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We investigate transport through a mononuclear transition-metal complex with strong tunnel coupling to two electrodes. The ground state of this molecule is a singlet while the first excited state is a triplet. We show that a modulation of…

强关联电子 · 物理学 2007-05-23 K. Kikoin , M. N. Kiselev , M. R. Wegewijs

The low-temperature transport properties of a molecule are studied in the field-effect transitor geometry. The molecule has an internal mechanical mode that modulates its electronic levels and renormalizes both the interactions and the…

强关联电子 · 物理学 2008-01-23 P. S. Cornaglia , Gonzalo Usaj , C. A. Balseiro

Here we present a theoretical analysis of inelastic effects on thermoelectric properties of molecular-scale junction in both linear and nonlinear response regimes. Considered device is composed of molecular quantum dot (with discrete energy…

介观与纳米尺度物理 · 物理学 2015-06-25 Kamil Walczak

A time-dependent approach is used to explore inelastic effects during electron transport through few-level systems. We study a tight-binding chain with one and two sites connected to vibrations. This simple but transparent model gives…

介观与纳米尺度物理 · 物理学 2009-11-13 S. Monturet , N. Lorente

We study inelastic electron tunneling through a molecular junction using the non-equilibrium Green function (NEGF) formalism. The effect of the mutual influence between the phonon and the electron subsystems on the electron tunneling…

介观与纳米尺度物理 · 物理学 2009-11-10 Michael Galperin , Mark A. Ratner , Abraham Nitzan

Transistors, regardless of their size, rely on electrical gates to control the conductance between source and drain contacts. In atomic-scale transistors, this conductance is exquisitely sensitive to single electrons hopping via individual…

A theoretical analysis of inelastic electron tunneling spectroscopy (IETS) experiments conducted on molecular junctions are presented, where the second derivative of the current with respect to voltage is usually plotted as a function of…

介观与纳米尺度物理 · 物理学 2009-11-13 Kamil Walczak

Quantum transport through single molecules is essentially affected by molecular vibrations. We investigate the behavior of the prototype single-level model with intermediate electron-vibron coupling and arbitrary coupling to the leads. We…

介观与纳米尺度物理 · 物理学 2009-11-13 Dmitry A. Ryndyk , Gianaurelio Cuniberti

Magnetic inelastic electron tunneling spectroscopy (IETS) shows sharp increases in conductance when a new conductance channel associated to a change in magnetic structure is open. Typically, the magnetic moment carried by an adsorbate can…

介观与纳米尺度物理 · 物理学 2012-06-19 Richard Korytár , Nicolás Lorente , Jean-Pierre Gauyacq

We theoretically analyzed inelastic effects in the electron transport through molecular junctions originating from electron-vibron interactions. The molecular bridge was simulated by a periodic chain of identical interacting hydrogen-like…

材料科学 · 物理学 2010-01-03 Natalya A. Zimbovskaya , Maija M. Kuklja

Vibrational modes of molecules are fundamental properties determined by intramolecular bonding, atomic masses, and molecular geometry, and often serve as important channels for dissipation in nanoscale processes. Although single-molecule…

介观与纳米尺度物理 · 物理学 2014-03-06 Y. Li , P. Doak , L. Kronik , J. B. Neaton , D. Natelson

The effect of electron-phonon coupling on the current noise in a molecular junction is investigated within a simple model. The model comprises a 1-level bridge representing a molecular level that connects between two free electron…

介观与纳米尺度物理 · 物理学 2007-05-23 Michael Galperin , Abraham Nitzan , Mark A. Ratner

Access to magnetic excitation spectra of single atoms deposited on surfaces is nowadays possible by means of low-temperature inelastic scanning tunneling spectroscopy. We present a first-principles method for the calculation of inelastic…

强关联电子 · 物理学 2015-06-22 Benedikt Schweflinghaus , Manuel dos Santos Dias , Antonio T. Costa , Samir Lounis

The evolution of electron conductance in the presence of inelastic effects is studied as an atomic gold contact is formed evolving from a low-conductance regime (tunneling) to a high-conductance regime (contact). In order to characterize…

介观与纳米尺度物理 · 物理学 2007-06-25 Thomas Frederiksen , Nicolas Lorente , Magnus Paulsson , Mads Brandbyge

Tunneling spectroscopy is applied to tunnel junctions with only one or no ferromagnetic electrode to study the excitation of quasi particles in magnetic tunnel junctions. The bias dependence is investigated with high accuracy by inelastic…

材料科学 · 物理学 2010-08-03 Volker Drewello , Zoë Kugler , Günter Reiss , Andy Thomas

The appealing feature of molecular electronics is the possibility of exploiting functionality built within a single molecule. This functionality can be employed, for example, for sensing or switching purposes. Thus, ideally, the associated…

We have carried out a computational study of the inelastic electron tunneling spectrum (IETS) of the two vibrational modes of a single hydrogen atom on a Cu(100) surface in a scanning tunneling microscopy (STM) junction. This study…

材料科学 · 物理学 2007-05-23 Sami Paavilainen , Mats Persson

Recent advances in on-surface chemistry, combined with scanning probe microscopy, have enabled the synthesis of correlated molecules on surfaces and the characterization of their chemical and electronic properties with unprecedented spatial…

介观与纳米尺度物理 · 物理学 2026-03-25 Marco Lozano , Manish Kumar , Pavel Jelinek , Diego Soler-Polo

Molecular systems can exhibit a complex, chemically tailorable inner structure which allows for targeting of specific mechanical, electronic and optical properties. At the single-molecule level, two major complementary ways to explore these…

介观与纳米尺度物理 · 物理学 2017-04-05 Rocco Gaudenzi , Maciej Misiorny , Enrique Burzurí , Maarten R. Wegewijs , Herre S. J. van der Zant

We address quantum invisibility in the context of electronics in nanoscale quantum structures. We make use of the freedom of design that quantum corrals provide and show that quantum mechanical objects can be hidden inside the corral, with…

介观与纳米尺度物理 · 物理学 2010-05-18 J. Fransson , H. C. Manoharan , A. V. Balatsky