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We theoretically study the transport properties of a supramolecular spin valve, consisting of a carbon nanotube with two attached magnetic molecules, weakly coupled to metallic contacts. The emphasis is put on analyzing the change of the…

介观与纳米尺度物理 · 物理学 2019-03-19 A. Plominska , I. Weymann

We explore theoretically the scanning tunneling microscopy of single molecules on substrates using a framework of two local probes. This framework is appropriate for studying electron flow in tip/molecule/substrate systems where a thin…

介观与纳米尺度物理 · 物理学 2016-08-31 John Buker , George Kirczenow

We theoretically show how the spin orientation of a single magnetic adatom can be controlled by spin polarized electrons in a scanning tunneling microscope configuration. The underlying physical mechanism is spin assisted inelastic…

介观与纳米尺度物理 · 物理学 2010-03-11 F. Delgado , J. J. Palacios , J. Fernandez-Rossier

We demonstrate a device geometry for single-molecule electronics experiments that combines both the ability to adjust the spacing between the electrodes mechanically and the ability to shift the energy levels in the molecule using a gate…

介观与纳米尺度物理 · 物理学 2015-06-24 A. R. Champagne , A. N. Pasupathy , D. C. Ralph

A key to building functional devices on the basis of single molecule magnets in the framework of molecular electronics is the ability to deposit and study these molecules on a surface, because the structural, electronic and magnetic…

介观与纳米尺度物理 · 物理学 2016-01-26 Judith Donner , Jan-Philipp Broschinski , Bastian Feldscher , Anja Stammler , Hartmut Bögge , Thorsten Glaser , Daniel Wegner

The interplay between discrete vibrational and electronic degrees of freedom directly influences the chemical and physical properties of molecular systems. This coupling is typically studied through optical methods such as fluorescence,…

介观与纳米尺度物理 · 物理学 2007-05-23 B. J. LeRoy , S. G. Lemay , J. Kong , C. Dekker

We present a new semi-empirical model for calculating electron transport in atomic-scale devices. The model is an extension of the Extended H\"uckel method with a self-consistent Hartree potential. This potential models the effect of an…

介观与纳米尺度物理 · 物理学 2012-04-04 Kurt Stokbro , Dan Erik Petersen , Søren Smidstrup , Anders Blom , Mads Ipsen , Kristen Kaasbjerg

We theoretically analyzed inelastic effects in the electron transport through molecular junctions originating from electron-vibron interactions. The molecular bridge was simulated by a periodic chain of identical interacting hydrogen-like…

材料科学 · 物理学 2010-01-03 Natalya A. Zimbovskaya , Maija M. Kuklja

We investigate electronic transport through two types of conjugated molecules. Mechanically controlled break-junctions are used to couple thiol endgroups of single molecules to two gold electrodes. Current-voltage characteristics (IVs) of…

介观与纳米尺度物理 · 物理学 2009-11-07 J. Reichert , R. Ochs , D. Beckmann , H. B. Weber , M. Mayor , H. v. Loehneysen

Tunneling of single electrons has been thoroughly studied both theoretically and experimentally during last ten years. By the present time the basic physics is well understood, and creation of useful single-electron devices becomes the…

凝聚态物理 · 物理学 2007-05-23 Alexander N. Korotkov

We have fabricated hybrid magnetic complexes from V atoms and tetracyanoethylene (TCNE) ligands via atomic manipulation with a cryogenic scanning tunneling microscope. Using tunneling spectroscopy we observe spin-polarized molecular…

Predictions state that graphene can spontaneously develop magnetism from the Coulomb repulsion of its $\pi$-electrons, but its experimental verification has been a challenge. Here, we report on the observation and manipulation of individual…

介观与纳米尺度物理 · 物理学 2019-01-15 Jingcheng Li , Sofia Sanz , Martina Corso , Deung Jang Choi , Diego Peña , Thomas Frederiksen , Jose Ignacio Pascual

We show that in the presence of ferromagnetic electronic reservoirs and spin-dependent tunnel couplings, molecular vibrations in nonmagnetic single molecular transistors induce an effective intramolecular exchange magnetic field. It…

介观与纳米尺度物理 · 物理学 2015-07-29 S. Weiss , J. Brüggemann , M. Thorwart

The process of creating an atomically defined and robust metallic tip is described and quantified using measurements of contact conductance between gold electrodes and numerical simulations. Our experiments show how the same conductance…

材料科学 · 物理学 2012-05-30 C. Sabater , C. Untiedt , J. J. Palacios , M. J. Caturla

Magnetic switching of a single molecular magnet (SMM) due to spin-polarized current flowing between ferromagnetic metallic electrodes is investigated theoretically. Magnetic moments of the electrodes are assumed to be collinear and parallel…

介观与纳米尺度物理 · 物理学 2016-08-16 Maciej Misiorny , Józef Barnas

The presence of spin-orbit scattering within an aluminum nanoparticle affects measurements of the discrete energy levels within the particle by (1) reducing the effective g-factor below the free-electron value of 2, (2) causing avoided…

介观与纳米尺度物理 · 物理学 2009-10-31 D. G. Salinas , S. Guéron , D. C. Ralph , C. T. Black , M. Tinkham

The electronic and vibrational density of states of a semiconducting carbon nanotube in a crossed junction was investigated by elastic and inelastic scanning tunneling spectroscopy. The strong radial compression of the nanotube at the…

材料科学 · 物理学 2009-11-11 L. Vitali , M. Burghard , P. Wahl , M. A. Schneider , K. Kern

A single-electron transistor incorporated as part of a nanomechanical resonator represents an extreme limit of electron-phonon coupling. While it allows for fast and sensitive electromechanical measurements, it also introduces backaction…

介观与纳米尺度物理 · 物理学 2020-07-01 Yutian Wen , N. Ares , F. J. Schupp , T. Pei , G. A. D. Briggs , E. A. Laird

We study the transmission through single and double ferromagnetic barriers on the surface of a topological insulator. By adjusting the gate voltage and magnetization oreintation, the ferromagnetic barrier can be tuned into various…

介观与纳米尺度物理 · 物理学 2009-09-03 Jinhua Gao , Wei-Qiang Chen , Xiao-Yong Feng , X. C. Xie , Fu-Chun Zhang

We report on the single-molecule electronic and thermoelectric properties of strategically chosen anthracene-based molecules with anchor groups capable of binding to noble metal substrates, such as gold and platinum. Specifically, we study…