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A homogeneous thin polymer film with a stepped height profile levels due to the presence of Laplace pressure gradients. Here we report on studies of polymeric samples with precisely controlled, spatially inhomogeneous molecular weight…

软凝聚态物质 · 物理学 2014-01-07 Joshua D. McGraw , Thomas Salez , Oliver Bäumchen , Elie Raphaël , Kari Dalnoki-Veress

Surface tension-driven flow techniques have recently emerged as an efficient means of shedding light into the rheology of thin polymer films. Motivated by experimental and theoretical approaches in films bearing a varying surface…

软凝聚态物质 · 物理学 2017-04-26 Ioannis Tanis , Hendrik Meyer , Thomas Salez , Elie Raphaël , Anthony C. Maggs , Jörg Baschnagel

Flow in thin films is highly dependent on the boundary conditions. Here, we study the capillary levelling of thin bilayer films composed of two immiscible liquids. Specifically, a stepped polymer layer is placed atop another, flat polymer…

软凝聚态物质 · 物理学 2021-01-27 Vincent Bertin , Carmen Lee , Thomas Salez , Elie Raphael , Kari Dalnoki-Veress

A thin liquid film with non-zero curvature at its free surface spontaneously flows to reach a flat configuration, a process driven by Laplace pressure gradients and resisted by the liquid's viscosity. Inspired by recent progresses on the…

We report on the numerical implementation of thin film equations that describe the capillary-driven evolution of viscous films, in two-dimensional configurations. After recalling the general forms and features of these equations, we focus…

Thin viscous liquid films driven by capillarity are well described in the lubrication theory through the thin film equation. In this article, we present an analytical solution of this equation for a particular initial profile: a stepped…

软凝聚态物质 · 物理学 2015-06-11 Thomas Salez , Joshua D. McGraw , Oliver Bäumchen , Kari Dalnoki-Veress , Élie Raphaël

The surface of a thin liquid film with nonconstant curvature flattens as a result of capillary forces. While this leveling is driven by local curvature gradients, the global boundary conditions greatly influence the dynamics. Here, we study…

We compare the capillary levelling of a random surface perturbation on a thin polystyrene film with a theoretical study on the two-dimensional capillary-driven thin film equation. Using atomic force microscopy, we follow the time evolution…

软凝聚态物质 · 物理学 2014-10-16 Michael Benzaquen , Paul Fowler , Laetitia Jubin , Thomas Salez , Kari Dalnoki-Veress , Elie Raphaël

We study the free-surface deformation dynamics of an immersed glassy thin polymer film supported on a substrate, induced by an air nanobubble at the free surface.We combine analytical and numerical treatments of the glassy thin film…

材料科学 · 物理学 2021-04-08 Christian Pedersen , Shuai Ren , Yuliang Wang , Andreas Carlson , Thomas Salez

We study theoretically the profile evolution of a thin viscoelastic film supported onto a no-slip flat substrate. Due to the nonconstant initial curvature at the free surface, there is a flow driven by Laplace pressure and mediated by…

软凝聚态物质 · 物理学 2014-05-16 Michael Benzaquen , Thomas Salez , Elie Raphaël

We present experiments to study the relaxation of a nano-scale cylindrical perturbation at one of the two interfaces of a thin viscous free-standing polymeric film. Driven by capillarity, the film flows and evolves towards equilibrium by…

软凝聚态物质 · 物理学 2020-05-13 Vincent Bertin , John Niven , Howard A. Stone , Thomas Salez , Elie Raphael , Kari Dalnoki-Veress

The study of viscous thin film flow has led to the development of highly nonlinear partial differential equations that model how the evolution of the film height is affected by different forces. We investigate a model of interaction between…

流体动力学 · 物理学 2024-07-25 Steven A Kedda , Michael C Dallaston , Scott W McCue

We report on the capillary-driven levelling of a topographical perturbation at the surface of a free-standing liquid nanofilm. The width of a stepped surface profile is found to evolve as the square root of time. The hydrodynamic model is…

Thin polymer films have striking dynamical properties that differ from their bulk counterparts. With the simple geometry of a stepped polymer film on a substrate, we probe mobility above and below the glass transition temperature…

Confining glassy polymer into films can substantially modify their local and film-averaged properties. We present a lattice model of film geometry with void-mediated facilitation behaviors but free from any elasticity effect. We analyze the…

软凝聚态物质 · 物理学 2024-05-17 Qiang Zhai , Xin-Yuan Gao , Chun-Shing Lee , Chin-Yuan Ong , Ke Yan , Hai-Yao Deng , Sen Yang , Chi-Hang Lam

We find solutions that describe the levelling of a thin fluid film, comprising a non-Newtonian power-law fluid, that coats a substrate and evolves under the influence of surface tension. We consider the evolution from both periodic and…

流体动力学 · 物理学 2024-04-12 Michael C Dallaston

We present a control-volume approach for deriving a simplified model for the gravity-driven flow of an axisymmetric liquid film along a vertical fiber. The model accounts for gravitational, viscous, inertial and surface tension effects and…

流体动力学 · 物理学 2021-04-14 Y. Ruan , A. Nadim , L. Duvvoori , M. Chugunova

The surface structure of converging thin fluid films displays self-similar behavior, as was shown in the work by Diez et al [Q. Appl. Math 210, 155, 1990]. Extracting the related similarity scaling exponents from either numerical or…

We have studied the liquid-like response of the surface of vapour-deposited glassy films of polystyrene to the introduction of gold nanoparticles on the surface. The build-up of polymer material was measured as a function of time and…

We consider thin fluid films placed on thermally conductive substrates and exposed to time-dependent spatially uniform heat source. The evolution of the films is considered within the long-wave framework in the regime such that both…

软凝聚态物质 · 物理学 2016-06-16 Nanyi Dong , Lou Kondic
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