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Recent theoretical predictions and experimental measurements have demonstrated that equilibrium free energy differences can be obtained from exponential averages of nonequilibrium work values. These results are similar in structure, but not…

统计力学 · 物理学 2009-11-11 Christopher Jarzynski

The Jarzynski relation is a recently discovered result relating the average exponential of the work done under nonequilibrium conditions to an equilibrium free energy difference. We illustrate this remarkable relation by considering the…

统计力学 · 物理学 2007-05-23 Rhonald C. Lua

We suggest and discuss a simple model of an ideal gas under the piston to gain an insight into the workings of the Jarzynski identity connecting the average exponential of the work over the non-equilibrium trajectories with the equilibrium…

统计力学 · 物理学 2007-05-23 R. C. Lua , A. Y. Grosberg

Exponential averages that appear in integral fluctuation theorems can be recast as a sum over moments of thermodynamic observables. We use two examples to show that such moment series can exhibit non-uniform convergence in certain singular…

统计力学 · 物理学 2022-05-31 Hila Katznelson , Saar Rahav

A central endeavor of thermodynamics is the measurement of free energy changes. Regrettably, although we can measure the free energy of a system in thermodynamic equilibrium, typically all we can say about the free energy of a…

统计力学 · 物理学 2012-04-10 David A. Sivak , Gavin E. Crooks

The objective of the present paper is to establish exponential large deviation inequalities, and to use them to show exponential concentration inequalities for the free energy of a polymer in general random environment, its rate of…

概率论 · 数学 2009-09-11 Quansheng Liu , Frédérique Watbled

An expression is derived for the classical free energy difference between two configurations of a system, in terms of an ensemble of finite-time measurements of the work performed in parametrically switching from one configuration to the…

统计力学 · 物理学 2009-10-28 C. Jarzynski

We investigate extreme value theory for physical systems with a global conservation law which describe renewal processes, mass transport models and long-range interacting spin models. As shown previously, a special feature is that the…

统计力学 · 物理学 2020-11-04 Marc Höll , Wanli Wang , Eli Barkai

We study two different forms of fluctuation-dissipation processes generating anomalous relaxations to equilibrium of an initial out of equilibrium condition, the former being based on a stationary although very slow correlation function and…

数据分析、统计与概率 · 物理学 2017-10-18 Rohisha Tuladhar , Mauro Bologna , Paolo Grigolini

Calculating free energy differences is a topic of substantial interest and has many applications including molecular docking and hydration, solvation, and binding free energies which is used in computational drug discovery. However, in…

化学物理 · 物理学 2013-10-16 Asaf Farhi

Rare events refer to qualitatively unlikely events whose realization can nevertheless have important consequences. Typically, the prediction of the kinetics of these events relies on Arrhenius laws, with exponentially distributed waiting…

统计力学 · 物理学 2025-12-18 Apurba Biswas , Thomas Guérin

The transition between a regime in which thermodynamic relations apply only to ensembles of small systems coupled to a large environment and a regime in which they can be used to characterize individual macroscopic systems is analyzed in…

统计力学 · 物理学 2015-05-30 Alberto Suárez , Robert Silbey , Irwin Oppenheim

Rare events can potentially occur in many applications. When manifested as opportunities to be exploited, risks to be ameliorated, or certain features to be extracted, such events become of paramount significance. Due to their sporadic…

信息论 · 计算机科学 2012-10-10 Ali Tajer , H. Vincent Poor

We consider an ordinary differential equation with a unique hyperbolic attractor at the origin, to which we add a small random perturbation. It is known that under general conditions, the solution of this stochastic differential equation…

概率论 · 数学 2023-05-05 Gerardo Barrera , Milton Jara

The object of this paper is twofold. From one side we study the dichotomy, in terms of the Extremal Index of the possible Extreme Value Laws, when the rare events are centred around periodic or non periodic points. Then we build a general…

动力系统 · 数学 2016-03-24 Hale Aytaç , Jorge Milhazes Freitas , Sandro Vaienti

The Jarzynski equality is one of the most influential results in the field of non equilibrium statistical mechanics. This celebrated equality allows to calculate equilibrium free energy differences from work distributions of nonequilibrium…

统计力学 · 物理学 2017-09-13 Shahaf Asban , Saar Rahav

The relativistic Maxwell-Boltzmann distribution for the system of $N$ events with motion in space-time parametrized by an invariant ``historical time'' $\tau $ is considered without the simplifying approximation $m^2\cong M^2$, where $M$ is…

高能物理 - 唯象学 · 物理学 2009-10-22 L. Burakovsky , L. P. Horwitz

We show that the dynamics of simple disordered models, like the directed Trap Model and the Random Energy Model, takes place at a coexistence point between active and inactive dynamical phases. We relate the presence of a dynamic phase…

统计力学 · 物理学 2008-09-03 Kristina Van Duijvendijk , Grégory Schehr , Frédéric Van Wijland

Power law or generalized polynomial regressions with unknown real-valued exponents and coefficients, and weakly dependent errors, are considered for observations over time, space or space--time. Consistency and asymptotic normality of…

统计理论 · 数学 2012-05-14 Peter M. Robinson

The efficient calculation of rare-event kinetics in complex dynamical systems, such as the rate and pathways of ligand dissociation from a protein, is a generally unsolved problem. Markov state models can systematically integrate ensembles…

化学物理 · 物理学 2016-02-03 Benjamin Trendelkamp-Schroer , Frank Noe
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