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The structural and electronic properties of twisted bilayer graphene are investigated from first principles and tight binding approach as a function of the twist angle (ranging from the first "magic" angle $\theta=1.08^\circ$ to…

材料科学 · 物理学 2020-10-28 G. Cantele , D. Alfè , F. Conte , V. Cataudella , D. Ninno , P. Lucignano

By virtue of being atomically thin, the electronic properties of heterostructures built from two-dimensional materials are strongly influenced by atomic relaxation. The atomic layers behave as flexible membranes rather than rigid crystals.…

强关联电子 · 物理学 2025-01-07 Mohammed M. Al Ezzi , Gayani N. Pallewela , Christophe De Beule , E. J. Mele , Shaffique Adam

We present a multi-scale density functional theory (DFT) informed molecular dynamics and tight-binding (TB) approach to capture the interdependent atomic and electronic structures of twisted bilayer graphene. We calibrate the flat band…

介观与纳米尺度物理 · 物理学 2022-03-17 Nicolas Leconte , Srivani Javvaji , Jiaqi An , Appalakondaiah Samudrala , Jeil Jung

Van der Waals heteroepitaxy allows deterministic control over lattice mismatch or azimuthal orientation between atomic layers to produce long wavelength superlattices. The resulting electronic phases depend critically on the superlattice…

We introduce a complete physical model for the single-particle electronic structure of twisted bilayer graphene (tBLG), which incorporates the crucial role of lattice relaxation. Our model, based on $k \cdot p$ perturbation theory, combines…

介观与纳米尺度物理 · 物理学 2019-08-14 Stephen Carr , Shiang Fang , Ziyan Zhu , Efthimios Kaxiras

We present efficient angle-dependent low-energy Hamiltonians to describe the properties of the twisted bilayer graphene (tBLG) heterostructure, based on {\it ab initio} calculations of mechanical relxation and electronic structure. The…

介观与纳米尺度物理 · 物理学 2019-08-02 Shiang Fang , Stephen Carr , Ziyan Zhu , Daniel Massatt , Efthimios Kaxiras

A major hurdle in understanding the phase diagram of twisted bilayer graphene (TBLG) are the roles of lattice relaxation and electronic structure on isolated band flattening near magic twist angles. In this work, the authors develop an…

介观与纳米尺度物理 · 物理学 2024-03-28 Shivesh Pathak , Tawfiqur Rakib , Run Hou , Andriy Nevidomskyy , Elif Ertekin , Harley T. Johnson , Lucas K. Wagner

Twisted double bilayer graphene has recently emerged as an interesting moir\'e material that exhibits strong correlation phenomena that are tunable by an applied electric field. Here we study the atomic and electronic properties of three…

Atomically thin moir\'e materials behave like elastic membranes where at very small twist angles, the van der Waals adhesion energy much exceeds the strain energy. In this ``marginal twist" regime, regions with low adhesion energy expand,…

介观与纳米尺度物理 · 物理学 2025-03-26 Christophe De Beule , Gayani N. Pallewela , Mohammed M. Al Ezzi , Liangtao Peng , E. J. Mele , Shaffique Adam

The interplay of twist and strain in bilayer graphene enables the formation of moir\'e patterns and narrow bands that host correlated and topological phases. While magic-angle twisted bilayer graphene has been widely studied, strain…

介观与纳米尺度物理 · 物理学 2026-03-10 Federico Escudero , Dong Wang , Pierre A. Pantaleón , Shengjun Yuan , Francisco Guinea , Zhen Zhan

Twisted bilayer graphene (TBG) has drawn significant interest due to recent experiments which show that TBG can exhibit strongly correlated behavior such as the superconducting and correlated insulator phases. Much of the theoretical work…

数学物理 · 物理学 2025-05-23 Tianyu Kong , Alexander B. Watson , Mitchell Luskin , Kevin D. Stubbs

We present a comprehensive first-principles study of twisted bilayer graphene (tBLG) for a wide range of twist angles, with a focus on structural and electronic properties. By employing density functional theory (DFT) with an optimized…

介观与纳米尺度物理 · 物理学 2026-05-13 Albert Zhu , Daniel Bennett , Daniel T. Larson , Mohammed M. Al Ezzi , Efstratios Manousakis , Efthimios Kaxiras

Twisted bilayer graphene (TBG) exhibits a wide range of intriguing physical properties, such as superconductivity, ferromagnetism, and superlubricity. Depending on the twist angle, periodic moir\'e superlattices form in twisted bilayer…

介观与纳米尺度物理 · 物理学 2022-06-07 Vahid Morovati , Zhiming Xue , Kenneth M. Liechti , Rui Huang

We theoretically study the lattice relaxation in the twisted bilayer graphene (TBG) and its effect on the electronic band structure. We develop an effective continuum theory to describe the lattice relaxation in general TBGs and obtain the…

材料科学 · 物理学 2017-09-06 Nguyen N. T. Nam , Mikito Koshino

The interlayer energy of the twisting bilayer graphene is investigated by the molecular mechanics method using both the registry-dependent potential and the Lennard-Jones potential. Both potentials show that the interlayer energy is…

材料科学 · 物理学 2013-07-12 Jin-Wu Jiang , Bing-Shen Wang , Timon Rabczuk

Twisted bilayer graphene exhibits isolated, relatively flat electronic bands near charge neutrality when the interlayer rotation is tuned to specific magic angles. These small misalignments, typically below 1.1{\deg}, result in long-period…

介观与纳米尺度物理 · 物理学 2026-03-26 Antonio Palamara , Michele Pisarra , Antonello Sindona

We study the stability and electronic structure of magic-angle twisted bilayer graphene on the hexagonal boron nitride (TBG/BN). Full relaxation has been performed for commensurate supercells of the heterostructures with different twist…

介观与纳米尺度物理 · 物理学 2021-04-20 Xianqing Lin , Kelu Su , Jun Ni

Although the strongly interacting flat bands in twisted bilayer graphene (TBG) have been approached using the minimal Bistritzer-MacDonald (BM) Hamiltonian, there is mounting evidence that strain and lattice relaxation are essential in…

介观与纳米尺度物理 · 物理学 2025-09-26 Jonah Herzog-Arbeitman , Jiabin Yu , Dumitru Călugăru , Haoyu Hu , Nicolas Regnault , Oskar Vafek , Jian Kang , B. Andrei Bernevig

In the presence of a finite interlayer displacement field bilayer graphene has an energy gap that is dependent on stacking and largest for the stable AB and BA stacking arrangements. When the relative orientations between layers are twisted…

介观与纳米尺度物理 · 物理学 2018-07-11 Dmitry K. Efimkin , Allan H. MacDonald

We introduce a minimum tight-binding model with only three parameters extracted from graphene and untwisted bilayer graphene. This model reproduces quantitatively the electronic structure of not only these two systems and bulk graphite near…

介观与纳米尺度物理 · 物理学 2018-09-12 Xianqing Lin , David Tománek
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