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Binding of anthracycline antibiotic carminomycin (CM) to synthetic polyribonucleotides poly(A) and poly(U) was studied in solution of low ionic strength in a wide phosphate-to-dye (P/D) range using absorption and polarized fluorescence…

生物物理 · 物理学 2020-06-23 N. N. Zhigalova , V. N. Zozulya , O. A. Ryazanova

Binding of neutral Pheophorbide-a methyl ester (MePheo-a) to various synthetic polynucleotides, double-stranded poly(A)-poly(U), poly(G)-poly(C) and four-stranded poly(G), as well as to calf thymus DNA, was studied using the methods of…

生物物理 · 物理学 2018-11-06 Olga Ryazanova , Victor Zozulya , Igor Voloshin , Larysa Dubey , Igor Dubey

In this study, we synthesised a phosphonium-based ligand, trimethyl(tetradecyl)phosphonium bromide (TTP-Br), and employed it in the post-synthesis surface treatment of Cs-oleate-capped CsPbBr3 NCs. The photoluminescence quantum yield (PLQY)…

Porphyrinic materials show a range of interesting and useful optical and electrical properties. The less well-known sub-class of porphyrin diacids has been used in this work to construct an ionic hybrid organic-inorganic material in…

When a chromophore interacts with titrable molecular sites, the modeling of its photophysical properties requires to take into account all their possible protonation states. We have developed a multi-scale protocol, based on constant-pH…

化学物理 · 物理学 2018-09-10 Elisa Pieri , Vincent Ledentu , Nicolas Ferré

Iridium-based photosensitizers have attracted significant attention in photodynamic therapy (PDT) due to their exceptional photophysical properties and chemical stability, as well as tunable phosphorescence emission spectrum and high…

化学物理 · 物理学 2026-05-08 Aynur Matyusup , Jia-ying Zhao , Yu-dan Zhang , Qi Zhaoa , Ai-min Ren , Jing-fu Guo

Understanding of degradation mechanisms in polymer:fullerene bulk-heterojunctions on the microscopic level aimed at improving their intrinsic stability is crucial for the breakthrough of organic photovoltaics. These materials are vulnerable…

材料科学 · 物理学 2012-01-04 Andreas Sperlich , Hannes Kraus , Carsten Deibel , Hubert Blok , Jan Schmidt , Vladimir Dyakonov

A novel type of a graphene/porphyrin hybrid with a direct covalent linker between graphene and a nickel(II) tetraphenylporphyrin unit has successfully been synthesized by the reductive exfoliation/functionalization of potassium intercalated…

化学物理 · 物理学 2018-05-24 Hui-Lei Hou , Daniela Dasler , Frank Hauke , Andreas Hirsch

Photo-physical and nonlinear-optical properties of a new amphiphilic conjugated polymer: hydroxylated pyridyl para-phenylene (Py-PhPPP) both in CH2Cl2 solution and in thin films have been investigated. By using Z-scan technique with…

材料科学 · 物理学 2007-05-23 W. Ji , Hendry Izaac Elim , Jun He , F. Fitrilawati , C. Baskar , S. Valiyaveettil , W. Knoll

The use of exogenous pulmonary surfactant (EPS) to deliver other relevant drugs to the lung is a promising strategy for combined therapy. We evaluated the interaction of polymyxin B (PxB) with clinically used EPS, the poractant alfa…

Inclusion of heavy metal atoms in a polymer backbone allows transitions between the singlet and triplet manifolds. Interfacial dissociation of triplet excitons constitutes a viable mechanism for enhancing photovoltaic (PV) efficiencies in…

材料科学 · 物理学 2009-08-10 K. Yang , U. Scherf , S. Guha

Binding of Pheophorbide-a of to poly-L-lysine (PLL) have been studied in neutral aqueous buffered solutions of low and near-physiological ionic strengths with low ethanol content (2.4-5.9 %) a wide range of molar polymer-to-dye ratios (P/D)…

生物物理 · 物理学 2021-11-30 Olga Ryazanova , Victor Zozulya , Igor Voloshin , Victor Karachevtsev

We show the possibility of tailoring the molecular arrangement, as well as the chemical and structural modifications, of porphyrins at the monolayer saturation coverage on TiO2(110) by Synchrotron photoemission, electron diffraction, STM…

On-surface metal porphyrins can undergo electronic and conformational changes that play a crucial role in determining the chemical reactivity of the molecular layer. Therefore, understanding those properties is pivotal for the design and…

Hy brid composites obtained upon blending conjugated polymers and colloidal inorganic semiconductor nanocrystals are regarded as attractive photo-active materials for optoelectronic applications. Here we demonstrate that tailoring…

Porphyrins are organic molecules that exhibit excellent opto-electronics properties, making them suitable for a variety of applications. Nevertheless, their functionality strongly depends on the surface onto which they are deposited, and on…

By applying a phase-modulation fluorescence approach to 2D electronic spectroscopy, we studied the conformation-dependent exciton-coupling of a porphyrin dimer embedded in a phospholipid bilayer membrane. Our measurements specify the…

Coordination chemistry relies on harnessing active metal sites within organic matrices. Polynuclear complexes - consisting of organic ligands binding to clusters of several metal atoms are of particular interest, owing to their…

介观与纳米尺度物理 · 物理学 2018-09-05 Cornelius Krull , Marina Castelli , Prokop Hapala , Dhaneesh Kumar , Pavel Jelinek , Agustin Schiffrin

Ruthenium(II) polypyridine compounds often have a relatively long lived triplet metalligand charge transfer (3MLCT) state, making these complexes useful as chromophores for photoactivated electron transfer in photomolecular devices (PMDs).…

化学物理 · 物理学 2025-03-05 Ala Aldin M. H. M. Darghouth , Denis Magero , Mark E. Casida

A coupling-limited approach for the Ullmann reaction-like on-surface synthesis of a two-dimensional covalent organic network starting from a halogenated metallo-porphyrin is demonstrated. Copper-octabromo-tetraphenylporphyrin molecules can…

化学物理 · 物理学 2015-02-23 Lars Smykalla , Pavel Shukrynau , Marcus Korb , Heinrich Lang , Michael Hietschold
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