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We present a methodology for simulating multi-dimensional electronic spectra of molecular aggregates with coupling of electronic excitation to a structured environment using the stochastic non-Markovian quantum state diffusion (NMQSD)…

量子物理 · 物理学 2022-09-28 Lipeng Chen , Doran I. G. Bennett , Alexander Eisfeld

Non-Markovian Quantum State Diffusion (NMQSD) has turned out to be an efficient method to calculate excitonic properties of aggregates composed of organic chromophores, taking into account the coupling of electronic transitions to…

Non-Markovian quantum state diffusion (NMQSD) is a non-relativistic but otherwise exact theory which expresses the reduced density matrix of an arbitrary subsystem, interacting linearly with an uncoupled harmonic oscillator bath, as an…

量子物理 · 物理学 2007-05-23 Joshua Wilkie , Ray Ng

Non-Markovian quantum state diffusion (NMQSD) is an exact method for calculating the reduced density matrix of an arbitrary subsystem interacting linearly with the radiation field. Applications of the theory have however been few due to the…

量子物理 · 物理学 2007-05-23 Joshua Wilkie , Ray Ng

We present a theory that efficiently describes the quantum dynamics of an electronic excitation that is coupled to a continuous, highly structured phonon environment. Based on a stochastic approach to non-Markovian open quantum systems, we…

量子物理 · 物理学 2009-11-05 Jan Roden , Alexander Eisfeld , Wolfgang Wolff , Walter T. Strunz

We investigate a quantum dot (QD) system coupled to a vibrational environment with a super-Ohmic spectral density and weakly to a leaky cavity mode, a model relevant for semiconductor-based single-photon sources. The phonon coupling induces…

介观与纳米尺度物理 · 物理学 2024-12-31 Sebastian Toivonen , Kimmo Luoma

Non-Markovian quantum state diffusion (NMQSD) provides a powerful approach to the dynamics of an open quantum system in bosonic environments. Here we develop an NMQSD method to study the open quantum system in fermionic environments. This…

量子物理 · 物理学 2015-06-04 Mi Chen , J. Q. You

A master equation, derived from the non-Markovian quantum state diffusion (NMQSD), is used to calculate excitation energy transfer in the photosynthetic Fenna-Matthews-Olson (FMO) pigment-protein complex at various temperatures. This…

量子物理 · 物理学 2012-02-07 G. Ritschel , J. Roden , W. T. Strunz , A. Eisfeld

We present a perturbation theory for non-Markovian quantum state diffusion (QSD), the theory of diffusive quantum trajectories for open systems in a bosonic environment [Physical Review {\bf A 58}, 1699, (1998)]. We establish a systematic…

量子物理 · 物理学 2016-08-15 Ting Yu , Lajos Diósi , Nicolas Gisin , Walter T. Strunz

Two perturbation methods for the non-Markovian quantum state diffusion (NMQSD) equation are investigated. The first perturbation method under investigation is based on a functional expansion of the NMQSD equation, while the second one…

量子物理 · 物理学 2014-10-30 Jie Xu , Xinyu Zhao , Jun Jing , Lian-Ao Wu , Ting Yu

Capturing non-Markovian dynamics of open quantum systems is generally a challenging problem, especially for strongly-interacting many-body systems. In this work, we combine recently developed non-Markovian quantum state diffusion techniques…

量子物理 · 物理学 2022-02-23 Stuart Flannigan , François Damanet , Andrew J. Daley

We introduce an exact open system method to describe the dynamics of quantum systems that are strongly coupled to specific types of environments comprising of spins, such as central spin systems. Our theory is similar to the established…

量子物理 · 物理学 2023-09-06 Valentin Link , Kimmo Luoma , Walter T. Strunz

In the microscopic modeling of new-generation electronic quantum nanodevices a variety of simulation strategies have been proposed and employed. Aim of this Letter is to point out virtues versus intrinsic limitations of non-Markovian…

介观与纳米尺度物理 · 物理学 2016-01-28 Rita Claudia Iotti , Fausto Rossi

Including the effect of the molecular environment in the numerical modeling of time-resolved electronic spectroscopy remains an important challenge in computational spectroscopy. In this contribution, we present a general approach for the…

量子物理 · 物理学 2024-12-17 Federico Gallina , Matteo Bruschi , Roberto Cacciari , Barbara Fresch

Non-Markovian dynamics is studied for two interacting quibts strongly coupled to a dissipative bosonic environment. For the first time, we have derived the non-Markovian quantum state diffusion (QSD) equation for the coupled two-qubit…

量子物理 · 物理学 2011-09-07 Xinyu Zhao , Jun Jing , Brittany Corn , Ting Yu

An accurate treatment of electronic spectra in large systems with a technique such as time dependent density functional theory (TDDFT) is computationally challenging. Due to the Nyquist sampling theorem, direct real time simulations must be…

材料科学 · 物理学 2024-01-17 Matthias Kick , Ezra Alexander , Anton Beiersdorfer , Troy Van Voorhis

Dissipative phase transitions in quantum systems have been largely studied under the so-called Markovian approximation, where the environments to which the systems are coupled are memoryless. Here, we present a generalization of the…

量子物理 · 物理学 2024-10-28 Baptiste Debecker , John Martin , François Damanet

A direct numerical algorithm for solving the time-nonlocal non-Markovian master equation in the second Born approximation is introduced and the range of utility of this approximation, and of the Markov approximation, is analyzed for the…

化学物理 · 物理学 2011-06-30 Navinder Singh , Paul Brumer

We discuss the absorption spectrum of dirty s-wave superconductors in the nonequilibrium steady state under a homogeneous and monochromatic microwave. In this state, there exists a finite density of states at lower energies than the…

超导电性 · 物理学 2023-06-28 Takanobu Jujo

The linear and the nonlinear non-Markovian quantum state diffusion equation (NMQSD) are well known tools for the description of certain non-Markovian open quantum systems. In this work, we systematically investigate whether the normalized…

量子物理 · 物理学 2012-09-03 Sven Krönke , Walter T. Strunz
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