相关论文: Intensity of Two-Photon Absorption Transitions for…
Two-photon excitation is an attractive means for controlling chemistry in both space and time. Isoenergetic one- and two-photon excitations (OPE and TPE) in non-centrosymmetric molecules are often assumed to reach the same excited state…
We study one-photon transitions between heavy baryon states in the framework of a relativistic three-quark model. We calculate the one-photon transition rates for ground-state to ground-state transitions and for some specific excited state…
Two-photon decay rates in simple atoms such as hydrogenlike systems represent rather interesting fundamental problems in atomic physics. The sum of the energies of the two emitted photons has to fulfill an energy conservation condition, the…
In a joint experimental and theoretical endeavour, photoionization of metastable C4+(1s 2s 3S1) ions via intermediate levels with hollow, double-K-vacancy configurations 2s2p, 2s3p, 2p3s, 2p3d, 2s4p, 2p4s and 2p4d has been investigated.…
The electronic structure of atomic quantum systems and their dynamical interaction with light is reflected in transition dipole matrix elements coupling the system's energy eigenstates. In this work, we measure phase shifts of the…
Two-photon absorption (TPA) and other nonlinear interactions of molecules with time-frequency-entangled photon pairs (EPP) has been predicted to display a variety of fascinating effects. Therefore, their potential use in practical…
Atomic negative ions are fragile quantum systems in which correlation among the valence electrons plays a very important role. For doubly excited states correlation becomes dominant. Photodetachment is the process where a negative ion…
Single and two-mode multiphoton states are the cornerstone of many quantum technologies, e.g., metrology. In the optical regime these states are generally obtained combining heralded single-photons with linear optics tools and…
It is well known that energy-time entanglement can enhance two photon absorption (TPA) by simultaneously optimizing the two photon resonance and the coincidence rate of photons at the absorber. However, the precise relation between…
It is known that ensembles of interacting oscillators or qubits can exhibit the phenomenon of quantum synchronization. In this work we consider a set of $N$ identical two-state systems that we call ``harmonic qubits'', because the kinetic…
In this contribution, we show that the use of conditional measurements in the resonant interaction of two quantized electromagnetic fields gives rise to nonclassical multiphoton processes. Furthermore, we demonstrate that this phenomenon…
We are the first to show with clear experimental results that photons that have energy lower than the transition energy between quantum dots states and valance band can still contribute greatly to the photocurrent via both one-photon…
The complete measurement of the quantum state of two correlated photons requires reconstructing the amplitude and phase of the biphoton wavefunction. We show how, by means of spatially resolved single photon detection, one can infer the…
The problem of the complete transfer of quantum states and entanglement in a four qubits system composed of two single-mode cavities and two two-level atoms is investigated. The transfer of single and double excitation states is discussed…
We demonstrate several building blocks for an ion-photon interface based on a trapped Ca ion in an optical cavity. We identify a favorable experimental configuration and measure system parameters, including relative motion of the trapped…
We present ultrafast transient absorption spectra of two oligofluorene derivatives in dilute solution. These spectra display clear vibronic structure, which we analyze rigorously using a time-dependent formalism of absorption to extract the…
We have studied the ground and excited state spectra of a semiconductor quantum dot for successive numbers of electron occupancy using linear and nonlinear magnetoconductance measurements. We present the first observation of direct…
Two-photon states are essential for quantum technologies such as metrology, lithography, and communication. One of the primary methods of two-photon generation is based on parametric down-conversion, but this suffers from low efficiency and…
Studying the excited states of doublets is challenging for their typically multiconfigurational character. We employ light-scanning-tunneling microscopy (light-STM) to investigate photon-induced currents on a single open-shell PTCDA anion…
The ground state of 2D electrons in high magnetic field is studied by the density matrix renormalization group method. The ground state energy, excitation gap, and pair correlation functions are systematically calculated at various fillings…