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We explore the novel capabilities offered by attosecond extreme ultraviolet and x-ray pulses that can be now generated by free-electron lasers and high-harmonics generation sources for probing photon-induced electron dynamics in molecules.…

量子物理 · 物理学 2023-02-15 Marvin Reuner , Daria Popova-Gorelova

Characterizing time delays in molecular photoionization as a function of the ejected electron emission direction relative to the orientation of the molecule and the light polarization axis pro-vides unprecedented insights into the…

Explaining observed properties in terms of underlying shape degrees of freedom is a well--established prism with which to understand atomic nuclei. Self--consistent mean--field models provide one tool to understand nuclear shapes, and their…

核理论 · 物理学 2015-12-01 P. D. Stevenson , P. M. Goddard , A. Rios

The dynamic of complex ordering systems with active rotational degrees of freedom exemplified by protein self-assembly is explored using a machine learning workflow that combines deep learning-based semantic segmentation and rotationally…

Today's high-power laser systems are capable of reaching photon intensities up to $10^{22}$ W/cm^2, generating plasmas when interacting with material. The high intensity and ultrashort laser pulse duration (fs) make direct observation of…

Coherent control of ultrafast quantum phenomena benefits from pulse-shaping capabilities allowing to modulate the envelope and instantaneous phase of optical fields on femtosecond time scales. While such control is available for optical…

光学 · 物理学 2026-02-05 Nelin Laštovičková Streshkova , Martin Kozák

Time integrated spectroscopic measurements are carried out to characterize transient plasma stream produced in a coaxial pulsed plasma accelerator. This method allows the estimation of different plasma parameters and its evolution with…

等离子体物理 · 物理学 2020-08-04 A. Ahmed , S. Singha , S. Borthakur , N. K. Neog , T. K. Borthakur , J. Ghosh

We perform time- and angle-resolved photoelectron spectroscopy on p-type GaAs(110). We observe an optically excited population in the conduction band, from which the time scales of intraband relaxation and surface photovoltage decay are…

材料科学 · 物理学 2013-12-06 Shuolong Yang , Jonathan A. Sobota , Patrick S. Kirchmann , Zhi-Xun Shen

Short-time filtering of the photoionization amplitude extracted straight from the numerical solution of the time-dependent Schr\"{o}dinger equation (TDSE) is used to identify dominant pathways that form photoelectron spectra in strong…

原子物理 · 物理学 2020-10-21 V. A. Tulsky , D. Bauer

Using time dependent density functional theory (TDDFT) we examine the energy, angular and time-resolved photoelectron spectra (TRPES) of ethylene in a pump-probe setup. To simulate TRPES we expose ethylene to an ultraviolet (UV) femtosecond…

原子与分子团簇 · 物理学 2014-08-28 Alison Crawford-Uranga , Umberto De Giovannini , Duncan John Mowbray , Stefan Kurth , Angel Rubio

A numerical modeling of the radiation emitted from a Luminescent dye embedded in a finite one-dimensional photonic crystal is presented. The Photonic Band Structure and the Photonic Density of States are derived using classical…

光学 · 物理学 2010-12-30 J. Manzanares-Martinez , P. Castro-Garay

Development of ultrafast lasers and non-linear optical techniques over the last two decades provides tools to access real-time dynamics of low energy excitations in superconductors. For example, time-resolved THz spectroscopy and time- and…

超导电性 · 物理学 2022-04-20 Jure Demsar

The electron motion in atoms and molecules is at the heart of all phenomena in nature that occur outside the nucleus. Recently, ultrafast electron and X-ray imaging tools have been developed to image the ultrafast dynamics of matter in real…

Recent advances in time-resolved angle-resolved photoemission spectroscopy have enabled access to ultrafast electron states and their spin dynamics in solids. Atomically thin transition metal dichalcogenides are paradigmatic two-dimensional…

介观与纳米尺度物理 · 物理学 2025-02-13 Alejandro S. Gómez , Yuriko Baba , Francisco Domínguez-Adame , Rafael A. Molina

We present the results of the first strong lens time delay challenge. The motivation, experimental design, and entry level challenge are described in a companion paper. This paper presents the main challenge, TDC1, which consisted of…

Real-time deformability cytometry (RT-DC) is an established method that quantifies features like size, shape, and stiffness for whole cell populations on a single-cell level in real time. To extract the cell stiffness, a lookup table (LUT)…

定量方法 · 定量生物学 2022-08-29 Lucas Daniel Wittwer , Felix Reichel , Paul Müller , Jochen Guck , Sebastian Aland

Time-to-Digital Converters (TDCs) are major components for the measurements of time intervals. Recent developments in Field-Programmable Gate Array (FPGA) have enabled the opportunity to implement high-performance TDCs, which were only…

系统与控制 · 电气工程与系统科学 2024-10-28 Yuanyuan Hua , Danial Chitnis

An analytical approach to quantum mechanical wave packet dynamics of laser-driven particles is presented. The time-dependent Schroedinger equation is solved for an electron exposed to a linearly polarized plane wave of arbitrary shape. The…

量子物理 · 物理学 2007-05-23 M. Verschl , C. H. Keitel

Spectroscopic photoemission microscopy is a well-established method to investigate the electronic structure of surfaces. In modern photoemission microscopes the electron optics allows imaging of the image plane, momentum plane, or…

The squeezed photons, as a quantum-correlated light with reduced noise, have emerged as a great resource for sensing the structures of matter. Here we study the transient absorption (TA) scheme using the squeezed photons whose spectral…

量子物理 · 物理学 2026-05-29 Jiahao Joel Fan , Feihong Liu , Dangyuan Lei , Zhedong Zhang