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The photochemical CO2 reduction reaction represents a zero-carbon pathway for converting CO2 into value-added chemicals, yet its industrial implementation has been constrained by low selectivity and product diversity. Dirac nodal arc…

材料科学 · 物理学 2026-02-23 Kangwang Wang , Jie Zhan , Jun Liu , Zaichen Xiang , Wanyi Zhang , Lingyong Zeng , Kai Yan , Yan Sun , Huixia Luo

Efficient and selective CO2 electroreduction into value-added chemicals and fuels emerged as a significant approach for CO2 conversion, however, it relies on catalysts with controllable product selectivity and reaction paths. In this work,…

介观与纳米尺度物理 · 物理学 2022-10-26 Wei Xun , Xiao Yang , Qing-Song Jiang , Ming-Jun Wang , Yin-Zhong Wu , Ping Li

Novel photoelectrocatalysts that use sunlight to power the CO$_2$ reduction reaction will be crucial for carbon-neutral power and energy-efficient industrial processes. Scalable photoelectrocatalysts must satisfy a stringent set of…

Chirality is a fundamental property of great importance in physics, chemistry, and biology, and has recently been found to generate unexpected spin polarization for electrons passing through organic molecules, known as chirality-induced…

介观与纳米尺度物理 · 物理学 2024-01-25 Qun Yang , Yongkang Li , Claudia Felser , Binghai Yan

Methane (CH4) and nitrous oxide (N2O) are potent greenhouse gases that represent substantial chemical energy. Conversion of these abundant waste gases to high-value chemicals typically requires high temperatures up to 1000 C, producing…

Chiral-induced spin selectivity (CISS) is a phenomenon in which electron spins are polarized as they are transported through chiral molecules, and the spin polarization depends on the handedness of the chiral molecule. In this study, we…

介观与纳米尺度物理 · 物理学 2023-02-09 Nguyen Thanh Phuc

Chirality-induced spin selectivity is a spin-splitting phenomenon from a helical structure with a considerably effective spin-orbit coupling. This unexpectedly large spin-splitting phenomenon has been experimentally observed in chiral…

强关联电子 · 物理学 2024-05-08 Meng Xu , Yan Chen

Bio-spinterfaces present numerous opportunities to study spintronics across the biomolecules attached to (ferro)magnetic electrodes. While it offers various exciting phenomena to investigate, it's simultaneously challenging to make stable…

Here we review a universal model for chirally induced spin-selectivity (CISS) as a standalone effect occurring in chiral molecules. We tie together the results of forward scattering in the gas phase to the results for photoelectrons in…

介观与纳米尺度物理 · 物理学 2024-06-24 Miguel Mena , Solmar Varela , Bertrand Berche , Ernesto Medina

Chiral-Induced Spin Selectivity (CISS) describes the emergence of spin-polarized electron transport in chiral systems without magnetic fields, a remarkable effect in light-element materials with weak intrinsic spin-orbit coupling (SOC).…

Manipulation of spin-polarized electronic states of two-dimensional (2D) materials under ambient conditions is necessary for developing new quantum devices with small physical dimensions. Here, we explore spin-dependent electronic…

介观与纳米尺度物理 · 物理学 2021-11-24 Rajibul Islam , Barun Ghosh , Carmine Autieri , Sugata Chowdhury , Arun Bansil , Amit Agarwal , Bahadur Singh

The materials with spin-polarized electronic states have attracted a huge amount of interest due to their potential applications in spintronics. Based on first-principles calculations, we study the electronic characteristics of a series of…

材料科学 · 物理学 2022-01-13 Shenda He , Ruirong Kang , Pan Zhou , Zehou Li , Yi Yang , Lizhong Sun

Chirality describes the asymmetry between an object and its mirror image and manifests itself in diverse functionalities across all scales of matter - from molecules and aggregates to thin films and bulk chiral materials. A particularly…

Despite ongoing research, the rational design of nontrivial topological semimetal surface states for the selective photocatalytic CO$_2$ conversion into valuable products remains full of challenges. Herein, we present the synthesis of…

Photoelectrochemical solar water splitting is a promising approach to convert solar energy into sustainable hydrogen fuel using semiconductor electrodes. Due to their visible light absorption properties, oxynitrides have shown to be…

Spin-resolved photoelectron spectroscopy (PES) is a major experimental probe of chirality-induced spin selectivity (CISS), yet it remains unclear whether the measured spin polarization reflects molecular chirality itself or the broader…

材料科学 · 物理学 2026-03-25 Amos Afugu , Gyanu P. Kafle , Zhen-Fei Liu

Polarization control is a critical function in integrated photonic circuits, directly impacting performance, stability, and signal integrity. In this work, we demonstrate the integration of multiferroic two-dimensional (2D) material…

Materials with chiral electronic structures are of great interest. We report a triazatruxene, TAT, molecular semiconductor with chiral alkyl side chains that crystallises from solution to form chirally-stacked columns with a helical pitch…

Photonic bound states in the continuum (BICs) have emerged as a versatile tool for enhancing light-matter interactions by strongly confining light fields. Chiral BICs are photonic resonances with a high degree of circular polarisation,…

Electrical generation of polarized spins in nonmagnetic materials is of great interest for the underlying physics and device potential. One such mechanism is chirality-induced spin selectivity (CISS), with which structural chirality leads…

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