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相关论文: Polaritonic Chemistry Enabled by Non-Local Metasur…

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Material characteristics and input-field specifics limit the controllability of nonlinear electromagnetic-field interactions. As these nonlinear interactions could be exploited to create strongly localized bright and dark waves, such as…

Few-photon optical nonlinearity in planar solid-state systems is challenging yet crucial for quantum and classical optical information processing. Polaritonic nonlinear metasurfaces have emerged as a promising candidate to push the photon…

We review both the fundamental aspects and the applications of functional magneto-optic and opto-magnetic metamaterials displaying collective and coupling effects on the nanoscale, where the concepts of optics and magnetism merge to produce…

材料科学 · 物理学 2020-03-12 Nicolò Maccaferri

Molecular strong coupling offers exciting prospects in physics, chemistry and materials science. Whilst attention has been focused on developing realistic models for the molecular systems, the important role played by the entire photonic…

Chiral photonics provides powerful routes for controlling the light handedness, yet nonlinear chiral responses are typically associated with intricate three-dimensional systems. Here, we demonstrate that strong nonlinear chirality can…

Under vibrational strong coupling (VSC), the formation of molecular polaritons may significantly modify the photo-induced or thermal properties of molecules. In an effort to understand these intriguing modifications, both experimental and…

化学物理 · 物理学 2022-04-07 Tao E. Li , Abraham Nitzan , Joseph E. Subotnik

Optical metamaterials and metasurfaces which emerged in the course of the last few decades have revolutionized our understanding of light and light-matter interaction. While solid materials are naturally employed as key building elements…

光学 · 物理学 2019-12-16 Shimon Rubin , Yeshaiahu Fainman

Understanding the quantum dynamics of strongly coupled molecule-cavity systems remains a significant challenge in molecular polaritonics. This work develops a comprehensive self-consistent model simulating electromagnetic interactions of…

化学物理 · 物理学 2025-01-29 Maxim Sukharev , Joseph E. Subotnik , Abraham Nitzan

Laser control of solids was so far mainly discussed in the context of strong classical nonlinear light-matter coupling in a pump-probe framework. Here we propose a quantum-electrodynamical setting to address the coupling of a…

超导电性 · 物理学 2018-07-02 Michael A. Sentef , Michael Ruggenthaler , Angel Rubio

Strong interactions between surface plasmons in ultra-compact nanocavities and excitons in two dimensional materials have attracted wide interests for its prospective realization of polariton devices at room temperature. Here, we propose a…

Sub-wavelength electromagnetic field localization has been central in photonic research in the last decade, allowing to enhance sensing capabilities as well as increasing the coupling between photons and material excitations. The…

介观与纳米尺度物理 · 物理学 2021-10-26 Shima Rajabali , Erika Cortese , Mattias Beck , Simone De Liberato , Jérôme Faist , Giacomo Scalari

Atomically thin semiconductors exhibit tunable exciton resonances that can be harnessed for dynamic manipulation of visible light in ultra-compact metadevices. However, the rapid nonradiative decay and dephasing of excitons at room…

光学 · 物理学 2025-02-18 Tom Hoekstra , Jorik van de Groep

Multiresonant metasurfaces could enable many applications in filtering, sensing and nonlinear optics. However, developing a metasurface with more than one high-quality-factor or high-Q resonance at designated resonant wavelengths is…

Sub-wavelength thick photonic crystal (PhC) slabs coupled to 2D excitonic materials, such as transition metal dichalcogenides (TMDs), are a promising platform for highly tunable, room-temperature, on-chip optoelectronic devices. Unlike…

Photonic technologies continue to drive the quest for new optical materials with unprecedented responses. A major frontier in this field is the exploration of nonlocal (spatially dispersive) materials, going beyond the local,…

Selectively exciting target molecules to high vibrational states is inefficient in the liquid phase, which restricts the use of IR pumping to catalyze ground-state chemical reactions. Here, we demonstrate that this inefficiency can…

化学物理 · 物理学 2022-12-27 Tao E. Li , Abraham Nitzan , Joseph E. Subotnik

The electromagnetic field in an optical cavity can dramatically modify and even control chemical reactivity via vibrational strong coupling (VSC). Since the typical vibration and cavity frequencies are considerably higher than thermal…

量子物理 · 物理学 2021-09-29 Peiyun Yang , Jianshu Cao

Actively tunable and reconfigurable wavefront shaping by optical metasurfaces poses a significant technical challenge often requiring unconventional materials engineering and nanofabrication. Most wavefront-shaping metasurfaces can be…

光学 · 物理学 2020-08-24 Stephanie C. Malek , Adam C. Overvig , Sajan Shrestha , Nanfang Yu

Recently in nanophotonics, a rigorous evolution from passive to active metasurfaces has been witnessed. This advancement not only brings forward interesting physical phenomena but also elicits opportunities for practical applications.…

光学 · 物理学 2023-07-21 R. Kaissner , J. X. Li , W. Z. Lu , X. Li , F. Neubrech , J. F. Wang , N. Liu

Nonlinear phononics relies on the resonant optical excitation of infrared-active lattice vibrations to coherently induce targeted structural deformations in solids. This form of dynamical crystal-structure design has been applied to control…

应用物理 · 物理学 2021-05-19 Meredith Henstridge , Michael Först , Edward Rowe , Michael Fechner , Andrea Cavalleri