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Conversion of solar energy with high quantum efficiencies is a key challenge in energy technologies. Excitation energy transfer (EET) mechanisms, such as F\"orster resonance energy transfer (FRET), play a crucial role in facilitating…

Single molecule F\"orster resonance energy transfer (smFRET) is widely used to monitor conformations and interactions dynamics at the molecular level. However, conventional smFRET measurements are ineffective at donor-acceptor distances…

For many chemical processes the accurate description of solvent effects are vitally important. Here, we describe a hybrid ansatz for the explicit quantum mechanical description of solute-solvent and solvent-solvent interactions based on…

Fluorescence resonance energy transfer (FRET) from individual, dye-labeled RNA molecules confined in freely-diffusing attoliter-volume aqueous droplets is carefully compared to FRET from unconfined RNA in solution. The use of…

生物物理 · 物理学 2015-05-21 Sheema Rahmanseresht , Peker Milas , Kieran P. Ramos , Ben D. Gamari , Lori S. Goldner

F\"orster theory describes electronic exciton energy migration in molecular assemblies as an incoherent hopping process between donor and acceptor molecules. The rate is expressed in terms of the overlap integral between donor fluorescence…

化学物理 · 物理学 2018-10-17 Marco Schröter , Tõnu Pullerits , Oliver Kühn

By studying the lowest excitations of an exactly solvable one-dimensional molecular model, we show that components of Kohn-Sham ensembles can be used to describe charge transfers. Furthermore, we compute the approximate excitation energies…

化学物理 · 物理学 2018-05-22 Tim Gould , Leeor Kronik , Stefano Pittalis

F\"orster resonance energy transfer has an important role in nature and technology, rendering its exact theoretical understanding significant. To this end, a system of two electronically decoupled quantum dots (QDs) is considered,…

介观与纳米尺度物理 · 物理学 2025-09-22 Liubov S. Sirkina , Luke M. J. Hall , Amy Morreau , Wolfgang Langbein , Egor A. Muljarov

The stochastic model that describes radiative heat transfer in dielectric medium is built. The model is based on the representation that heat transfer is realized both by heat conductivity mechanism in it and due to the electromagnetic…

统计力学 · 物理学 2017-03-20 Yuri Petrovich Virchenko , Lam Tan Phat

Both spontaneous emission and resonant energy transfer can be enhanced significantly when the emitter is placed in the vicinity of metallic or crystal structures. This enhancement can be described using the electromagnetic Green tensor and…

光学 · 物理学 2022-07-27 Asaf Farhi , Aristide Dogariu

We study the nature of the energy transfer process within a pair of coupled two-level systems (donor and acceptor) subject to interactions with the surrounding environment. Going beyond a standard weak-coupling approach, we derive a master…

量子物理 · 物理学 2011-04-05 Dara P. S. McCutcheon , Ahsan Nazir

Using detailed balance and scaling properties of integrals that appear in the Coulomb gas reformulation of quantum impurity problems, we establish exact relations between the nonequilibrium transfer rates of the boundary sine-Gordon and the…

介观与纳米尺度物理 · 物理学 2009-11-10 Holger Baur , Andrea Fubini , Ulrich Weiss

We propose a scheme to simulate the exciton energy transfer (EET) of photosynthetic complexes in a quantum superconducting circuit system. Our system is composed of two pairs of superconducting charge qubits coupled to two separated high-Q…

量子物理 · 物理学 2020-08-28 Ming-Jie Tao , Ming Hua , Na-Na Zhang , Wan-Ting He , Qing Ai , Fu-Guo Deng

We derive equations of motion for the reduced density matrix of a molecular system which undergoes energy transfer dynamics competing with fast internal conversion channels. Environmental degrees of freedom of such a system have no time to…

化学物理 · 物理学 2017-05-24 Joachim Seibt , Tomas Mancal

In this theoretical study, we explore F\"orster resonant energy transfer of a single exciton within a two-dimensional array of self-assembled quantum dots arranged randomly on a circular mesa. Employing the stochastic simulation method, we…

介观与纳米尺度物理 · 物理学 2024-06-04 Karol Kawa , Paweł Machnikowski

Heat dissipation is ubiquitous in living systems, which constantly convert distinct forms of energy into each other. The transport of thermal energy in liquids and even within proteins is well understood but kinetic energy transfer across a…

软凝聚态物质 · 物理学 2026-01-07 Brandon Neff , Matthias Heyden

Underlying physical principles for the high efficiency of excitation energy transfer in light-harvesting complexes are not fully understood. Notably, the degree of robustness of these systems for transporting energy is not known considering…

量子物理 · 物理学 2015-03-19 Masoud Mohseni , Alireza Shabani , Seth Lloyd , Herschel Rabitz

A transfer-matrix formalism is introduced to evaluate exactly the partition function of the Munoz-Eaton model, relating the folding kinetics of proteins of known structure to their thermodynamics and topology. This technique can be used for…

统计力学 · 物理学 2009-11-07 Pierpaolo Bruscolini , Alessandro Pelizzola

We study the direct incoherent energy transfer from an immobile excited donor molecule to acceptor molecules, which are all attached to polymer chains, randomly arranged in a viscous solvent. The decay forms are found explicitly, in terms…

凝聚态物理 · 物理学 2008-02-03 G. Oshanin , J. De Coninck , A. Blumen , S. F. Burlatsky , M. Moreau

Excitation energy transfer (EET) in an organic/inorganic nanohybrid system, composed of a single \textit{para}-sexiphenyl (6P) molecule physisorbed on a finite-sized MoS$_2$ nanoflake, is investigated theoretically. % The electronic…

介观与纳米尺度物理 · 物理学 2026-01-22 Yan Meng , Kainan Chang , Luxia Wang

Heat, work and entropy production: the statistical distribution of such quantities are constrained by the fluctuation theorems (FT), which reveal crucial properties about the nature of non-equilibrium dynamics. In this paper we report…

量子物理 · 物理学 2021-10-15 K. Khan , J. Sales Araújo , W. F. Magalhães , G. H. Aguilar , B. de Lima Bernardo