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The probability that photoionization of the caged atom in an endohedral system is accompanied by excitation of the fullerene shell is shown to be close to unity in broad intervals of the photoelectron energies. The result is obtained by…

原子物理 · 物理学 2015-06-15 E. G. Drukarev , M. Ya. Amusia

Near-threshold resonances have been studied for Be-like ions with a focus on overlapping resonances among Rydberg series converging to different thresholds. The behavior of the overlapping as a function of Z and the approach to the limit of…

原子物理 · 物理学 2012-05-25 W. -C. Chu , H. -L. Zhou , A. Hibbert , S. T. Manson

Ta2NiSe5 is considered a promising excitonic insulator (EI) candidate with slight phonon contributions, since it exhibits a tiny orthorhombic-to-monoclinic structural distortion at 328 K without any superlattice structure. Our synchrotron…

Inter-Coulombic decay (ICD) resonances in the photoionization of Cl@C60 endofullerene molecule are calculated using a perturbative density functional theory (DFT) method. This is the first ICD study of an open shell atom in a fullerene…

原子与分子团簇 · 物理学 2021-08-11 Ruma De , Esam Ali , Steven T. Manson , Himadri S. Chakraborty

The ionization of liquefied noble gases by radiation is known to be accompanied by fluctuations much larger than predicted by Poisson statistics. We have studied the fluctuations of both scintillation and ionization in liquid xenon and have…

We demonstrate strong interference patterns in the photoionization cross-section of the subvalent subshells of noble gas (NG) endohedral atoms NG@F. This interference is a result of common action of three factors: the effect of neighboring…

原子与分子团簇 · 物理学 2007-10-25 M. Ya. Amusia , A. S. Baltenkov , L. V. Chernysheva

We have investigated the electronic structures of newly discovered superconductor FeSe1-x by bulk-sensitive photoemission spectroscopy (PES). The large Fe 3d spectral weight is located in the vicinity of the Fermi level (EF) and it…

超导电性 · 物理学 2010-11-10 A. Yamasaki , S. Imada , K. Takase , T. Muro , Y. Kato , H. Kobori , A. Sugimura , N. Umeyama , H. Sato , Y. Hara , N. Miyakawa , S. I. Ikeda

We study the ground state structure and aspects of photoionization dynamics of the $Na_{20}@C_{240}$ endofullerene. The structure shows effects from the electronic coupling between the nested cluster and the fullerene cage. They include the…

原子与分子团簇 · 物理学 2024-12-20 Rasheed Shaik , Hari R. Varma , Mohamed El-Amine Madjet , Fulu Zheng , Himadri S. Chakraborty

Photoionization cross sections, photoelectron angular-asymmetry parameters and photoionization time delays for $A$@C$_{60}$ endohedral atoms are studied with account for both the individual and combined effects of dipole static polarization…

原子物理 · 物理学 2018-09-11 V. K. Dolmatov

Ultraintense pulses from X-ray free-electron lasers can drive, within femtoseconds, multiple processes in the inner shells of atoms and molecules in all phases of matter. The ensuing complex ionization pathways of outer-shell electrons from…

We use femtosecond resonant soft x-ray diffraction to measure the optically stimulated ultrafast changes of charge density wave correlations in underdoped YBa2Cu3O6.6. We find that when coherent interlayer transport is enhanced by optical…

A photofragmentation study of gas-phase indole (C$_8$H$_7$N) upon single-photon ionization at a photon energy of 420 eV is presented. Indole was primarily inner-shell ionized at its nitrogen and carbon $1s$ orbitals. Electrons and ions were…

A hole in a 4d orbital of atomic xenon relaxes through Auger decay after a lifetime of 3 fs. Adding electronegative fluorine ligands to form xenon fluoride molecules, results in withdrawal of valence-electron density from Xe. Thus, within…

化学物理 · 物理学 2008-02-23 Christian Buth , Robin Santra , Lorenz S. Cederbaum

We investigated CdTe nanocrystal tetrapods of different sizes by resonant inelastic light scattering at room temperature and under cryogenic conditions. We observe a strongly resonant behavior of the phonon scattering with the excitonic…

介观与纳米尺度物理 · 物理学 2007-05-23 R. Krahne , G. Chilla , C. Schueller , L. Carbone , S. Kudera , G. Mannarini , L. Manna , D. Heitmannb , R. Cingolani

It is demonstrated that in fullerene C70 which can be considered as a deformed fullerene C60 in some sense there is a withdrawal of an electrodynamical forbiddance of a strong quadrupole light-molecule interaction which is realized in the…

光学 · 物理学 2017-12-12 V. P. Chelibanov A. M. Polubotko

Effects of the interchannel coupling on the spin polarization of energetic photoelectrons emitted from atomic Ne valence subshells are examined. Like previously obtained results for cross sections and angular distributions, the…

原子物理 · 物理学 2021-06-08 Himadri S. Chakraborty , Pranawa C. Deshmukh , Steven T. Manson

We report on experimental and theoretical results for the photoionization of Ag-like xenon ions, Xe$^{7+}$, in the photon energy range 95 to 145~eV. The measurements were carried out at the Advanced Light Source at an energy resolution of…

Coherent resonance is the effect of resonant excitation of nonlinear coherent modes in trapped Bose condensates. This novel effect is shown to be feasible for Bose-condensed trapped gases. Conditions for realizing this effect are derived. A…

软凝聚态物质 · 物理学 2007-05-23 V. I. Yukalov , E. P. Yukalova , V. S. Bagnato

In this Letter, we investigate the time delay of photoelectrons by fullerenes shell in endohedrals. We present general formulas in the frame of the random phase approximation with exchange (RPAE) applied to endohedrals A@CN that consist of…

原子与分子团簇 · 物理学 2020-10-28 M. Ya. Amusia , L. V. Chernysheva

The Fe K X-ray absorption near edge structure (XANES) of BaFe2-xCoxAs2 superconductors was investigated. No appreciable alteration in shape or energy position of this edge was observed with Co substitution. This result provides experimental…