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Heterobilayers formed by stacking two-dimensional atomic crystals are particularly promising for low-dimensional semiconductor optics, as they host interlayer excitons, bound states of electrons and holes residing in different layers. They…

介观与纳米尺度物理 · 物理学 2025-07-31 Suvadip Masanta , Chumki Nayak , Premananda Chatterjee , Atindra Nath Pal , Indrani Bose , Achintya Singha

Layered two-dimensional materials exhibit rich transport and optical phenomena in twisted or lattice-incommensurate heterostructures with spatial variations of interlayer hybridization arising from moir\'e interference effects. Here, we…

In monolayer transition metal dichalcogenides, tightly bound excitons have been discovered with a valley pseudospin that can be optically addressed through polarization selection rules. Here, we show that this valley pseudospin is strongly…

介观与纳米尺度物理 · 物理学 2014-05-20 Hongyi Yu , Guibin Liu , Pu Gong , Xiaodong Xu , Wang Yao

Excitons in monolayer semiconductors have large optical transition dipole for strong coupling with light field. Interlayer excitons in heterobilayers, with layer separation of electron and hole components, feature large electric dipole that…

介观与纳米尺度物理 · 物理学 2019-03-07 Wei-Ting Hsu , Bo-Han Lin , Li-Syuan Lu , Ming-Hao Lee , Ming-Wen Chu , Lain-Jong Li , Wang Yao , Wen-Hao Chang , Chih-Kang Shih

The recent proposal of using an anisotropic vacuum for generating valley coherence in transition metal dichalcogenide (TMDC) monolayers has expanded the potential of such valley degrees of freedom for applications in valleytronics. In this…

光学 · 物理学 2020-10-28 Mandar Sohoni , Pankaj K. Jha , Muralidhar Nalabothula , Anshuman Kumar

The impressive physics and applications of intra- and interlayer excitons in a transition metal dichalcogenide twisted-bilayer make these systems compelling platforms for exploring the manipulation of their optoelectronic properties through…

In stacks of transition metal dichalcogenide monolayers with arbitrary twisting angles, we explore a new class of bright excitons arising from the pronounced F\"{o}rster coupling, whose dimensionality is tuned by its in-plane momentum. The…

介观与纳米尺度物理 · 物理学 2023-11-01 Ci Li , Wang Yao

Transition metal dichalcogenide (TMDC) heterostructures have unique properties that depend on the twisting angle and stacking order of two or more monolayers. However, their practical applications are limited by the low photoluminescence…

We report robust room temperature interlayer excitons in transition metal dichalcogenide heterostructures engineered via precise stacking orientation and twist-angle control. We integrate 2H-stacked…

Monolayers of transition metal dichalcogenides, namely, molybdenum and tungsten disulfides and diselenides demonstrate unusual optical properties related to the spin-valley locking effect. Particularly, excitation of monolayers by…

介观与纳米尺度物理 · 物理学 2015-11-12 M. M. Glazov , E. L. Ivchenko , G. Wang , T. Amand , X. Marie , B. Urbaszek , B. L. Liu

We show that, because of the inevitable twist and lattice mismatch in heterobilayers of transition metal dichalcogenides, interlayer excitons have six-fold degenerate light cones anomalously located at finite velocities on the parabolic…

介观与纳米尺度物理 · 物理学 2015-11-05 Hongyi Yu , Yong Wang , Qingjun Tong , Xiaodong Xu , Wang Yao

The emerging field of valleytronics aims to exploit the valley pseudospin of electrons residing near Bloch band extrema as an information carrier. Recent experiments demonstrating optical generation and manipulation of exciton valley…

介观与纳米尺度物理 · 物理学 2017-05-24 Kai Hao , Lixiang Xu , Fengcheng Wu , Philipp Nagler , Kha Tran , Xin Ma , Christian Schüller , Tobias Korn , Allan H. MacDonald , Galan Moody , Xiaoqin Li

We observe the interlayer A1s^I, A2s^I, and B1s^I excitons in bilayer WSe2 under applied electric fields using reflectance contrast spectroscopy. Remarkably, these interlayer excitons remain optically bright despite being well separated…

Monolayer transition metal dichalcogenides (TMDs) exhibit a remarkably strong Coulomb interaction that manifests in tightly bound excitons. Due to the complex electronic band structure exhibiting several spin-split valleys in the conduction…

The presence of two spin-split valleys in monolayer (1L) transition metal dichalcogenide (TMD) semiconductors supports versatile exciton species classified by their spin and valley quantum numbers. While the spin-0 intravalley exciton,…

介观与纳米尺度物理 · 物理学 2020-07-22 Yueh-Chun Wu , Sarath Samudrala , Andrew McClung , Takashi Taniguchi , Kenji Watanabe , Amir Arbabi , Jun Yan

In twisted homobilayer transition metal dichalcogenides, intra- and inter-layer valley excitons hybridize with the layer configurations spatially varying in the moir\'e. The ground state valley excitons are trapped at two high-symmetry…

介观与纳米尺度物理 · 物理学 2021-05-27 Hongyi Yu , Wang Yao

Monolayers of transition metal dichalcogenides (TMDCs) feature exceptional optical properties that are dominated by excitons, tightly bound electron-hole pairs. Forming van der Waals heterostructures by deterministically stacking individual…

Moir\'e superlattices of transition metal dichalcogenide (TMD) heterostructures give rise to rich excitonic phenomena associated with the interlayer twist angle and induced changes in the involved quantum states. Theoretical calculations of…

材料科学 · 物理学 2022-09-13 Sudipta Kundu , Tomer Amit , H. R. Krishnamurthy , Manish Jain , Sivan Refaely-Abramson

Two-dimensional semiconductors feature valleytronics phenomena due to locking of the spin and momentum valley of the electrons. However, the valley polarization is intrinsically limited in monolayer crystals by the fast intervalley…

介观与纳米尺度物理 · 物理学 2019-07-10 Long Zhang , Rahul Gogna , G. William Burg , Jason Horng , Eunice Paik , Yu-Hsun Chou , Kyounghwan Kim , Emanuel Tutuc , Hui Deng

Monolayer transition-metal dichalcogenides (TMDCs) have recently emerged as possible candidates for valleytronic applications, as the spin and valley pseudospin are directly coupled and stabilized by a large spin splitting. In these…

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