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With the empirical bond polarizability model, the nonresonant Raman spectra of the chiral and achiral single-wall carbon nanotubes (SWCNTs) under uniaxial and torsional strains have been systematically studied by \textit{ab initio} method.…

介观与纳米尺度物理 · 物理学 2007-07-31 Gang Wu , Jian Zhou , Jinming Dong

Phonon softening phenomena of the $\Gamma$ point optical modes including the longitudinal optical mode, transverse optical mode and radial breathing mode in "metallic" single wall carbon nanotubes are reviewed from a theoretical point of…

介观与纳米尺度物理 · 物理学 2010-05-13 K. Sasaki , H. Farhat , R. Saito , M. S. Dresselhaus

A phonon frequency shift of the radial breathing mode for metallic single wall carbon nanotubes is predicted as a function of Fermi energy. Armchair nanotubes do not show any frequency shift while zigzag nanotubes exhibit phonon softening,…

介观与纳米尺度物理 · 物理学 2008-12-05 K. Sasaki , R. Saito , G. Dresselhaus , M. S. Dresselhaus , H. Farhat , J. Kong

We have used a femtosecond pump-probe impulsive Raman technique to explore the ultrafast dynamics of micelle suspended single walled carbon nanotubes (SWNTs) in various pH environments. The structures of coherent phonon spectra of the…

介观与纳米尺度物理 · 物理学 2010-11-17 Kotaro Makino , Atsushi Hirano , Kentaro Shiraki , Yutaka Maeda , Muneaki Hase

In this study, we performed comprehensive investigations on the Raman active phonon modes in cubic bixbyite In$_2$O$_3$, an important oxide based, wide-bandgap semiconductor. Fundamental insights into the lattice dynamics are revealed, by…

We review recent studies of coherent phonons (CPs) corresponding to the radial breathing mode (RBM) and G-mode in single-wall carbon nanotubes (SWCNTs) and graphene. Because of the bandgap-diameter relationship, RBM-CPs cause bandgap…

介观与纳米尺度物理 · 物理学 2013-03-28 J. -H. Kim , A. R. T. Nugraha , L. G. Booshehri , E. H. Hároz , K. Sato , G. D. Sanders , K. -J. Yee , Y. -S. Lim , C. J. Stanton , R. Saito , J. Kono

Coherent phonons in single wall carbon nanotubes (SWNTs) are observed as oscillations of the differential absorption coefficient as a function of time by means of pump-probe spectroscopy. For the radial breathing mode (RBM) of a SWNT, the…

介观与纳米尺度物理 · 物理学 2015-06-22 A. R. T. Nugraha , E. H. Hasdeo , G. D. Sanders , C. J. Stanton , R. Saito

Raman spectroscopy is used to probe the structure and electronic properties of nanotubes dispersed in a liquid phase. We show that the radial breathing modes are upshifted in suspensions due to the molecular pressure of the solvent. On the…

其他凝聚态物理 · 物理学 2016-08-16 Nicolas Izard , Alain Pénicaud , Eric Anglaret

We have studied the coherent dynamics of G-band phonons in single-walled carbon nanotubes through impulsive stimulated Stokes and anti-Stokes Raman scattering. The probe energy dependence of phonon amplitude as well as preferential…

介观与纳米尺度物理 · 物理学 2012-11-13 J. -H. Kim , K. -J. Yee , Y. -S. Lim , L. G. Booshehri , E. H. Haroz , J. Kono

We investigate vibration modes and their Raman activity of single-walled carbon nanotubes that are bent within their intrinsic elastic limits. By implementing novel boundary conditions for density-functional based tight-binding, and using…

材料科学 · 物理学 2009-11-13 Sami Malola , Hannu Häkkinen , Pekka Koskinen

Using the molecular dynamics simulations and the force constant model we have studied the Raman-active tangential modes (TMs) of a (10, 0) single-wall carbon nanotube (SWNT) under hydrostatic pressure. With increasing pressure, the atomic…

介观与纳米尺度物理 · 物理学 2009-11-13 Wei Yang , Ru-Zhi Wang , Yu-Fang Wang , Xue-Mei Song , Bo Wang , Hui Yan

Raman spectra and electrical conductance of individual, pristine, suspended, metallic single-walled carbon nanotubes are measured under applied gate potentials. The G- band is observed to downshift with small applied gate voltages, with the…

介观与纳米尺度物理 · 物理学 2015-05-13 Adam W. Bushmaker , Vikram V. Deshpande , Scott Hsieh , Marc W. Bockrath , Stephen B. Cronin

We present a first-principles study on lattice vibrational modes of Si/Ge core-shell nanowires (NWs). In addition to quantum confinement, the internal strain induced by the lattice mismatch between core and shell contributes to significant…

介观与纳米尺度物理 · 物理学 2012-07-04 Shouting Huang , Li Yang

The tangential G-band in the Raman spectra of a metallic single-wall carbon nanotube shows two peaks: a higher frequency component having the Lorentzian shape and a lower-frequency component of lower intensity with a Breit-Wigner-Fano…

其他凝聚态物理 · 物理学 2009-11-11 S. M. Bose , S. Gayen , S. N. Behera

In this paper, we investigate the low frequency Raman spectra of multi-wall carbon nanotubes (MWNT) prepared by the electric arc method. Low frequency Raman modes are unambiguously identified on purified samples thanks to the small internal…

介观与纳米尺度物理 · 物理学 2009-11-07 J. M. Benoit , J. P. Buisson , O. Chauvet , C. Godon , S. Lefrant

Large variations of up to two orders of magnitude are observed in the Raman intensity of pristine, suspended quasi-metallic single-walled carbon nanotubes in response to applied gate potentials. No change in the resonance condition is…

介观与纳米尺度物理 · 物理学 2009-05-07 Adam W. Bushmaker , Vikram V. Deshpande , Scott Hsieh , Marc W. Bockrath , Stephen B. Cronin

The radial-breathing-like phonon modes (RBLMs) of the double-walled carbon nanotubes are studied in a simple analytical model, in which the interaction force constants (FCs) can be obtained analytically from the continuous model. The RBLMs…

介观与纳米尺度物理 · 物理学 2007-07-31 Gang Wu , Jian Zhou , Jinming Dong

We report the existence of broad and weakly asymmetric features in the high-energy (G) Raman modes of freely suspended metallic carbon nanotubes of defined chiral index. A significant variation in peak width (from 12 cm-1 to 110 cm-1) is…

We develop a continuous theory of low-frequency dynamics for nanotubes with truly two-dimensional (2D) walls constituted by single-atom monolayer. In this frame topological bending elasticity of the monolayer is not related to its vanishing…

材料科学 · 物理学 2015-06-16 S. B. Rochal , V. L. Lorman , Yu. I. Yuzyuk

The Raman spectra of two G-bands and a radial breathing mode (RBM) of unfilled and filled single-wall semiconducting and metallic carbon nanotubes have been investigated theoretically, in the presence of electron-phonon and phonon-phonon…

其他凝聚态物理 · 物理学 2009-11-13 S. Gayen , S. N. Behera , S. M. Bose
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