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We present derivation and implementation of the Multi-Configurational Strong-Field Approximation with Gaussian nuclear Wave Packets (MC-SFA-GWP) -- a version of the molecular strong-field approximation which treats all electronic and…

化学物理 · 物理学 2017-11-10 Serguei Patchkovskii , Michael S. Schuurman

We present experimental results showing the appearance of a near-continuum in the high-order harmonic generation (HHG) spectra of atomic and molecular species as the driving laser intensity of an infrared pulse increases. Detailed…

The observation of non-perturbative harmonic emission in solids from ultrashort laser pulses [1] sparked a wave of studies [2,3] as a probe of charge carrier dynamics in solids under strong fields and a route to extreme ultraviolet (XUV)…

We experimentally observe a new type of quantum-path interference, in two-dimensions (2D-QPI), in high-harmonic generation (HHG) driven by an orthogonally-polarised highly-bichromatic field. This regime is marked by comparable intensities…

High-harmonic generation (HHG) in crystalline solids have been examined so far on the basis of one-body energy-band structures arising from electron itineracy in a periodic potential. Here, we show emergence of HHG signals which are…

强关联电子 · 物理学 2020-04-22 Shohei Imai , Atsushi Ono , Sumio Ishihara

We investigate harmonic generation (HG) from ground-state Ar+ aligned with M=1 at a laser wavelength of 390-nm and intensity of 4x10(14) Wcm-2. Using time-dependent R-matrix theory, we find that an initial state with magnetic quantum number…

原子物理 · 物理学 2013-10-01 A. C. Brown , Hugo W. van der Hart

We present a theoretical investigation into the two-center interference in aligned H$_2^+$. The influence of the laser field on the recombination step is investigated by comparing laser-induced harmonic generation with harmonic generation…

原子物理 · 物理学 2015-05-19 Elmar V. van der Zwan , Manfred Lein

We theoretically study multielectron effects in high-harmonic generation (HHG), using all-electron first-principles simulations for a one-dimensional (1D) model atom. In addition to usual plateau and cutoff (from a cation in the present…

原子物理 · 物理学 2017-05-24 Iliya Tikhomirov , Takeshi Sato , Kenichi L. Ishikawa

An analytic description of high harmonic generation (HHG) in solids induced by intense low-frequency pulses is presented within an adiabatic approach, which treats laser-matter interactions nonperturbatively. We derive the analytical…

光学 · 物理学 2026-01-01 A. V. Flegel , Liang-Wen Pi , M. V. Frolov

We describe phase-dependent wavelength scaling of high-order harmonic generation efficiency driven by ultra-short laser fields in the mid-infrared. We employ both numerical solution of the time-dependent Schr\"{o}dinger equation and the…

原子物理 · 物理学 2015-06-17 I. Yavuz , E. A. Bleda , Z. Altun , T. Topcu

High-harmonic generation (HHG) normally requires a careful adjustment of the driving laser intensity (typically $10^{14} - 10^{15}$ W/cm$^2$) and gas medium parameters to enable good phase matching conditions. In contrast with conventional…

For the high-order harmonic generation in solids, we find a distinct and clean interference pattern in the high-energy end of the spectrum which can be interpreted as a Michelson interferometer of the Bloch electron. Our results are…

We study numerically the Bloch electron wave-packet dynamics in periodic potentials to simulate laser-solid interactions. We introduce a quasi-classical model in the \emph{k} space combined with the energy band structure to understand the…

光学 · 物理学 2017-01-05 Tao-Yuan Du , Xue-Bin Bian

We propose a new scheme for high gain harmonic generation free electron lasers (HGHG FELs), which is seeded by a pair of intersecting laser beams to interact with an electron beam in a modulator undulator located in a dispersive section.…

加速器物理 · 物理学 2017-03-17 Takashi Tanaka , Ryota Kinjo

High-order harmonic generation (HHG) in simultaneous intense near-infrared (NIR) laser light and brilliant x rays above an inner-shell absorption edge is examined. A tightly bound inner-shell electron is transferred into the continuum.…

We consider harmonics generation and wave-mixing by two-color multi photon resonant excitation of three-level atoms/molecules in strong laser fields. The coherent part of the spectra corresponding to multicolor harmonics generation is…

原子物理 · 物理学 2016-08-24 H. K. Avetissian , B. R. Avchyan , G. F. Mkrtchian

We address the influence of the orbital symmetry and of the molecular alignment with respect to the laser-field polarization on laser-induced nonsequential double ionization of diatomic molecules, in the length and velocity gauges. We work…

原子物理 · 物理学 2009-11-13 C. Figueira de Morisson Faria , T. Shaaran , X. Liu , W. Yang

We theoretically investigate high-order harmonic generation (HHG) in Rydberg atoms driven by spatially inhomogeneous laser fields, induced, for instance, by plasmonic enhancement. It is well known that the laser intensity should to exceed…

原子物理 · 物理学 2016-07-08 Y. Tikman , I. Yavuz , M. F. Ciappina , A. Chacon , Z. Altun , M. Lewenstein

By using Bohmian trajectory method, we investigate the dynamic interference in diatomic molecular high-order harmonic generation progress. It is demonstrated that the main characteristics of the molecular harmonic spectrum can be well…

原子物理 · 物理学 2013-08-05 Yang Song , Bing-Bing Wang , Fu-Ming Guo , Su-Yu Li , Xue-Shen Liu , Ji-Gen Chen , Si-Liang Zeng , Yu-Jun Yang

High-harmonic generation (HHG) is a strong-field phenomenon that is sensitive to the attosecond dynamics of tunnel ionization and coherent transport of electron-hole pairs in solids. While the foundations of solid HHG have been established,…