相关论文: Coherent all X-ray four wave mixing at core shell …

Dark-field X-ray microscopy (DFXM) is a nondestructive full-field imaging technique providing three dimensional mapping of microstructure and local strain fields in deeply embedded crystalline elements. This is achieved by placing an…

A theory is developed and applied to the study of opportunities and specific features of coherent control of four-wave mixing as well as of the accompanying processes in the continuous-wave regime, which involve transitions between bound…

Enabled by x-ray free-electron lasers, nonlinear optical phenomena can be explored in the x-ray domain nowadays. Among the multitude of newly accessible processes, this theoretical study focuses parametric x-ray optical wavemixing for…

Highly coherent and powerful light sources capable of generating soft x-ray frequency combs are essential for high precision measurements and rigorous tests of fundamental physics. In this work, we derive the analytical conditions required…

A search for sub-eV scalar fields coupling to two photons has been performed via four-wave mixing at a quasi-parallel laser collider for the first time. The experiment demonstrates the novel approach to search for resonantly produced sub-eV…

We present a novel time- and phase-resolved, background-free scheme to study the extreme ultraviolet dipole emission of a bound electronic wavepacket, without the use of any extreme ultraviolet exciting pulse. Using multiphoton transitions,…

Multimode fibers (MMFs) show great promise as miniature probes for sensing, imaging and spectroscopy applications. Different parameters of the fibers, such as numerical aperture, refractive index profile and length, have been already…

We combine multi-channel electronic structure theory with quantum optimal control to derive Raman pulse sequences that coherently populate a valence excited state. For a neon atom, Raman target populations of up to 13% are obtained.…

X-ray phase-contrast imaging has recently led to a revolution in resolving power and tissue contrast in biomedical imaging, microscopy and materials science. The necessary high spatial coherence is currently provided by either large-scale…

Resonant inelastic x-ray scattering (RIXS) is a widely used spectroscopic technique, providing access to the electronic structure and dynamics of atoms, molecules, and solids. However, RIXS requires a narrow bandwidth x-ray probe to achieve…

To date X-ray spectroscopy has become a routine tool that can reveal highly local and element-specific information on the electronic structure of atoms in complex environments. Here, we focus on nuclear dynamical effects in X-ray spectra…

In this paper we explore unsupervised spectral decomposition methods for distinguishing the effect of different spectral components for a set of consecutive spectra from an X-ray binary. We use well-established linear methods for the…

The evolution from 3rd to 4th generation synchrotron radiation (SR) sources significantly enhanced their coherence, making coherent scattering techniques such as coherent X-ray diffraction imaging (CXDI) and X-ray photon correlation…

High-quality total scattering data, a key tool for understanding atomic-scale structure in disordered materials, require stable instrumentation and access to high momentum transfers. This is now routine at dedicated synchrotron…

Efficient frequency conversion of photons has important applications in optical quantum technology because the frequency range suitable for photon manipulation and communication usually varies widely. Recently, an efficient frequency…

Compact silicon integrated devices, such as micro-ring resonators, have recently been demonstrated as efficient sources of quantum correlated photon pairs. The mass production of integrated devices demands the implementation of fast and…

Compact coherent x-ray sources have been the focus of extensive research efforts over the past decades. As a result, several novel schemes like optical and nano-undulators for generating x-ray emissions in "table-top" setups are proposed,…

Four-wave mixing can be used to generate coherent output beams, with frequencies difficult to acquire in commercial lasers. Here a single narrow ECDL locked to the two photon 5s-5d transition in rubidium is combined with a tapered amplifier…

We study the perspectives of measuring the phenomenon of vacuum birefringence predicted by quantum electrodynamics using an x-ray free-electron laser (XFEL) alone. We devise an experimental scheme allowing the XFEL beam to collide with…

A deep understanding of molecular photo-transformations is challenging because of the complex interaction between the configurations of electrons and nuclei. An initial optical excitation dissipates energy into electronic and structural…