A Pérez-Hernández , M F Ciappina , L Roso , G A Torchia

We show that the dependence of high-order harmonic generation (HHG) on the molecular orientation can be understood within a theoretical treatment that does not involve the strong field of the laser. The results for H_2 show excellent…

原子物理 · 物理学 2009-11-10 B. Zimmermann , M. Lein , J. M. Rost

We propose a novel picture of high-harmonic generation (HHG) in solids based on the concept of temporally changing band structures. To demonstrate the utility of this picture, we focus on the high-order sideband generation (HSG) caused by…

材料科学 · 物理学 2019-08-14 Tomohiro Tamaya , Takeo Kato

High harmonic generation (HHG) is an established means of producing coherent, short wavelength, ultrafast pulses from a compact set-up. Table-top high-harmonic sources are increasingly being used to image physical and biological systems…

光学 · 物理学 2016-08-02 David T. Lloyd , Kevin O'Keeffe , Patrick N. Anderson , Simon M. Hooker

High-harmonic generation (HHG) provides short-wavelength light that is useful for precision spectroscopy and probing ultrafast dynamics. We report efficient, phase-coherent harmonic generation up to 9th-order (333 nm) in chirped…

The generation of high-order harmonics in bulk solids subjected to intense ultrashort laser pulses has opened up new avenues for research in extreme nonlinear optics and light-matter interaction on sub-cycle timescales. Despite significant…

High harmonic generation (HHG) provides a flexible framework for the development of coherent light sources in the extreme-ultraviolet and soft x-ray regimes. However it suffers from low conversion efficiencies as the control of the HHG…

光学 · 物理学 2014-09-16 Alberto Castro , Angel Rubio , E. K. U. Gross

To clarify the microscopic origin of chirality-induced optical effect, we develop an analytical method that extracts the chiral part of the Hamiltonian of molecular electronic states. We demonstrate this method in a model chiral molecule…

材料科学 · 物理学 2024-09-04 Akihito Kato , Nobuhiko Yokoshi