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We extend the covariance-matrix description of atom--light quantum interfaces, originally developed for real and effective spin-1/2 atoms, to include "spin alignment" degrees of freedom. This allows accurate modeling of optically-probed…

We propose a powerful extension to combined molecular and spin dynamics that fully captures the coupling between the atomic and spin subsystems via spin-orbit interactions. Its foundation is the inclusion of the local magnetic anisotropies…

We present a joint experiment-theory study on the role of fluorine adatoms in spin and momentum scattering of charge carriers in dilute fluorinated graphene and bilayer graphene. The experimental spin-flip and momentum scattering rates and…

介观与纳米尺度物理 · 物理学 2019-07-24 Susanne Wellnhofer , Adam Stabile , Denis Kochan , Martin Gmitra , Ya-Wen Chuang , Jun Zhu , Jaroslav Fabian

We investigate the inelastic spin-flip rate for electrons in a quantum dot due to their contact hyperfine interaction with lattice nuclei. In contrast to other works, we obtain a spin-phonon coupling term from this interaction by taking…

介观与纳米尺度物理 · 物理学 2007-05-23 Veniamin A. Abalmassov , Florian Marquardt

We investigate spin dynamics in antiferromagnetic (AF) molecular rings at finite temperature in the presence of spin-phonon (s-p) interaction. We derive a general expression for the spin susceptibility in the weak s-p coupling limit and…

介观与纳米尺度物理 · 物理学 2009-11-11 Leonardo Spanu , Alberto Parola

The coupling between electronic spins and lattice vibrations is fundamental for driving relaxation in magnetic materials. The debate over the nature of spin-phonon coupling dates back to the 40's, but the role of spin-spin, spin-orbit and…

量子物理 · 物理学 2019-03-06 Alessandro Lunghi , Stefano Sanvito

We study theoretically the phonon-induced relaxation and decoherence of spin states of two electrons in a lateral double quantum dot in a SiGe/Si/SiGe heterostructure. We consider two types of singlet-triplet spin qubits and calculate their…

介观与纳米尺度物理 · 物理学 2018-05-29 Viktoriia Kornich , Christoph Kloeffel , Daniel Loss

We investigate the magnetic properties of a range of low-dimensional ferromagnets using a combination of first-principles calculations and atomistic spin dynamics simulations. This approach allows us to evaluate the ground state and finite…

材料科学 · 物理学 2016-11-26 Lars Bergqvist , Andrea Taroni , Anders Bergman , Corina Etz , Olle Eriksson

We propose a new universal mechanism that makes it possible to drive an individual atomic spin using a spin polarized scanning tunnel microscope (STM) with an oscillating electric signal. We show that the combination of the distance…

介观与纳米尺度物理 · 物理学 2017-11-15 J. L. Lado , A. Ferron , J. Fernandez-Rossier

We study the relaxation of the exciton spin (longitudinal relaxation time $T_{1}$) in single asymmetrical quantum dots due to an interplay of the short--range exchange interaction and acoustic phonon deformation. The calculated relaxation…

介观与纳米尺度物理 · 物理学 2009-11-10 E. Tsitsishvili , R. v. Baltz , H. Kalt

We employ the method of the theory of open quantum systems to analyze spin relaxation and decoherence in semiconductors in the presence of a magnetic field. We derive a set of Bloch equations for electron spin with a fully microscopic…

凝聚态物理 · 物理学 2007-05-23 Vadim I. Puller , Lev G. Mourokh , Norman J. M. Horing , Anatoly Yu. Smirnov

We study the spin-phonon relaxation rate of both Kramers and non-Kramers molecular magnets in strongly diluted samples at low temperature. Using the "rotational" contribution to the spin-phonon Hamiltonian, universal formulae for the…

强关联电子 · 物理学 2018-01-31 Le Tuan Anh Ho , Liviu F. Chibotaru

Nuclear spins owe their long-lived magnetic states to their excellent isolation from the environment. At the same time, a finite degree of interaction with their surroundings is necessary for reading and writing the spin state. Therefore,…

Molecular vibrations are increasingly seen as a key factor for spin dynamics in single-ion magnets and molecular spin qubits. Herein we show how an inexpensive combination of molecular dynamics calculations and a crystal field analysis can…

介观与纳米尺度物理 · 物理学 2018-08-10 Lorena E. Rosaleny , Kirill Zinovjev , Iñaki Tuñón , Alejandro Gaita-Ariño

The possibility of transporting spin information over long distances in graphene, owing to its small intrinsic spin-orbit coupling (SOC) and the absence of hyperfine interaction, has led to intense research into spintronic applications.…

介观与纳米尺度物理 · 物理学 2018-05-01 Dinh Van Tuan , Frank Ortmann , David Soriano , Sergio O. Valenzuela , Stephan Roche

Special arrangements of atoms with more than one atom per unit cell, including honeycomb or kagome (woven bamboo mat) lattices, can host propagating excitations with non-trivial topology as defined by their evolution along closed paths in…

Paramagnetic molecules can show long spin-coherence times, which make them good candidates as quantum bits. Reducing the efficiency of the spin-phonon interaction is the primary challenge towards achieving long coherence times over a wide…

Electron spin decoherence caused by elastic spin-phonon processes is investigated comprehensively in a zero-dimensional environment. Specifically, a theoretical treatment is developed for the processes associated with the fluctuations in…

其他凝聚态物理 · 物理学 2009-11-11 Y. G. Semenov , K. W. Kim

Although silicon is a promising material for quantum computation, the degeneracy of the conduction band minima (valleys) must be lifted with a splitting sufficient to ensure formation of well-defined and long-lived spin qubits. Here we…

介观与纳米尺度物理 · 物理学 2013-07-01 C. H. Yang , A. Rossi , R. Ruskov , N. S. Lai , F. A. Mohiyaddin , S. Lee , C. Tahan , G. Klimeck , A. Morello , A. S. Dzurak

We present a generally applicable parameter-free first-principles method to determine electronic spin relaxation times and apply it to the technologically important group-IV materials silicon, diamond and graphite. We concentrate on the…

介观与纳米尺度物理 · 物理学 2012-09-19 Oscar D. Restrepo , Wolfgang Windl