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Defects play an important role in determining the type of carriers as well as on tuning the physical properties of layered materials. In this study, we have demonstrated that by varying the growth kinetics one can control the defects and…

材料科学 · 物理学 2023-07-03 Sonali Baral , Indu Rajput , Mukesh Kumar Dasoundhi , Devendra Kumar , Archana Lakhani

With a large band gap and a single Dirac cone responsible for the topological surface states, Bi2Se3 is widely regarded as a prototypical 3D topological insulator. Further applications of the bulk material has, however, been hindered by…

材料科学 · 物理学 2023-06-02 Rodrigo T. Paulino , Marcos A. Avila

We report molecular beam epitaxy growth of Sr-doped Bi$_2$Se$_3$ films on (111) BaF$_2$ substrate, aimed to realize unusual superconducting properties inherent to Sr$_x$Bi$_2$Se$_3$ single crystals. Despite wide range of the compositions,…

Bismuth selenide Bi$_2$Se$_3$ was grown by molecular beam epitaxy while carrier density and mobility were measured directly \emph{in situ} as a function of film thickness. Carrier density shows high interface n-doping (1.5 x 10$^{13}$…

Despite numerous studies on three-dimensional topological insulators (3D TIs), the controlled growth of high quality (bulk-insulating and high mobility) TIs remains a challenging subject. This study investigates the role of growth methods…

Combining high resolution scanning tunneling microscopy and first principle calculations, we identified the major native defects, in particular the Se vacancies and Se interstitial defects that are responsible for the bulk conduction and…

材料科学 · 物理学 2016-09-07 Jixia Dai , Damien West , Xueyun Wang , Yazong Wang , Daniel Kwok , S-W. Cheong , S. B. Zhang , Weida Wu

Bi2Se3 is a topological insulator with metallic surface states residing in a large bulk bandgap. It is believed that Bi2Se3 gets additional n-type doping after exposure to atmosphere, thereby reducing the relative contribution of surface…

Using first-principles method within the framework of the density functional theory, we study the influence of native point defect on the structural and electronic properties of Bi$_2$Se$_3$. Se vacancy in Bi$_2$Se$_3$ is a double donor,…

材料科学 · 物理学 2012-07-03 L. Xue , P. Zhou , C. X. Zhang , C. Y. He , G. L. Hao , L. Z. Sun , J. X. Zhong

Achieving true bulk insulating behavior in Bi$_2$Se$_3$, the archetypal topological insulator with a simplistic one-band electronic structure and sizable band gap, has been prohibited by a well-known self-doping effect caused by selenium…

材料科学 · 物理学 2017-01-19 Paul Syers , Johnpierre Paglione

A comparative study of the properties of topological insulator Bi2Te2Se (BTS) crystals grown by the vertical Bridgeman method is described. Two defect mechanisms that create acceptor impurities to compensate for the native n-type carriers…

We present a study of the structural and electronic properties of highly doped topological insulator Bi2Se3 single crystals synthesized by the Bridgman method. Lattice structural characterizations by X-ray diffraction, scanning tunneling…

材料科学 · 物理学 2012-12-07 Helin Cao , Suyang Xu , Ireneusz Miotkowski , Jifa Tian , Deepak Pandey , M. Zahid Hasan , Yong P. Chen

The layered delafossite-like antiferromagnet AgCrSe$_2$ is a superionic conductor at high temperatures and has been reported to exhibit anomalous Hall behavior and Kondo physics at low temperatures. These extraordinary transport properties…

Bismuth selenide (Bi2Se3) is a good topological insulator (TI) with its surface band Dirac point inside the bulk bandgap. However, Bi2Se3 films grown by molecular beam epitaxy (MBE) often require tuning of Fermi level near the Dirac point…

介观与纳米尺度物理 · 物理学 2025-09-11 Shu-Wei Wang , Hang Chi , Jui-Che Chung

Single crystals of KNbO3 and KNbO3 : Fe have been grown using the flux method at various technological conditions. The investigations of optical absorption of these crystals were carried out. Marked influence of technological conditions and…

凝聚态物理 · 物理学 2007-05-23 M. Milata , K. Wojcik , K. Zieleniec

Atomic level defects such as dislocations play key roles in determining the macroscopic properties of crystalline materials. Their effects are important and wide-reaching, and range from increased chemical reactivity to enhanced mechanical…

Topological insulators possess a non-conductive bulk and present surface states, henceforth, they are electrically conductive along their boundaries. Bismuth selenide ($Bi_2Se_3$) is one of the most promising topological insulators.…

We employed first-principles calculations to investigate the thermoelectric transport properties of the compound As$_2$Se$_3$. Early experiments and calculations have indicated that these properties are controlled by a kind of native defect…

材料科学 · 物理学 2023-07-27 Anderson S. Chaves , Murilo Aguiar Silva , Alex Antonelli

Here, we report the effect of europium (Eu) doping in Bi2Se3 topological insulator (TI) by using different characterization techniques viz. X-ray diffraction (XRD), scanning electron microscopy (SEM) coupled with energy dispersive X-ray…

材料科学 · 物理学 2019-09-09 Rabia Sultana , Ganesh Gurjar , Bhasker Gahtori , Satyabrata Patnaik , V. P. S. Awana

We report the detailed study of structural micro-structuraland high magnetic field magneto transport propertiesof Bi2Se3single crystal. Bi2Se3 single crystal is grown through conventional solid-state reaction route via the self-flux method.…

An archetypical layered topological insulator Bi$_2$Se$_3$ becomes superconductive upon doping with Sr, Nb or Cu. Superconducting properties of these materials in the presence of in-plane magnetic field demonstrate spontaneous symmetry…

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