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In this study, we evaluate the predictive power of density functional theory (DFT) for the magnetic properties of MnBi\(_2\)Te\(_4\) (MBT), an intrinsically magnetic topological insulator with potential applications in spintronics and…

We present first principles calculations of the dynamic susceptibility in strained and doped ferromagnetic MnBi using time-dependent density functional theory. In spite of being a metal, MnBi exhibits signatures of strong correlation and a…

材料科学 · 物理学 2022-11-08 Thorbjørn Skovhus , Thomas Olsen , Henrik M. Rønnow

Doped transition-metal dichalcogenides monolayers exhibit exciting magnetic properties for the benefit of two-dimensional spintronic devices. Using density functional theory (DFT) incorporating Hubbard-type of correction (DFT$+U$) to…

材料科学 · 物理学 2021-05-12 Adlen Smiri , Sihem Jaziri , Samir Lounis , Iann C. Gerber

MnBi2Te4(MBT) is a promising van der Waals layered antiferromagnetic (AF) topological insulator that combines a topologically non-trivial inverted Bi-Te band gap with ferromagnetic (FM) layers of Mn ions. We perform inelastic neutron…

强关联电子 · 物理学 2021-12-06 Bing Li , D. M. Pajerowski , S. Riberolles , Liqin Ke , J. Q. Yan , R. J. McQueeney

The intrinsically anti-ferromagnetic topological insulator, MnBi$_2$Te$_4$ (MBT), has garnered significant attention recently. The excitement for this layered van der Waals bonded compound stems from its potential to host numerous exotic…

We study the effect of stacking faults on the topological properties of the magnetic topological insulator MnBi$_{2}$Te$_{4}$ (MBT) using density functional theory calculations and the Hubbard $U$ being tuned with many-body diffusion Monte…

材料科学 · 物理学 2023-05-17 Jeonghwan Ahn , Seoung-Hun Kang , Mina Yoon , Panchapakesan Ganesh , Jaron T. Krogel

Monolayer MnO$_2$ is one of the few predicted two-dimensional (2D) ferromagnets that has been experimentally synthesized and is commercially available. The Mermin-Wagner theorem states that magnetic order in a 2D material cannot persist…

强关联电子 · 物理学 2022-03-28 Daniel Wines , Kayahan Saritas , Can Ataca

Two-dimensional (2D) 1T-VSe$_2$ has prompted significant interest due to the discrepancies regarding alleged ferromagnetism (FM) at room temperature, charge density wave (CDW) states and the interplay between the two. We employed a combined…

Bulk MnBi$_2$Te$_4$ (MBT) is an intrinsic antiferromagnetic topological insulator. However, its low N\'eel temperature of $\sim 25\,\mathrm{K}$ severely restricts its practical applications. Here, we propose a van der Waals heterostructure…

材料科学 · 物理学 2025-08-12 Yuanhao Zhu , Xixi Yuan , Ying Zhao , Jin Zhang , Zijing Ding , Huixia Fu

Understanding the magnetic properties of the various Mn doping configurations that can be encountered in $2H$-MoS$_2$ monolayer could be beneficial for its use in spintronics. Using density functional theory plus Hubbard U (DFT$+$U)…

材料科学 · 物理学 2019-09-04 Adlen Smiri , Iann Gerber , Samir Lounis , Sihem Jaziri

Multipolar magnetic phases in correlated insulators represent a great challenge for Density Functional Theory (DFT) due to the coexistence of intermingled interactions, typically spin-orbit coupling, crystal field and complex non-collinear…

强关联电子 · 物理学 2022-07-27 Dario Fiore Mosca , Leonid V. Pourovskii , Cesare Franchini

MnBi$_2$Te$_4$ and MnBi$_4$Te$_7$ are antiferromagnetic topological insulators belonging to the MnBi$_{2n}$Te$_{3n+1}$ series, where structural layering provides a natural route to tune magnetic interaction in van der Waals magnets. Despite…

材料科学 · 物理学 2026-03-12 Nazma Firdosh , Shreyashi Sinha , Sujit Manna

MnBi$_2$Te$_4$ (MBT) materials are promising antiferromagnetic topological insulators where field driven ferromagnetism is predicted to cause a transition between axion insulator and Weyl semimetallic states. However, the presence of…

材料科学 · 物理学 2021-06-03 You Lai , Liqin Ke , Jiaqiang Yan , Ross D. McDonald , Robert J. McQueeney

We study the structural, electronic and vibrational properties of single-layer 1TNbSe$_2$ from first principles. Within the generalized gradient approximation, the 1T polytype is highly unstable with respect to the 2H. The DFT+U method…

材料科学 · 物理学 2018-07-18 Matteo Calandra

Manipulating the optical and quantum properties of two-dimensional (2D) materials through strain engineering is not only fundamentally interesting but also provides significant benefits across various applications. In this work, we employ…

材料科学 · 物理学 2025-09-23 Nguyen Tuan Hung , Vuong Van Thanh , Mingda Li , Takahiro Shimada

Density-functional theory is widely used to predict the physical properties of materials. However, it usually fails for strongly correlated materials. A popular solution is to use the Hubbard corrections to treat strongly correlated…

Two-dimensional van der Waals MnBi$_{2n}$Te$_{3n+1}$ (n = 1, 2, 3, 4) compounds have been recently found to be intrinsic magnetic topological insulators rendering quantum anomalous Hall effect and diverse topological states. Here, we…

强关联电子 · 物理学 2021-01-13 Lei Ding , Chaowei Hu , Erxi Feng , Chenyang Jiang , Iurii A. Kibalin , Arsen Gukasov , MiaoFang Chi , Ni Ni , Huibo Cao

We present a new approach based on the static density functional theory (DFT) to describe paramagentic MnO, which is a representative paramagnetic Mott insulator. We appended the spin noncollinearity and the canonical ensemble to the…

强关联电子 · 物理学 2020-07-14 Sangmoon Yoon , Seoung-Hun Kang , Sangmin Lee , Kuntae Kim , Jeong-Pil Song , Miyoung Kim , Young-Kyun Kwon

The magnetic state of UO$_2$ was determined experimentally to be anti-ferromagnetic. Starting from this experimental fact, researchers have calculated other properties within the Hubbard-corrected density-functional theory, DFT+U. Up to…

材料科学 · 物理学 2024-01-03 Mahmoud Payami

Accurate determination of electronic properties of correlated oxides remains a significant challenge for computational theory. Traditional Hubbard-corrected density functional theory (DFT+U) frequently encounters limitations in precisely…

材料科学 · 物理学 2024-03-19 Hyeondeok Shin , Kevin Gasperich , Tomas Rojas , Anh T. Ngo , Jaron T. Krogel , Anouar Benali
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