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The properties of excitons, or correlated electron-hole pairs, are of paramount importance to optoelectronic applications of materials. A central component of exciton physics is the electron-hole interaction, which is commonly treated as…

We investigate the influence of vibrational screening on the excitonic and optical properties of solids based on first-principles electronic-structure calculations. We solve the Bethe-Salpeter equation - the state-of-the-art description of…

材料科学 · 物理学 2024-09-24 Maximilian Schebek , Pasquale Pavone , Claudia Draxl , Fabio Caruso

The ab initio Bethe-Salpeter equation (BSE) approach, an established method for the study of excitons in materials, is typically solved in a limit where only static screening from electrons is captured. Here, we generalize this framework to…

材料科学 · 物理学 2021-08-10 Marina R. Filip , Jonah B. Haber , Jeffrey B. Neaton

Metasurfaces enable flat optical elements by leveraging optical resonances in metallic or dielectric nanoparticles to obtain accurate control over the amplitude and phase of the scattered light. While highly efficient, these resonances are…

光学 · 物理学 2022-09-07 Jason Lynch , Ludovica Guarneri , Deep Jariwala , Jorik van de Groep

The light-mediated interaction of fermionic and bosonic excitations governs the optoelectronic properties of condensed matter systems. In photoexcited semiconductors, the coupling of electron-hole pairs (excitons) to coherent optical…

Phonons are well known to be the main mechanism for the coupling between bright and dark excitons in nonmagnetic semiconductors. Here, we investigate diluted magnetic semiconductors where this process is in direct competition with the…

介观与纳米尺度物理 · 物理学 2019-03-12 Florian Ungar , Moritz Cygorek , Vollrath Martin Axt

Phonons play a key role in the physical properties of materials, and have long been a topic of study in physics. While the effects of phonons had historically been considered to be a hindrance, modern research has shown that phonons can be…

We study theoretically the contribution of quantum effects to the exciton diffusion coefficient in atomically thin crystals. It is related to the weak localization caused by the interference of excitonic wavefunctions on the trajectories…

介观与纳米尺度物理 · 物理学 2022-11-23 M. M. Glazov , Z. A. Iakovlev , S. Refaely-Abramson

Theoretical and numerical calculations of the optical absorption spectra of excitons interacting with longitudinal-optical phonons in quasi-2D polar semiconductors are presented. In II-VI semiconductor quantum wells, exciton binding energy…

介观与纳米尺度物理 · 物理学 2009-11-07 F. J. Rodriguez

Engineering of phonons, i.e., collective lattice vibrations in crystals, is essential for manipulating physical properties of materials such as thermal transport, electron-phonon interaction, confinement of lattice vibration, and optical…

材料科学 · 物理学 2022-02-04 Seung Gyo Jeong , Ambrose Seo , Woo Seok Choi

The effect of phonons on a nonlinear optical response of a quantum dot-cavity system in quantum strong coupling regime can be accounted for by a fully analytical treatment, provided that the exciton-phonon dynamics is much faster than the…

介观与纳米尺度物理 · 物理学 2023-06-30 L. S. Sirkina , E. A. Muljarov

We employ quasiparticle path integral molecular dynamics to study how the excitonic properties of model semiconductors are altered by electron-phonon coupling. We describe ways within a path integral representation of the system to evaluate…

材料科学 · 物理学 2022-09-28 Yoonjae Park , David T. Limmer

Tuning the electronic properties of a material by subjecting it to strain constitutes an important strategy to enhance the performance of semiconducting electronic devices. Using local strain, confinement potentials for excitons can be…

Excitonic quasi-particles, excitons/trions/bi-excitons, and their coupling with phonons and charge carriers play a crucial role in controlling the optical properties of atomically thin semiconducting 2D materials. In this work, we…

材料科学 · 物理学 2021-10-01 Deepu Kumar , Rahul Kumar , Mahesh Kumar , Pradeep Kumar

The weakly screened electron-hole interactions in an atomically thin semiconductor not only downshift its excitation spectrum from a quasiparticle one, but also redistribute excitation energies and wavefunction characters with profound…

介观与纳米尺度物理 · 物理学 2018-10-24 Yuanxi Wang , Bruno R. Carvalho , Vincent H. Crespi

We present a fully atomistic approach to exciton-phonon coupling in semiconductor quantum dots that bridges microscopic electronic-structure calculations with non-Markovian open-quantum-system dynamics. On the example of an InAsP quantum…

介观与纳米尺度物理 · 物理学 2026-02-03 Yasser Saleem , Moritz Cygorek

The optical properties of the two-dimensional (2D) crystals are dominated by tightly bound electron-hole pairs (excitons) and lattice vibration modes (phonons). The exciton-phonon interaction is fundamentally important to understand the…

材料科学 · 物理学 2021-02-09 Qing-Hai Tan , Yu-Jia Sun , Xue-Lu Liu , Yanyuan Zhao , Qihua Xiong , Ping-Heng Tan , Jun Zhang

The way nuclear motion affects electronic responses has become a very hot topic in materials science. Coherent acoustic phonons can dynamically modify optical, magnetic and mechanical properties at ultrasonic frequencies, with promising…

介观与纳米尺度物理 · 物理学 2018-08-29 Edoardo Baldini , Tania Palmieri , Adriel Dominguez , Pascal Ruello , Angel Rubio , Majed Chergui

The coupling of excitons with atomic vibrations plays a pivotal role on the nonequilibrium optical properties of layered semiconductors. However, addressing the dynamical interaction between excitons and phonons represents a hard task both…

Two-dimensional (2D) metals can host gapless plasmonic excitations, which strongly couple to electrons and thus may significantly affect superconductivity in layered materials. To investigate the dynamical interplay of the electron-electron…

超导电性 · 物理学 2024-08-21 Yann in 't Veld , Mikhail I. Katsnelson , Andrew J. Millis , Malte Rösner
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