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Strontium clusters of size 2 to 20 atoms have been studied within the local density approximation using the ab-initio molecular dynamics method with a plane wave basis in which the s and p electron wavefunctions are well represented. The…

材料科学 · 物理学 2007-05-23 Tabish Qureshi , Vijay Kumar

The electronic structure is found to be understandable in terms of free-atom term values and universal interorbital coupling parameters, since self-consistent tight-binding calculations indicate that Coulomb shifts of the d-state energies…

材料科学 · 物理学 2009-11-13 Walter A. Harrison

We have located the global minimum for all lead clusters with up to 160 atoms using a glue potential to model the interatomic interactions. The lowest-energy structures are not face-centred cubic as suggested previously. Rather, for N<40…

凝聚态物理 · 物理学 2007-05-23 Jonathan P. K. Doye , Shaun C. Hendy

A stable core-shell structure with Ih symmetry, Au12@Au30, has been investigated by first-principles calculations. It is composed of an icosahedron core and an icosidodecahedron shell. The stability of the core-shell Au42 structure is…

材料科学 · 物理学 2021-06-29 Chunyuan Bai , Hongfei Li , Zun Xie , Yichen Dong , Shu Lan Liu

We present the first ab initio study of the geometry, electronic structure, charged states, bonding and vibrational modes of the recently synthesized fullerene-like As@Ni12@As20 cluster which has icosahedral point symmetry [Science, 300,…

材料科学 · 物理学 2009-11-10 Tunna Baruah , Rajendra R. Zope , Steven L. Richardson , Mark R. Pederson , ;

A local and medium range atomic structure model for the face centred icosahedral (fci) Mg25Y11Zn64 alloy has been established in a sphere of r = 27 A. The model was refined by least squares techniques using the atomic pair distribution…

材料科学 · 物理学 2007-05-23 S. Bruehne , E. Uhrig , C. Gross , W. Assmus , A. S. Masadeh , S. J. L. Billinge

There has long been a discrepancy between the size distributions of Ar$_n^+$ clusters measured by different groups regarding whether or not magic numbers appear at sizes corresponding to the closure of icosahedral (sub-)shells. We show that…

原子与分子团簇 · 物理学 2019-12-04 Michael Gatchell , Paul Martini , Lorenz Kranabetter , Bilal Rasul , Paul Scheier

The structural and bonding properties of small neutral alkali-halide clusters (AX)n, with n less than or equal to 10, A=Li, Na, K, Rb and X=F, Cl, Br, I, are studied using the ab initio Perturbed Ion (aiPI) model and a restricted structural…

原子与分子团簇 · 物理学 2009-10-30 A. Aguado , A. Ayuela , J. M. Lopez , J. A. Alonso

The crystal structure of the copper(II) tellurium(IV) oxochloride Cu$_{4}$Te$_{5}$O$_{12}$Cl$_{4}$ (Cu-45124) is composed of weakly coupled tetrahedral Cu clusters and shows crystallographic similarities with the intensively investigated…

We numerically study structural properties of mechanically stable packings of hard spheres (HS), in a wide range of packing fractions $0.53 \le \phi \le 0.72$. Detailed structural information is obtained from the analysis of orientational…

软凝聚态物质 · 物理学 2014-07-30 Boris A. Klumov , Yuliang Jin , Hernan A. Makse

The local nuclear and magnetic structure of wustite, Fe1-xO, and the coupling between them, has been examined using reverse Monte Carlo refinements of variable-temperature neutron total scattering data. The results from this analysis…

We carried out density functional calculation to study Co$_{13}$ clusters on graphene. We deposit several free isomers in different disposition respect to hexagonal lattice nodes, studying even the $hcp$ $2d$ isomer recently obtained as the…

材料科学 · 物理学 2015-12-25 Tomás Alonso-Lanza , Andrés Ayuela , Faustino Aguilera-Granja

Both even- and odd-numbered neutral carbon clusters Cn (n = 2-10) are systematically studied using the energy minimization method and the modified Brenner potential for the carbon-carbon interactions. Many stable configurations were found…

材料科学 · 物理学 2009-11-13 D. P. Kosimov , A. A. Dzhurakhalov , F. M. Peeters

Tight-binding molecular dynamics simulated annealing technique is employed to search for the ground state geometries of silicon clusters containing 11-17 atoms. These studies revealed that layer formation is the dominant growth pattern in…

chem-ph · 物理学 2009-10-28 Atul Bahel , Jun Pan , Mushti V. Ramakrishna

The structural and magnetic properties of Co$_{18-m}$Cu$_m$ ($0\leq m\leq 18$) clusters are investigated with a genetic algorithm and a $spd$-band model Hamiltonian in the unrestricted Hartree-Hock approximation respectively. In general, Cu…

原子与分子团簇 · 物理学 2007-05-23 Jinlan Wang , Guanghou Wang , Xiaoshuang Chen , Wei Lu , Jijun Zhao

Motivated by contradicting reports in the literature, we have investigated the structural stability of tungsten nanoparticles using density functional theory calculations. The comparison of BCC, FCC, A15, disordered, and icosahedral…

材料科学 · 物理学 2024-04-08 Laurent Pizzagalli , Sandrine Brochard , Julien Godet , Julien Durinck

We present structure calculations of neutral and singly ionized Mg clusters of up to 30 atoms, as well as Na clusters of up to 10 atoms. The calculations have been performed using density functional theory (DFT) within the local…

原子与分子团簇 · 物理学 2015-03-19 Stefan Janecek , Eckard Krotscheck , Michael Liebrecht , Roman Wahl

The thermal behaviour of the 309-atom Lennard-Jones cluster, whose structure is a complete Mackay icosahedron, has been studied by parallel tempering Monte Carlo simulations. Surprisingly for a magic number cluster, the heat capacity shows…

其他凝聚态物理 · 物理学 2007-05-23 Eva G. Noya , Jonathan P. K. Doye

The size-dependent electronic, structural, magnetic and vibrational properties of small pure cop- per and silver clusters and their alloys with one and two palladium atoms are studied by using full-potential all-electron density functional…

Shapes and energies of icosahedral fullerenes are studied on an atomically detailed level. The numerical results based on the effective binary carbon-carbon potential are related to the theory of elasticity of crystalline membranes with…

其他凝聚态物理 · 物理学 2007-05-23 A. Siber