相关论文: Excited states of linear polyenes

High precision (p,t) studies of the deformed nucleus 158Gd allowed the observation of 13 excited 0+ states below an excitation energy of 3.1 MeV. This high density of low energy states, and particularly their measured B(E2) transition…

Owing to ring-strain, cyclic ketones exhibit complex excited-state dynamics with multiple competing photochemical channels active on the ultrafast timescale. While the excited-state dynamics of cyclobutanone after $\pi^{\ast}\leftarrow n$…

The interaction between aligned dipoles is long-ranged and highly anisotropic: it changes from repulsive to attractive depending on the relative positions of the dipoles. We report on the observation of the attractive component of the…

Studying the excited states of doublets is challenging for their typically multiconfigurational character. We employ light-scanning-tunneling microscopy (light-STM) to investigate photon-induced currents on a single open-shell PTCDA anion…

Competition between polaron and bipolaron inconjugated polymers with nondegenerate ground state is systematically studied in the extended Hubbard-Peierls model with the symmetry-breaking Brazovskii-Kirova term, using the density matrix…

A microscopic approach is developed to determine the excitation energetics of highly correlated quasi-particles in optically excited semiconductors based entirely on a pair-correlation function input. For this purpose, the Wannier equation…

We find that the excitation energies of single analog states for odd-even nuclei in the f$_{7/2}$ shell with J=j=7/2$^{-}$ and the J=0$^{+}$ double analog states in the even-even nuclei are well described by the formulas $E^{*}(j,T+1) = b…

The nature may be disclosed that the glass transition is only determined by the intrinsic 8 orders of instant 2-D mosaic geometric structures, without any presupposition and relevant parameter. An interface excited state on the geometric…

The ground state energy of the two--dimensional uniform electron gas has been calculated with fixed--node diffusion Monte Carlo, including backflow correlations, for a wide range of electron densities as a function of spin polarization. We…

We introduce 1D and 2D models of a degenerate bosonic gas composed of ions with positive and negative charges (cations and anions). The system may exist in the mean-field condensate state, enabling the competition of the Coulomb coupling,…

The phase diagram of halogen-bridged mixed-valent metal complexes ($MX$) has been studied using a two-band extended Peierls-Hubbard model employing the recently developed Density Matrix Renormalization Group method. We present the energies,…

Exciton effects on soliton and bipolaron lattice states are investigated using an electron-lattice Peierls model with long-range Coulomb interactions. The Hartree-Fock (HF) approximation and the single-excitation configuration- interaction…

Internal conversion from the photoexcited state to a correlated singlet triplet-pair state is believed to be the precursor of singlet fission in carotenoids. We present numerical simulations of this process using a pi-electron model that…

Dynamical properties of photoexcited states are theoretically studied in a one-dimensional Mott insulator dimerized by the spin-Peierls instability. Numerical calculations combined with a perturbative analysis have revealed that the lowest…

The lowest electronic excitations of benzene and a set of donor-acceptor molecular complexes are calculated for the gas phase and on the Al(111) surface using the many-body Bethe-Salpeter equation (BSE). The energy of the charge-transfer…

We explore the possibility of calculating electronic excited states by using perturbation theory along a range-separated adiabatic connection. Starting from the energies of a partially interacting Hamiltonian, a first-order correction is…

We study the photoluminescence (PL) of a two-dimensional liquid of oriented dipolar excitons in In_{x}Ga_{1-x}As coupled double quantum wells confined to a microtrap. Generating excitons outside the trap and transferring them at lattice…

The ground state of 2D electrons in high magnetic field is studied by the density matrix renormalization group method. The ground state energy, excitation gap, and pair correlation functions are systematically calculated at various fillings…

The microscopic variant of the Grodzins relation and the Quasiparticle Phonon Model are applied to predict the excitation energies of the $2^+_1$ states of neutron deficient U and Pu isotopes. The P-factor systematics is used to determine…

For the one-dimensional, extended Peierls--Hubbard model we calculate analytically the ground-state energy and the single-particle gap to second order in the Coulomb interaction for a given lattice dimerization. The comparison with…