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We have performed extensive ab initio calculations to investigate phonon dynamics and their possible role in superconductivity in BaFe2As2 and related systems. The calculations are compared to inelastic neutron scattering data that offer…

超导电性 · 物理学 2009-11-13 M. Zbiri , H. Schober , M. R. Johnson , S. Rols , R. Mittal , Y. Su , M. Rotter , D. Johrendt

Spin and lattice dynamics of CaMn7O12 ceramics were investigated using infrared, THz and inelastic neutron scattering (INS) spectroscopies in the temperature range 2 to 590 K, and, at low temperatures, in applied magnetic fields of up to 12…

Quantum memories facilitate the storage and retrieval of quantum information for on-chip and long-distance quantum communications. Thus, they play a critical role in quantum information processing and have diverse applications ranging from…

介观与纳米尺度物理 · 物理学 2024-03-18 Manoj Settipalli , Xufeng Zhang , Sanghamitra Neogi

Self-stimulated echoes have recently been reported in the high cooperativity and inhomogeneous coupling regime of spin ensembles with superconducting resonators. In this work, we study their relative amplitudes using echo-silencing made…

量子物理 · 物理学 2023-09-21 Sebastian de Graaf , Aditya Jayaraman , Sergey Kubatkin , Andrey Danilov , Vishal Ranjan

Interfacing photonic and solid-state qubits within a hybrid quantum architecture offers a promising route towards large scale distributed quantum computing. In that respect, hybrid quantum systems combining circuit QED with ions doped into…

量子物理 · 物理学 2016-04-22 S. Probst , H. Rotzinger , A. V. Ustinov , P. A. Bushev

This study investigates the ultrafast dynamics of coherent phonons and phonon-polaritons in lithium niobate (LiNbO$_{3}$) crystals using reflective pump-probe spectroscopy with 25-fs time resolution. In addition to several coherent optical…

材料科学 · 物理学 2022-08-23 Aizitiaili Abulikemu , Takumi Fukuda , Muneaki Hase

We present the vibrational properties and phonon dispersion for quasi-2D hybrid organic-inorganic perovskites (BA)$_2$CsPb$_2$I$_7$, (HA)$_2$CsPb$_2$I$_7$, (BA)$_2$(MA)Pb$_2$I$_7$, and (HA)$_2$(MA)Pb$_2$I$_7$ calculated from first…

材料科学 · 物理学 2024-01-23 Emily Y. Chen , Bartomeu Monserrat

Strongly interacting phonons and orbital excitations are observed in the same energy range for CuSb$_2$O$_6$, unlocking a so-far unexplored type of electron-phonon interaction. An orbital wave at $\sim 550$ cm$^{-1}$ softens on warming and…

强关联电子 · 物理学 2018-05-17 D. T. Maimone , A. B. Christian , J. J. Neumeier , E. Granado

We investigate coherent lattice dynamics in optimally doped YBa$_2$Cu$_3$O$_{7-\delta}$ driven by ultrashort ($\sim$ 12 fs) near infrared (NIR) and near ultraviolet (NUV) pulses. Transient reflectivity experiments, performed at room…

材料科学 · 物理学 2023-05-08 Kunie Ishioka , Alexej Pashkin , Christian Bernhard , Hrvoje Petek , Xin Yao , Jure Demsar

The phonon renormalization across the semiconductor-to-metal crossover in FeSi is investigated by inelastic neutron scattering combined with \textit{ab-initio} lattice dynamical calculations. A significant part of reciprocal space with a…

Motivated by the recent experimental discovery of strongly surface-plane-dependent superconductivity at surfaces of KTaO$_3$ single crystals, we calculate the electron-phonon coupling strength, $\lambda$, of doped KTaO$_3$ along the…

材料科学 · 物理学 2023-02-21 Tobias Esswein , Nicola A. Spaldin

The phonon dispersion relations of crystal lattices can often be well-described with the harmonic approximation. However, when the potential energy landscape exhibits more anharmonicity, for instance, in case of a weakly bonded crystal or…

材料科学 · 物理学 2022-01-19 Jonathan Lahnsteiner , Menno Bokdam

We report a study of the lattice dynamics in superconducting NaFeAs (Tc = 8 K) and doped NaFe0.97Co0.03As (Tc = 20 K) using Raman light scattering. Five of the six phonon modes expected from group theory are observed. In contrast with…

超导电性 · 物理学 2016-11-25 Y. J. Um , Yunkyu Bang , B. H. Min , Y. S. Kwon , M. Le Tacon

Quantum repeaters based on heralded entanglement require quantum nodes that are able to generate multimode quantum correlations between memories and telecommunication photons. The communication rate scales linearly with the number of modes,…

Lattice dynamics and high pressure phase transitions in AWO4 (A = Ba, Sr, Ca and Pb) have been investigated using inelastic neutron scattering experiments, ab-initio density functional theory calculations and extensive molecular dynamics…

材料科学 · 物理学 2015-06-22 Prabhatasree Goel , M. K. Gupta , R. Mittal , S. Rols , S. N. Achary , A. K. Tyagi , S. L. Chaplot

Despite the tremendous progress in spintronic studies of van der Waals (vdW) room-temperature ferromagnet Fe3GaTe2, much less effort has been spent on its lattice dynamics and possible interaction with spintronic degrees of freedom. In this…

材料科学 · 物理学 2025-06-12 Xia Chen , Xi Zhang , Wenjie He , Yu Li , Jiating Lu , Dinghua Yang , Deren Li , Li Lei , Yong Peng , Gang Xiang

Synthetic powder, ore samples and mineral single crystals of goethite ($\alpha-$FeOOH) were investigated with polarized Raman spectroscopy at temperatures from 300 K to 473 K. The symmetry of the vibrational modes, observed in different…

材料科学 · 物理学 2020-06-24 M. V. Abrashev , V. G. Ivanov , B. S. Stefanov , N. D. Todorov , J. Rosell , V. Skumryev

A strong electron-phonon interaction arises from the modulation of the superexchange interaction by phonons. As is studied in Phys. Rev. B 70, 184514 (2004), Cu-O bond stretching modes can be soft around (pm pi/a, 0) and (0, pm pi/a), with…

超导电性 · 物理学 2015-06-25 Fusayoshi J. Ohkawa

We present neutron inelastic scattering measurements of the low-energy phonons in single crystal BiFeO3. The dispersions of the three acoustic phonon modes (LA along [100], TA1 along [010] and TA2 along [110]) and two low energy optic…

Radio-frequency compressed ultrafast electron diffraction has been used to probe the coherent and incoherent coupling of impulsive electronic excitation at 1.55 eV (800 nm) to optical and acoustic phonon modes directly from the perspective…