相关论文: Coherent all X-ray four wave mixing at core shell …
Controlling nonequilibrium responses in optically driven quantum materials is essential for advancing applications in energy conversion, ultrafast electronics, and quantum computation. Nonlinear optical spectroscopy serves as a powerful…
We introduce a framework for scalable and broadband free-space phase-matched four-wave mixing in ring resonators. This method for four-wave mixing reduces the complexity of coupling an emitter to a quantum network by combining the spatial…
We present a theoretical formulation of the coherent ultrafast nonlinear optical response of a strongly correlated system and discuss an example where the Coulomb correlations dominate. We separate out the correlated contributions to the…
We study a nonlinear Schr\"odinger equation which arises as an effective single particle model in X-ray Free Electron Lasers (XFEL). This equation appears as a first-principles model for the beam-matter interactions that would take place in…
The extremely high power densities and short durations of single pulses of x-ray free electron lasers (XFELs) have opened new opportunities in atomic physics, where complex excitation-relaxation chains allow for high ionization states in…
The most promising way to increase the output power of an X-ray FEL (XFEL) is by tapering the magnetic field of the undulator. Also, significant increase in power is achievable by starting the FEL process from a monochromatic seed rather…
Small parts of the electronic wavepacket of a multiple charged ion may still tunnel through the high Coulomb barrier for a sufficiently intense laser field of $10^{15}W/cm^2$ and higher. Solving numerically the corresponding Schr\"odinger…
We have recorded the coherent diffraction images of individual xenon clusters with intense extreme ultraviolet pulses to elucidate the influence of light-induced electronic changes on the diffraction pattern. Using the FLASH free-electron…
Optical spectroscopy with broadband femtosecond laser pulses often involves simultaneous excitation of multiple molecular species with close resonance frequencies. Interpreting the collective optical response from molecular mixtures…
The lack of available table-top extreme ultraviolet (XUV) sources with high enough fluxes and coherence properties have limited the availability of nonlinear XUV and x-ray spectroscopies to free electron lasers (FEL). Here, we demonstrate…
Wave mixing is an archetypical phenomenon in bosonic systems. In optomechanics, the bi-directional conversion between electromagnetic waves or photons at optical frequencies and elastic waves or phonons at radio frequencies is building on…
Structure determination is a key application of XFELs and 4th generation synchrotron sources, particularly using the coherent and pulsed X-ray radiation from X-ray free-electron lasers (XFEL). Scientific interest focuses on understanding…
Knowledge gained through X-ray crystallography fostered structural determination of materials and greatly facilitated the development of modern science and technology in the past century. Atomic details of sample structures is achievable by…
Ultrafast X-ray spectroscopy has been revolutionized in recent years due to the advent of fourth-generation X-ray facilities. In solid-state materials, core excitons determine the energy and line shape of absorption features in core-level…
Up to now, experiments involving M\"ossbauer nuclei have been restricted to the low-excitation regime. The reason for this is the narrow spectral line width of the nuclei. This defining feature enables M\"ossbauer spectroscopy with…
We present a novel three-dimensional (3D) imaging approach that combines two-dimensional spatial Fourier-domain imaging techniques with traditional radar pulse compression to recover both cross-range and down-range scene information. The…
We present a unified elucidation for the role temporal coherence properties of x-rays in surface x-ray standing wave analysis, under total external reflection condition. Analytical formulas have been derived that provide a direct relation…
We present results of a study of four-wave mixing in Rb vapour with highly nonlinear susceptibility, using both homodyne and heterodyne detection. We demonstrate that the spectra have different appearances for media possessing…
Coherent control of quantum dynamics is key to a multitude of fundamental studies and applications alike. In the visible or longer-wavelength domains, near-resonant light fields have become the primary tool to control electron dynamics.…
In this work we present a theoretical description of the transient response of the Fermi Edge Singularity (FES). We study the linear and the nonlinear response of an n-doped QW to laser pulses in the Coherent Control (CC) and Four Wave…