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We report on electrical Raman measurements in transparent and conducting single-wall carbon nanotube (SWNT) thin films. Application of external electric field results in downshifts of the D and G modes and in reduction of their intensity.…

材料科学 · 物理学 2015-06-25 Giovanni Fanchini , Husnu Emrah Unalan , Manish Chhowalla

We show by ab initio calculations that the electron-phonon coupling matrix element M of the radial breathing mode in single-walled carbon nanotubes depends strongly on tube chirality. For nanotubes of the same diameter the coupling strength…

材料科学 · 物理学 2009-11-10 M. Machon , S. Reich , H. Telg , J. Maultzsch , P. Ordejon , C. Thomsen

Hyper-Raman scattering has been measured on vitreous boron oxide, $v-$B$_2$O$_3$. This spectroscopy, complemented with Raman scattering and infrared absorption, reveals the full set of vibrations that can be observed with light. A mode…

无序系统与神经网络 · 物理学 2009-11-13 G. Simon , B. Hehlen , R. Vacher , E. Courtens

Molecular vibrations and their dynamics are of outstanding importance for electronic and thermal transport in nanoscale devices as well as for molecular catalysis. The vibrational dynamics of <100 molecules are studied through three-colour…

The appearance of a broad peak at $\sim$1550 cm$^{-1}$ (G$^{-}$ peak) in carbon nanotube resonant Raman scattering spectra has been conventionally attributed to the presence of metallic nanotubes. Here, we present resonant Raman…

介观与纳米尺度物理 · 物理学 2015-05-20 E. H. Haroz , J. G. Duque , W. D. Rice , C. G. Densmore , J. Kono , S. K. Doorn

We have studied polarized Raman spectra of (TMTSF)2PF6 single crystals in the wide spectral and temperature range using different laser energies. We observed and assigned 23 Raman active modes. The carbon C=C in-phase and out-of-phase…

强关联电子 · 物理学 2007-05-23 Z. V. Popovic , V. A. Ivanov , O. P. Khoung , T. Nakamura , G. Saito , V. V. Moshchalkov

The symmetry group analysis is applied to classify the phonon modes of $N$-stacked graphene layers (NSGL's) with AB- and AA-stacking, particularly their infra-red and Raman properties. The dispersions of various phonon modes are calculated…

材料科学 · 物理学 2008-06-30 Jin-Wu Jiang , Hui Tang , Bing-Shen Wang , Zhao-Bin Su

We present it ab-initio calculations of the non-resonant Raman spectra of zigzag and armchair BN nanotubes. In comparison, we implement a generalized bond-polarizability model where the parameters are extracted from first-principles…

材料科学 · 物理学 2013-08-07 Ludger Wirtz , Michele Lazzeri , Francesco Mauri , Angel Rubio

Vibrational properties of graphene nanoribbons are examined with density functional based tight-binding method and non-resonant bond polarization theory. We show that the recently discovered reconstructed zigzag edge can be identified from…

材料科学 · 物理学 2009-11-13 S. Malola , H. Häkkinen , P. Koskinen

We have generated and detected the radial-breathing mode of coherent lattice vibrations in single-walled carbon nanotubes using ultrashort laser pulses. Because the band gap is a function of diameter, these diameter oscillations cause…

介观与纳米尺度物理 · 物理学 2015-06-25 Y. S. Lim , K. J. Yee , J. H. Kim , J. Shaver , E. H. Haroz , J. Kono , S. K. Doorn , R. H. Hauge , R. E. Smalley

We report experimental studies of spin-wave excitations in individual 22 nm thick Ni80Fe20 nanotubes with diameters of about 150 nm by means of Brillouin light-scattering (BLS) spectroscopy. Irradiated by microwaves we resolve sets of…

介观与纳米尺度物理 · 物理学 2022-04-28 Maria Carmen Giordano , Mohammad Hamdi , Andrea Mucchietto , Dirk Grundler

A new numerical method is introduced for calculating the polarizability of an arbitrary dielectric object with position dependent complex permittivity. Three separate numerical approaches are provided to calculate the dipole moment of a…

材料科学 · 物理学 2022-03-18 Daniel B. Murray , Caleb H. Netting , Robin D. Mercer , Lucien Saviot

We investigated the atomic structures, Raman spectroscopic and electrical transport properties of individual graphene nanoribbons (GNRs, widths ~10-30 nm) derived from sonochemical unzipping of multi-walled carbon nanotubes (MWNTs).…

材料科学 · 物理学 2011-06-21 Liming Xie , Hailiang Wang , Chuanhong Jin , Xinran Wang , Liying Jiao , Kazu Suenaga , Hongjie Dai

The analysis of the Raman scattering cross section of the radial breathing modes of double-wall carbon nanotubes allowed to determine the optical transitions of the inner tubes. The Raman lines are found to cluster into species with similar…

软凝聚态物质 · 物理学 2007-05-23 R. Pfeiffer , F. Simon , H. Kuzmany , V. N. Popov

We report the existence of broad and weakly asymmetric features in the high-energy (G) Raman modes of freely suspended metallic carbon nanotubes of defined chiral index. A significant variation in peak width (from 12 cm-1 to 110 cm-1) is…

Various properties of the energy band structures (electronic, phonon, etc.), including systematic band degeneracy, sticking and extremes, following from the full line group symmetry of the single-wall carbon nanotubes are established. The…

介观与纳米尺度物理 · 物理学 2009-11-07 T. Vukovic , I. Milosevic , M. Damnjanovic

We investigate the vibrational and magnetic properties of thin layers of chromium tribromide (CrBr$_3$) with a thickness ranging from three to twenty layers (3~L to 20~L) revealed by the Raman scattering (RS) technique. Systematic…

Amorphous carbon nanotubes (a-CNT) with up to four walls and sizes ranging from 200 to 3200 atoms have been simulated, starting from initial random configurations and using the Gaussian Approximation Potential [Phys. Rev. B 95, 094203…

材料科学 · 物理学 2023-03-22 C. Ugwumadu , R. Thapa , Y. Al-Majali , J. Trembly , D. A. Drabold

Raman spectroscopy is used to probe the structure and electronic properties of nanotubes dispersed in a liquid phase. We show that the radial breathing modes are upshifted in suspensions due to the molecular pressure of the solvent. On the…

其他凝聚态物理 · 物理学 2016-08-16 Nicolas Izard , Alain Pénicaud , Eric Anglaret

For molecules and materials responding to femtosecond-scale optical laser pulses, we predict maximum relative excitation of a Raman-active vibrational mode with period T when the pulse has an FWHM duration of 0.42 T. This result follows…

介观与纳米尺度物理 · 物理学 2015-05-14 Xiang Zhou , Zhibin Lin , Chenwei Jiang , Meng Gao , Roland E. Allen