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Two-dimensional atomic crystals can radically change their properties in response to external influences such as substrate orientation or strain, resulting in essentially new materials in terms of the electronic structure. A striking…

Manipulating the valley degree of freedom to encode information for potential valleytronic devices has ignited a new direction in solid-state physics. A significant, fundamental challenge in the field of valleytronics is how to generate and…

介观与纳米尺度物理 · 物理学 2020-07-02 Hui-Ying Mu , Yi-Tong Yao , Jie-Ru Li , Guo-Cai Liu , Chao He , Ying-Jie Sun , Guang Yang , Xing-Tao An , Yong-Zhe Zhang , Jian-Jun Liu

We study the electronic band structure in the K/K' valleys of the Brillouin zone of monolayer WSe2 and MoSe2 by optical reflection and photoluminescence spectroscopy on dual-gated field-effect devices. Our experiment reveals the distinct…

介观与纳米尺度物理 · 物理学 2017-02-21 Zefang Wang , Liang Zhao , Kin Fai Mak , Jie Shan

Transition metal dichalcogenide (TMD) monolayers present a singular coupling in their spin and valley degrees of freedom. Moreover, by applying an external magnetic field it is possible to break the energy degeneracy between their K and…

Polymorphic structures of transition-metal dichalcogenides (TMDs) host exotic electronic states, like charge density wave and superconductivity. However, the number of these structures is limited by crystal symmetries, which poses a…

材料科学 · 物理学 2024-05-31 Le Lei , Jiaqi Dai , Haoyu Dong , Yanyan Geng , Feiyue Cao , Cong Wang , Rui Xu , Fei Pang , Fangsen Li , Zhihai Cheng , Guang Wang , Wei Ji

Exploring the coupling between layer, magnetism, valley, and topology in two-dimensional (2D) materials is an important approach to deepen our understanding of materials properties. We propose 27 stable ferromagnetic semiconductor…

材料科学 · 物理学 2025-03-03 Xinyu Tian , Zixuan Zhang , Lixiu Guan , Xiaobiao Liu , Xiaoyu Zhao , Linyang Li

This investigation demonstrates that the pentagonal PdTe2 (penta-PdTe2) monolayer is a highly tunable two-dimensional (2D) photocatalyst, characterized by the bandgap of 1.75 eV and high hole mobility. Using density functional theory…

材料科学 · 物理学 2026-03-31 Narender Kumar , Shambhu Bhandari , Dario Alfè , Nacir Tit , Ravindra Pandey

Recent synthesis of monolayer fullerene networks [$Nature$ 606, 507 (2022)] provides new opportunities for photovoltaics and photocatalysis because of their versatile crystal structures for further tailoring of electronic, optical and…

材料科学 · 物理学 2023-12-29 Cory Jones , Bo Peng

Valleytronics is a rising topic to explore the emergent degree of freedom for charge carriers in energy band edges and has attracted a great interest due to many intriguing quantum phenomena and potential application in information…

Two-dimensional semimetals with tilted Dirac cones in the electronic band structure are shown to exhibit spatial separation of carriers belonging to different valleys under illumination. In stark contrast to gapped Dirac materials this…

介观与纳米尺度物理 · 物理学 2023-11-08 A. Wild , E. Mariani , M. E. Portnoi

Stacking two-dimensional (2D) van der Waals materials with different interlayer atomic registry in a heterobilayer causes the formation of a long-range periodic superlattice that may bestow the heterostructure with exotic properties such as…

The evolution of the physical properties of two-dimensional material from monolayer limit to the bulk reveals unique consequences from dimension confinement and provides a distinct tuning knob for applications. Monolayer 1T'-phase…

The two-fold valley degeneracy in two-dimensional (2D) semiconducting transition metal dichalcogenides (TMDCs) (Mo,W)(S,Se)2 is suitable for "valleytronics", the storage and manupulation of information utilizing the valley degree of…

介观与纳米尺度物理 · 物理学 2015-06-24 Shao-Yu Chen , Changxi Zheng , Michael S. Fuhrer , Jun Yan

The selective excitation of coherent phonons provides unique capabilities to control fundamental properties of quantum materials on ultrafast time scales. For instance, in the presence of strong electron-phonon coupling, the electronic band…

材料科学 · 物理学 2020-06-02 P. Hein , S. Jauernik , H. Erk , L. Yang , Y. Qi , Y. Sun , C. Felser , M. Bauer

The concept of ferrovalley materials has been proposed very recently. The existence of spontaneous valley polarization, resulting from ferromagnetism, in such hexagonal two-dimensional materials makes nonvolatile valleytronic applications…

材料科学 · 物理学 2018-07-11 Xin-Wei Shen , Wen-Yi Tong , Shi-Jing Gong , Chun-Gang Duan

Monolayer semiconducting transition metal dichalcogenides possess broken inversion symmetry and strong spin-orbit coupling, which leads to unique spin-valley locking effect. In 2H stacked pristine multilayers, the spin-valley locking yields…

介观与纳米尺度物理 · 物理学 2023-06-07 Yinong Zhang , Chengxin Xiao , Dmitry Ovchinnikov , Jiayi Zhu , Xi Wang , Takashi Taniguchi , Kenji Watanabe , Jiaqiang Yan , Wang Yao , Xiaodong Xu

Benefiting from improved stability due to stronger interlayer van der Waals interactions, few-layer fullerene networks are experimentally more accessible compared to monolayer polymeric C$_{60}$. However, there is a lack of systematic…

材料科学 · 物理学 2025-03-27 Dylan Shearsby , Jiaqi Wu , Dekun Yang , Bo Peng

For a long time, two-dimensional (2D) hexagonal MoS2 was proposed as a promising material for valleytronic system. However, the limited size of growth and low carrier motilities in MoS2 restrict its further application. Very recently, a new…

材料科学 · 物理学 2021-01-27 Chen Yang , Zhigang Song , Xiaotian Sun , Jing Lu

Ferroelectricity and metallicity cannot coexist due to the screening effect of conducting electrons, and a large number of stable monolayers with 1T/1T$^{\prime}$ phase lack spontaneous polarization due to inversion symmetry. In this work,…

材料科学 · 物理学 2023-09-26 Haohao Sheng , Zhong Fang , Zhijun Wang

The mechanical behavior of two-dimensional (2D) materials across 2D phase changes is unknown, and the finite temperature ($T$) elasticity of paradigmatic SnSe monolayers -- ferroelectric 2D materials turning paraelectric as their unit cell…

材料科学 · 物理学 2022-06-15 Joseph E. Roll , John M. Davis , John W. Villanova , Salvador Barraza-Lopez