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We have used tight-binding molecular-dynamics simulations to investigate the role of point defects (vacancies and interstitials) on structural relaxation in amorphous silicon. Our calculations give unambiguous evidence that point defects…

材料科学 · 物理学 2007-05-23 Cristiano L. Dias , Laurent J. Lewis , S. Roorda

The defect relaxation volumes obtained from density-functional theory (DFT) calculations of charged vacancies and interstitials are much larger than their neutral counterparts, seemingly unphysically large. In this work, we investigate the…

Point defects in body-centred cubic Fe, Cr and concentrated random magnetic Fe-Cr are investigated using density functional theory and theory of elasticity. The volume of a substitutional Cr atom in ferromagnetic bcc Fe is approximately…

Modeling point defects at an atomic scale requires careful treatment of the long-range atomic relaxations. This elastic field can strongly affect point defect properties calculated in atomistic simulations because of the finite size of the…

材料科学 · 物理学 2013-10-23 Céline Varvenne , Fabien Bruneval , Mihai-Cosmin Marinica , Emmanuel Clouet

The low energy structures of irradiation-induced defects have been studied in detail, as these determine the available modes by which a defect can diffuse or relax. As a result, there are many studies concerning the relative energies of…

A combinatorial approach is employed to investigate the atomic and electronic structures of a metal vacancy in titanium carbide. It turns out that the usual relaxed geometry of the vacancy is just a metastable state representing a local…

材料科学 · 物理学 2023-10-10 Ekaterina Smirnova , Mehdi Nourazar , Pavel A. Korzhavyi

We study in experiment and with computer simulation the free energy and the kinetics of vacancy and interstitial defects in two-dimensional dipolar crystals. The defects appear in different local topologies which we characterize by their…

软凝聚态物质 · 物理学 2015-06-23 Wolfgang Lechner , David Polster , Georg Maret , Christoph Dellago , Peter Keim

The characteristics of intrinsic defects are important for the understanding of self-diffusion processes, mechanical strength, brittleness, and plasticity of tungsten carbide, which present in the divertor of fusion reactors. Here, we use…

材料科学 · 物理学 2015-05-19 Xiang-Shan Kong , Yu-Wei You , J. H. Xia , C. S. Liu , Q. F. Fang , G. -N. Luo , Qun-Ying Huang

In this paper we use computer simulations to examine point defects in systems of "soft" colloidal particles including Hertzian spheres, and star polymers. We use Monte Carlo simulations to determine the deformation of the different crystals…

软凝聚态物质 · 物理学 2021-04-15 Marjolein de Jager , Joris de Jong , Laura Filion

We discuss the roles of continuum linear elasticity and atomistic calculations in determining the formation volume and the strain energy of formation of a point defect in a crystal. Our considerations bear special relevance to defect…

材料科学 · 物理学 2007-05-23 K. Garikipati , M. L. Falk , M. Bouville , B. Puchala , H. Narayanan

In materials science, point defects play a crucial role in materials properties. This is particularly well known for the wide band gap insulators where the defect formation/compensation determines the equilibrium Fermi level and generally…

材料科学 · 物理学 2023-11-29 Harshan Reddy Gopidi , Lovelesh Vashist , Oleksandr I. Malyi

Defects are inevitably present in two-dimensional (2D) materials and usually govern their various properties. Here a comprehensive density functional theory-based investigation of 7 kinds of point defects in a recently produced {\gamma}…

材料科学 · 物理学 2021-03-15 Andrey A. Kistanov , Vladimir R. Nikitenko , Oleg V. Prezhdo

Point defects play a crucial role in crystalline materials as they do not only impact the thermodynamic properties but are also central to kinetic processes. While they are necessary in thermodynamic equilibrium spontaneous defect formation…

材料科学 · 物理学 2020-08-03 Erik Fransson , Paul Erhart

Columnar crystals contain defects in the form of vacancy/interstitial loops or strings of vacancies and interstitials bounded by column ``heads'' and ``tails''. These defect strings are oriented by the columnar lattice and can change size…

软凝聚态物质 · 物理学 2009-10-31 Shilpa Jain , David R. Nelson

Using first principles calculations we have studied the formation energies, electron and hole affinities, and electronic levels of intrinsic point defects in zircon. The atomic structures of charged interstitials, vacancies, Frenkel pairs…

材料科学 · 物理学 2007-05-23 J. M. Pruneda , Emilio Artacho

Point defect species and concentrations in metastable Fe-C alloys are determined using density functional theory and a constrained free-energy functional. Carbon interstitials dominate unless iron vacancies are in significant excess,…

材料科学 · 物理学 2007-05-23 Clemens J. Foerst , Jan Slycke , Krystyn J. Van Vliet , Sidney Yip

We present a comprehensive first-principles investigation of carbon self-interstitial defects in diamond, ranging from mono- to hexa-interstitial complexes. By quantum mechanical density functional theory, empowered by interatomic potential…

材料科学 · 物理学 2026-05-01 Nima Ghafari Cherati , Arsalan Hashemi , Ádám Gali

We formulate a model for a point defect embedded in a homogeneous multilattice crystal with an empirical interatomic potential interaction. Under a natural, phonon stability assumption we quantify the decay of the long-range elastic fields…

偏微分方程分析 · 数学 2016-10-03 Derek Olson , Christoph Ortner

Crystal defects crucially influence the properties of crystalline materials and have been extensively studied. Even for the simplest type of defect - the point defect - however, basic properties such as their diffusive behavior, and their…

软凝聚态物质 · 物理学 2024-06-05 Max P. M. Schelling , Janne-Mieke Meijer

Vacancy formation energetics fundamentally govern the structural integrity and catalytic behavior of metal surfaces. Contrary to conventional coordination-dependent broken-bond models, we identify an anomalous thermodynamic inversion on…

材料科学 · 物理学 2026-05-26 Yiming Tan , Pai Li
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