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We report on calculations of harmonic generation by neon in a mixed (800-nm + time-delayed 400-nm) laser pulse scheme. In contrast with previous studies we employ a short (few-cycle) 400-nm pulse, finding that this affords control of the…

原子物理 · 物理学 2017-01-20 K. R. Hamilton , H. W. van der Hart , A. C. Brown

We experimentally and numerically study the atomic response and pulse propagation effects of high-order harmonics generated in Xe, Kr, and Ar driven by a 2.1-\mu m infrared femtosecond light source. The light source is an optical parametric…

In recent years, techniques of intense THz laser have enabled us to experimentally observe nonlinear spin dynamics in antiferromagnets since the elementary excitations such as magnons reside on a THz to GHz range in antiferromagnets and THz…

强关联电子 · 物理学 2026-04-09 Yuto Jita , Minoru Kanega , Takumi Ogawa , Shunsuke C. Furuya , Masahiro Sato

Recent measurements on high-order harmonic generation (HHG) from N$_2$ aligned perpendicular to the driving laser polarization [B. K. McFarland {\it el al}, Science {\bf 322}, 1232 (2008)] have shown a maximum at the rotational…

原子物理 · 物理学 2009-10-30 Anh-Thu Le , R. R. Lucchese , C. D. Lin

The use of structured light to drive highly nonlinear processes in matter not only enables imprinting spatially-resolved properties onto short-wavelength radiation, but also opens alternative avenues for exploring the dynamics of nonlinear…

We theoretically investigate high-order harmonic generation (HHG) in graphene under mid-infrared (MIR) and terahertz (THz) fields based on a quantum master equation. Numerical simulations show that MIR-induced HHG in graphene can be…

材料科学 · 物理学 2023-07-03 Wenwen Mao , Angel Rubio , Shunsuke A. Sato

By combining analytical and numerical approaches, we study resonantly enhanced second-harmonic generation (SHG) by individual high-index dielectric nanoparticles made of centrosymmetric materials. Considering both bulk and surface…

光学 · 物理学 2018-01-08 Daria Smirnova , Alexander I. Smirnov , Yuri S. Kivshar

We explore with ab-initio theory high harmonic generation (HHG) from a series of gas-phase fullerenes (from C$_{20}$ to C$_{60}$, including isomers) under varying laser conditions (different ellipticities, angular orientations, intensities…

光学 · 物理学 2026-02-27 Km Akanksha Dubey , Ofer Neufeld

High-harmonic generation (HHG) is a coherent optical process in which the incident photon energy is up-converted to the multiples of its initial energy. In solids, under the influence of a strong laser field, electron-hole (e-h) pairs are…

We extend the semi-classical trajectory description for the high-order harmonic generation~(HHG) from solids by integrating the effect of electron-scattering. Comparing the extended semi-classical trajectory model with a one-dimensional…

We investigate the generation of higher-order harmonics from a quantum optics perspective via the interaction of a semiconductor with a coherent pump field focusing on the regime where strong-field intraband excitations dominate. The…

High-order harmonic generation (HHG) from molecular ion HeH$^{2+}$ in two initial states of $1s\sigma$ (ground state) and $2p\sigma$ (first excited state) is investigated theoretically, in homogeneous and plasmonic-enhanced laser fields.…

原子物理 · 物理学 2018-07-04 Nehzat Safaei

Quantum high-harmonic generation (HHG) is a prominent and growing field of research with potential capabilities of providing high photon-number entangled states of light. However, there is an open debate regarding the theory level required…

量子物理 · 物理学 2026-03-16 Sebastián de-la-Peña , Heiko Appel , Angel Rubio , Ofer Neufeld

We experimentally explore the fingerprint of the microscopic electron dynamics in second-order harmonic generation (SHG). It is shown that the interbond electron hopping induces a novel source of nonlinear polarization and plays an…

High-harmonic generation in solids allows probing and controlling electron dynamics in crystals on few femtosecond timescales, paving the way to lightwave electronics. In the spatial domain, recent advances in the real-space interpretation…

We theoretically study the high-harmonic generation (HHG) in one-dimensional spin systems. While in electronic systems the driving by AC electric fields produces radiation from the dynamics of excited charges, we consider here the situation…

强关联电子 · 物理学 2019-05-24 Shintaro Takayoshi , Yuta Murakami , Philipp Werner

Backscattering of delocalized electrons has been recently established [Phys. Rev. A 105, L041101 (2022)] as a mechanism to enhance high-order harmonic generation (HHG) in periodic systems with broken translational symmetry. Here we study…

原子物理 · 物理学 2022-07-12 Chuan Yu , Ulf Saalmann , Jan M. Rost

We study the crystal-momentum-resolved contributions to the high-order harmonic generation (HHG) in band-gap materials, and identify the relevant initial crystal momenta for the first and higher plateaus of the HHG spectra. We do so by…

原子物理 · 物理学 2020-09-09 Chuan Yu , Hossein Iravani , Lars Bojer Madsen

We investigate the nonlinear optical response of bulk ZnO under intense short-wave infrared excitation, focusing on the interplay between high-harmonic generation (HHG) and photoluminescence (PL). While HHG exhibits non-perturbative…

The generation of high harmonics is a strongly nonlinear effect that allows to probe properties of the target and to study electron dynamics in matter. It has been investigated in many different kinds of targets, including molecular gases,…

量子物理 · 物理学 2026-05-06 Lina Bielke , Samuel Schöpa , Falk-Erik Wiechmann , Franziska Fennel , Dieter Bauer