相关论文: The Escape Rate of a Molecule
The change in the decay rate of an excited atom that is brought about by extinction and thermal-radiation effects in a nearby dielectric medium is determined from a quantummechanical model. The medium is a collection of randomly distributed…
A particle in the H\'enon-Heiles potential can escape when its energy is above the threshold value $E_{th}={1/6}$. We report a theoretical study on the the escape rates near threshold. We derived an analytic formula for the escape rate as a…
The narrow escape problem deals with the calculation of the mean escape time (MET) of a Brownian particle from a bounded domain through a small hole on the domain's boundary. Here we develop a formalism that allows us to evaluate the…
We have investigated the spontaneous decay rate of an excited molecule placed near a circular aperture in a metal film of finite thickness and finite conductivity. We have considered the metal film both suspended freely in vacuum and lying…
The time needed for a particle to exit a confining domain through a small window, called the narrow escape time (NET), is a limiting factor of various processes, such as some biochemical reactions in cells. Obtaining an estimate of the mean…
We consider the classical three-dimensional motion in a potential which is the sum of $n$ attracting or repelling Coulombic potentials. Assuming a non-collinear configuration of the $n$ centres, we find a universal behaviour for all…
We study the dynamics of an active Brownian particle with a nonlinear friction function located in a spatial cubic potential. For strong but finite damping, the escape rate of the particle over the spatial potential barrier shows a…
Quantum escape of a particle via a time-dependent confining potential in a semi-infinite one-dimensional space is discussed. We describe the time-evolution of escape states in terms of scattering states of the quantum open system, and…
Quantum escapes of a particle from an end of a one-dimensional finite region to $N$ number of semi-infinite leads are discussed by a scattering theoretical approach. Depending on a potential barrier amplitude at the junction, the…
We present the quantum master equation describing the coherent and incoherent dynamics of a rapidly rotating molecule in presence of a thermal background gas. The master equation relates the rate of rotational alignment decay and…
We study the escape rate of diffusion process with two approaches. We first give an upper rate function for the diffusion process associated with a symmetric, strongly local regular Dirichlet form. The upper rate function is in terms of the…
We study the escape rate of a particle in a metastable potential in presence of a dissipative bath coupled to the momentum of the particle. Using the semiclassical bounce technique, we find that this rate is exponentially enhanced. In…
We have studied numerically the quantum-classical crossover in the escape-rate for an uniaxial spin system with an arbitrarily directed field. Using the simple quantum transition-state theory, we have obtained the boundary separating the…
We investigate the absorption of diffusing molecules in a fluid-filled spherical beaker that contains many small reactive traps. The molecules are absorbed either by hitting a trap or by escaping via the beaker walls. In the physical…
Thermal escape out of a metastable well is considered in the weak friction regime, where the bottleneck for decay is energy diffusion, and at lower temperatures, where quantum tunneling becomes relevant. Within a systematic semiclassical…
Prompted by recent experimental developments, a theory of surface scattering of fast atoms at grazing incidence is developed. The theory gives rise to a quantum mechanical limit for ordered surfaces that describes coherent diffraction peaks…
The one-loop helicity amplitudes for the elastic scattering process $\gamma\nu\to\gamma\nu$ in the Standard Model are computed at high center of mass energies. A general decomposition of the amplitudes is utilized to investigate the…
The function of many membrane-enclosed intracellular structures relies on release of diffusing particles that exit through narrow pores or channels in the membrane. The rate of release varies with pore size, density, and length of the…
The time evolution of the thermally activated decay rates is considered. This evolution is of particular importance for the recent nanoscale experiments discussed in the literature, where the potential barrier is relatively low (or the…
We present classical trajectory calculations of the rotational vibrational scattering of a non-rigid methane molecule from a Ni(111) surface. Energy dissipation and scattering angles have been studied as a function of the translational…