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Despite extensive investigations, many aspects of charge density waves (CDWs) remain elusive, especially the relative roles of electron-phonon coupling and Fermi surface nesting as the underlying driving mechanisms responsible for the…

We report inelastic x-ray scattering measurements of the temperature dependence of phonon dispersion in the prototypical charge-density-wave (CDW) compound NbSe2. Surprisingly, acoustic phonons soften to zero frequency and become overdamped…

强关联电子 · 物理学 2011-11-01 F. Weber , S. Rosenkranz , J. -P. Castellan , R. Osborn , R. Hott , R. Heid , K. -P. Bohnen , T. Egami , A. H. Said , D. Reznik

This paper reports the first experimental observation of phonons and their softening on single crystalline LaPt$_2$Si$_2$ via inelastic neutron scattering. From the temperature dependence of the phonon frequency in close proximity to the…

Phonon softening is a ubiquitous phenomenon in condensed matter systems which is often associated with charge density wave (CDW) instabilities and anharmonicity. The interplay between phonon softening, CDW and superconductivity is a topic…

超导电性 · 物理学 2023-02-27 Cunyuan Jiang , Enrico Beneduce , Matteo Baggioli , Chandan Setty , Alessio Zaccone

A softening of phonon-dispersion has been observed experimentally in under-doped cuprate superconductors at the charge-density wave (CDW) ordering wave vector. Interestingly, the softening occurs below the superconducting (SC) transition…

超导电性 · 物理学 2021-02-24 Saheli Sarkar , Maxence Grandadam , Catherine Pépin

We present a high energy-resolution inelastic x-ray scattering investigation of the soft phonon mode in the charge-density-wave system TbTe$_3$. We analyze our data based on lattice dynamical calculations using…

强关联电子 · 物理学 2015-07-01 M. Maschek , S. Rosenkranz , R. Heid , A. H. Said , P. Giraldo-Gallo , I. R. Fisher , F. Weber

Using single crystal neutron and x-ray diffraction, we discovered a charge density wave (CDW) below 320 K, which accounts for the long-sought origin of the heat capacity and resistivity anomalies in UPt2Si2. The modulation wavevector, Qmod,…

The existence of a charge density wave (CDW) in transition metal dichalcogenide CuS$_2$ has remained undetermined since its first experimental synthesis nearly 50 years ago. Despite conflicting experimental literature regarding its low…

介观与纳米尺度物理 · 物理学 2020-10-07 Yuxin Yin , Jennifer Coulter , Christopher J. Ciccarino , Prineha Narang

We investigate the interplay between charge density wave (CDW) instabilities and ferromagnetism in SmNiC$_2$ using diffuse and inelastic x-ray scattering together with Raman spectroscopy. We identify a soft acoustic phonon driving the…

Charge density wave (CDW), a symmetry-breaking collective phenomenon in condensed matter systems, exhibits periodic modulations of electron density coupled with lattice distortions, where the lattice plays a critical role via…

材料科学 · 物理学 2025-08-26 Wenqian Tu , Run Lv , Dingfu Shao , Yuping Sun , Wenjian Lu

BaNi$_2$As$_2$ is a nonmagnetic analogue of the iron pnictide superconductors, and in its tetragonal state exhibits an incommensurate charge-density-wave (IC-CDW) and a sizable elastoresistance. In this work, phonons in BaNi$_2$As$_2$…

A strong Kohn anomaly in ZrTe_3 is identified in the mostly transverse acoustic phonon branch along the modulation vector q_P with polarization along the a* direction. This soft mode freezes to zero frequency at the transition temperature…

强关联电子 · 物理学 2009-11-13 Moritz Hoesch , Alexey Bosak , Dmitry Chernyshov , Helmuth Berger , Michael Krisch

Among transition metal dichalcogenides (TMDs), VSe$_2$ is considered to develop a purely 3-dimensional (3D) charge-density wave (CDW) at T$_{CDW}$=110 K. Here, by means of high resolution inelastic x-ray scattering (IXS), we show that the…

Interactions with electronic excitations can soften and/or broaden phonons. They are greatly amplified at wavevectors Q+- that connect parallel (nested) sheets of the Fermi surface. In such a case, called a Kohn anomaly, the phonon…

强关联电子 · 物理学 2009-09-04 D. Lamago , M. Hoesch , M. Krisch , R. Heid , K. -P. Bohnen , P. Boeni , D. Reznik

We present a high energy-resolution inelastic x-ray scattering data investigation of the charge-density-wave (CDW) soft phonon mode upon entering the superconducting state in $2H$-NbSe$_2$. Measurements were done close to the CDW ordering…

超导电性 · 物理学 2016-11-23 F. Weber , S. Rosenkranz , R. Heid , A. H. Said

We investigate carrier and collective mode dynamics in 2H-NbSe$_2$ using time-resolved optical pump-probe spectroscopy and compare the results with first-principle calculations. Broadband ultrafast reflectivity studies of 2H-NbSe$_2$ in a…

强关联电子 · 物理学 2020-12-30 A. Anikin , R. D. Schaller , G. P. Wiederrecht , E. R. Margine , I. I. Mazin , G. Karapetrov

We report high-resolution inelastic x-ray measurements of the soft phonon mode in the charge-density-wave compound TiSe$_2$. We observe a complete softening of a transverse optic phonon at the L point, i.e. q = (0.5, 0, 0.5), at T ~…

强关联电子 · 物理学 2015-05-28 F. Weber , S. Rosenkranz , J. -P. Castellan , R. Osborn , G. Karapetrov , R. Hott , R. Heid , K. -P. Bohnen , A. Alatas

The interplay between charge density wave (CDW) order and superconductivity has attracted much attention. This is the central issue of along standing debate in simple transition metal dichalcogenides without strong electronic correlations,…

The charge-density wave (CDW) mechanism and resulting structure of the AV3Sb5 family of kagome metals has posed a puzzling challenge since their discovery four years ago. In fact, the lack of consensus on the origin and structure of the CDW…

The complex coupling between charge carriers and phonons is responsible for diverse phenomena in condensed matter. We apply ultrafast electron diffuse scattering to unravel electron-phonon coupling phenomena in 1T-TiSe$_2$ in both momentum…

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